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arXiv:2007.00404 · Physical Review Letters

Quantum Droplets of Dipolar Mixtures

R. N. Bisset, Luis A. Peña Ardila, Luis Santos

Published Jan 13, 2021• 109 citations
arXivHTMLPDF

Abstract

Recently achieved two-component dipolar Bose-Einstein condensates open exciting possibilities for the study of mixtures of ultradilute quantum liquids. While nondipolar self-bound (without external confinement) mixtures are necessarily miscible with an approximately fixed ratio between the two densities, the density ratio for the dipolar case is free. Therefore, self-bound dipolar mixtures present qualitatively novel and much richer physics, characterized by three possible ground-state phases: miscible, symmetric immiscible, and asymmetric immiscible, which may in principle occur at any population imbalance. Self-bound immiscible droplets are possible due to mutual nonlocal intercomponent attraction, which results in the formation of a droplet molecule. Moreover, our analysis of the impurity regime shows that quantum fluctuations in the majority component crucially modify the miscibility of impurities. Our work opens intriguing perspectives for the exploration of spinor physics in ultradilute liquids, which should resemble to some extent that of ^{4}He-^{3}He droplets and impurity-doped helium droplets.

DOI
10.1103/physrevlett.126.025301

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Recently achieved two-component dipolar Bose-Einstein condensates open exciting possibilities for the study of mixtures of ultradilute quantum liquids. While nondipolar self-bound (without external confinement) mixtures are necessarily miscible with an approximately fixed ratio between the two densities, the density ratio for the dipolar case is free. Therefore, self-bound dipolar mixtures present qualitatively novel and much richer physics, characterized by three possible ground-state phases: miscible, symmetric immiscible, and asymmetric immiscible, which may in principle occur at any population imbalance. Self-bound immiscible droplets are possible due to mutual nonlocal intercomponent attraction, which results in the formation of a droplet molecule. Moreover, our analysis of the impurity regime shows that quantum fluctuations in the majority component crucially modify the miscibility of impurities. Our work opens intriguing perspectives for the exploration of spinor physics in ultradilute liquids, which should resemble to some extent that of ^{4}He-^{3}He droplets and impurity-doped helium droplets.
The recent realization of a binary dipolar Bose-Einstein condensate [A. Trautmann et al., Phys. Rev. Lett. 121, 213601 (2018)] presents new exciting aspects for studying quantum droplets and supersolids in a binary mixture. Motivated by this experiment, we study the ground-state phases and dynamics of a Dy-Dy mixture. The dipolar bosonic mixture exhibits qualitatively novel and rich physics. Relying on the three-dimensional numerical simulations in the extended Gross-Pitaevskii framework, we unravel the ground-state phase diagrams and characterize their different possible phases. The emergent phases include single-droplet (SD), multiple-droplets (MD), doubly supersolid (SS), and superfluid (SF) states in both miscible and immiscible phases. Intriguing mixed ground states are observed for an imbalanced binary mixture, including a combination of SS-SF, SS-MD, and SS-SS phases. We also explore the dynamics across the phase boundaries by linear quenches of interspecies and intraspecies scattering lengths. During these dynamical processes, we observe an abrupt change in phase which initially results in some instability in the system and forms some metastable states in the intermediate timescale. However, the state produced in long-time evolution is similar to our predicted ground state. Although we demonstrate the possible results for a Dy-Dy mixture and for a specific parameter range of intraspecies and interspecies scattering lengths, our results are in general valid for other dipolar mixtures and may become an important benchmark for future experimental scenarios.
Combining two Bose-Einstein condensates (BECs) may result in a miscible or immiscible mixture, or even a violent implosion. We theoretically demonstrate that dipolar two-component BECs produce far richer physics than their nondipolar counterparts. Intriguingly, when both components have equivalent dipoles, the transition to immiscibility is largely unaffected by dipolar physics, yet the dipoles maximally affect stability. Conversely, antiparallel dipoles strongly affect miscibility but have little effect on stability. By performing three-dimensional calculations of the ground states and their excitations, we find strong dependencies on the confinement geometry. We explore and elucidate the various phononic and rotonic phase transitions, as well as symmetry-preserving crossovers.
These lecture notes contain an introduction to quantum simulation of bosonic systems in the continuum, focusing on weakly interacting Bose-Bose mixtures with competing mean-field interactions. When the values of such interactions are fine-tuned to almost completely cancel the mean-field energy, quantum fluctuations become apparent and dominate the behavior of the system, stabilizing an ultradilute quantum liquid phase. An analogous situation appears in single-component dipolar quantum gases. We review the mechanism that gives rise to this exotic quantum liquid, which can form droplets that are self-bound in the absence of any external confinement, and discuss their properties and dynamics in both the mixture and the dipolar cases. In dipolar gases, arrays of dipolar droplets stabilized by quantum fluctuations can establish global phase coherence and form supersolids. In bosonic mixtures, supersolidity can emerge already at the mean-field level through spin-orbit coupling. We discuss the properties of such spin-orbit-coupled supersolids, comparing them to their dipolar counterparts. Specifically, we focus on their periodic density modulation, phase coherence, and peculiar excitation spectrum, which hosts both superfluid and crystal excitations. Finally, we conclude by discussing open research directions in the areas of quantum liquid droplets and spin-orbit-coupled supersolids, in particular at the interface of the two research topics.
Quantum droplets are a quantum analog to classical fluid droplets in that they are self-bound and display liquid-like properties---such as incompressibility and surface tension---though their stability is the result of quantum fluctuations. One of the major systems for observing quantum droplets is two-component Bose gases. Two-component droplets are typically considered to be balanced, having a fixed ratio between the densities of the two components. This work goes beyond the fixed density ratio by investigating spherical droplets in imbalanced mixtures. With increasing imbalance, the droplet is able to lower its energy up to a limit, at which point the droplet becomes saturated with the atoms of the majority component and any further atoms added to this component cannot bind to the droplet. Analyzing the breathing mode dynamics of imbalanced droplets indicates that the droplet can emit particles, as in balanced mixtures, but the imbalance leads to an intricate superposition of multiple simultaneously decaying collective oscillations.
We analyze the physics of self-bound droplets in a doubly dipolar Bose-Einstein condensate composed by particles with both electric and magnetic dipole moments. Using the particularly relevant case of dysprosium, we show that the anisotropy of the doubly dipolar interaction potential is highly versatile and nontrivial, depending critically on the relative orientation and strength between the two dipole moments. This opens novel possibilities for exploring intriguing quantum many-body physics. Interestingly, by varying the angle between the two dipoles we find a dimensional crossover from quasi-one-dimensional to quasi-two-dimensional self-bound droplets. This opens a so far unique scenario in condensate physics, in which a dimensional crossover is solely driven by interactions in the absence of any confinement.
Quantum droplets are small clusters of atoms self-bound by the balance of attractive and repulsive forces. Here, we report on the observation of droplets solely stabilized by contact interactions in a mixture of two Bose-Einstein condensates. We demonstrate that they are several orders of magnitude more dilute than liquid helium by directly measuring their size and density via in situ imaging. We show that the droplets are stablized against collapse by quantum fluctuations and that they require a minimum atom number to be stable. Below that number, quantum pressure drives a liquid-to-gas transition that we map out as a function of interaction strength. These ultradilute isotropic liquids remain weakly interacting and constitute an ideal platform to benchmark quantum many-body theories.