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arXiv:2006.06588

Insulating, metallic and superconducting behavior in a single nanowire

Jan Nicolas Voss, Yannick Schön, Micha Wildermuth, Dominik Dorer, Jared H. Cole, Hannes Rotzinger, Alexey Vladimirovich Ustinov

Published Jun 11, 2020• 0 citations
arXivHTMLPDF

Abstract

In systems with reduced dimensions quantum fluctuations have a strong influence on the electronic conduction, even at very low temperature. In superconductors this is especially interesting, since the coherent state of the superconducting electrons is strongly interacting with these fluctuations and therefore is a sensitive tool to study them. In this paper, we report on comprehensive measurements of superconducting nanowires in the quantum phase slip regime. Using an intrinsic electromigration process, we have developed a method to lower the resistance of lithographically fabricated highly resistive nanowires in situ and in small consecutive steps. At low temperature we observe critical (Coulomb) blockade voltages and superconducting critical currents, depending on the nanowire's normal-state resistance, in good agreement with theoretical models. Between these two regimes, we find a continuous transition displaying a nonlinear metallic-like behavior. The reported intrinsic electromigration technique is not limited to low temperatures as we find a similar change in resistance that spans over three orders of magnitude also at room temperature. Aside from superconducting quantum circuits, such a technique to reduce the resistance may also have applications in modern electronic circuits.

DOI
10.48550/arxiv.2006.06588

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In systems with reduced dimensions quantum fluctuations have a strong influence on the electronic conduction, even at very low temperature. In superconductors this is especially interesting, since the coherent state of the superconducting electrons is strongly interacting with these fluctuations and therefore is a sensitive tool to study them. In this paper, we report on comprehensive measurements of superconducting nanowires in the quantum phase slip regime. Using an intrinsic electromigration process, we have developed a method to lower the resistance of lithographically fabricated highly resistive nanowires in situ and in small consecutive steps. At low temperature we observe critical (Coulomb) blockade voltages and superconducting critical currents, depending on the nanowire's normal-state resistance, in good agreement with theoretical models. Between these two regimes, we find a continuous transition displaying a nonlinear metallic-like behavior. The reported intrinsic electromigration technique is not limited to low temperatures as we find a similar change in resistance that spans over three orders of magnitude also at room temperature. Aside from superconducting quantum circuits, such a technique to reduce the resistance may also have applications in modern electronic circuits.
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We present a detailed report of microwave irradiation of ultranarrow superconducting nanowires. In our nanofabricated circuits containing a superconducting NbSi nanowire, a dc blockade of current flow was observed at low temperatures below a critical voltage Vc{V}_{\mathrm{c}}Vc​, a strong indicator of the existence of quantum phase-slip (QPS) in the nanowire. We describe the results of applying microwaves to these samples, using a range of frequencies and both continuous-wave and pulsed drive, in order to search for dual Shapiro steps which would constitute an unambiguous demonstration of quantum phase-slip. We observed no steps, and our subsequent thermal analysis suggests that the electron temperature in the series CrO resistors was significantly elevated above the substrate temperature, resulting in sufficient Johnson noise to wash out the steps. To understand the system and inform future work, we have constructed a numerical model of the dynamics of the circuit for dc and ac bias (both continuous-wave and pulsed drive signals) in the presence of Johnson noise. Using this model, we outline important design considerations for device and measurement parameters which should be used in any future experiment to enable the observation of dual Shapiro steps at experimentally accessible temperatures and, thus, lead to the development of a QPS-based quantum current standard.
Abstract Quantum phase slip (QPS) is an important effect that occurs in one-dimensional (1D) or quasi-1D superconducting (SC) materials. Due to the extremely high requirements on the uniformity and quality of SC nanowires, it is currently very challenging to obtain repeatable and controllable QPS devices. Here, we report a systematic study of the QPS effect in NbN SC nanowires. High-quality NbN nanowires with different widths are fabricated by combining the processes of photo-lithography, electron beam lithography, and inductively coupled plasma etching. It is found that the electrical transport of the nanowires showed a systematic variation with the wire width, and a clear evolution from single to multiple QPS events with the decrease in wire width is uncovered at low temperatures. Based on these experimental results, the phase diagram reflecting the evolution of the physical states of the nanowires with wire width and temperature is obtained. In addition, we observed the features of the critical voltage, which is a characteristic of the occurrence of coherent QPS (cQPS), in samples with a width of 36 nm in the multiple QPS region. It is worth noting that this cQPS behavior was detected in a non-high-impedance environment.
The topic of superconducting nanowires has recently been an interesting field of research which has included the study of the superconductor to insulator transition (SIT), the observation of macroscopic quantum behavior such as quantum phase slips (QPS), and the potential use of nanowires as qubits. Superconducting coplanar microwave waveguide resonators have also become a popular way of studying superconducting junctions and qubits, as they provide an extremely low noise environment. For example, superconducting two-dimensional Fabry-Perot resonators have been used by other groups to make non-demolition measurements of a qubit. The motivation of this thesis will be the merging of the fields of superconducting nanowires and the technique of using superconducting microwave resonators to study junctions by incorporating a nanowire into the resonator itself at a current anti-node. By doing this, the nonlinear effects of the nanowire can be studied which may find application in single photon detectors, mixers, and the readout of qubits. We also employ the technique of molecular templating to fabricate some of the thinnest superconducting nanowires ever studied (down to ~ 5 nm in diameter in some cases). In this thesis, we extend the understanding of the nonlinear properties of a nanowire- resonator system and investigate a new type of nonlinearity that involves a pulsing regime between the superconducting and normal phases of the nanowire. We develop a model, which describes the results quantitatively and by modeling the system, we are able to extract information regarding the relaxation time of the nanowire back into the superconducting state. We also study double nanowire-resonator systems where two closely spaced parallel nanowires interrupt the resonator center conductor and form a loop where vortex tunneling processes can occur. Using a double nanowire-resonator we are able to observe the Little-Parks effect at low temperatures (where the resistance of the wires is immeasurably low) and are able to confirm the multivalued nature of the current phase relationship (CPR) in nanowires. Additionally, we observe an anomalous transmission regime where the periodic pulsing is replaced by stochastic amplitude fluctuations. In addition to microwave measurements on nanowires, we also study the normal state in resistively shunted nanowires with dc measurements where the inclusion of a shunt resistor is observed to change the nature of the normal state from the Joule heated state to a state that preserves phase coherence. Finally, the statistics on switching current events in graphene proximity junctions are analyzed and compared to the well known results for Josephson junctions. Only thermal activation (and no macroscopic quantum tunneling) is observed in graphene proximity superconducting junctions down to temperatures of ~ 300 mK.
Quantum phase transitions typically result in a broadened critical or crossover region at nonzero temperature. Josephson arrays are a model of this phenomenon, exhibiting a superconductor-insulator transition at a critical wave impedance, and a well-understood insulating phase. Yet high-impedance arrays used in quantum computing and metrology apparently evade this transition, displaying superconducting behavior deep into the nominally insulating regime. The absence of critical behavior in such devices is not well understood. Here we show that, unlike the typical quantum-critical broadening scenario, in Josephson arrays temperature dramatically shifts the critical region. This shift leads to a regime of superconductivity at high temperature, arising from the melted zero-temperature insulator. Our results quantitatively explain the low-temperature onset of superconductivity in nominally insulating regimes, and the transition to the strongly insulating phase. We further present, to our knowledge, the first understanding of the onset of anomalous-metallic resistance saturation. This work demonstrates a non-trivial interplay between thermal effects and quantum criticality. A practical consequence is that, counterintuitively, the coherence of high-impedance quantum circuits is expected to be stabilized by thermal fluctuations.
At low temperatures non-equilibrium voltage fluctuations can be generated in current-biased superconducting nanowires due to proliferation of quantum phase slips (QPS) or, equivalently, due to quantum tunneling of magnetic flux quanta across the wire. In this paper we review and further extend recent theoretical results related to this phenomenon. Employing the phase-charge duality arguments combined with Keldysh path integral technique we analyze such fluctuations within the two-point and four-point measurement schemes demonstrating that voltage noise detected in such nanowires in general depends on the particular measurement setup. In the low frequency limit we evaluate all cumulants of the voltage operator which turn out to obey Poisson statistics and exhibit a power law dependence on the external bias. We also specifically address a non-trivial frequency dependence of quantum shot noise power spectrum SΩ for both longer and shorter superconducting nanowires. In particular, we demonstrate that SΩ decreases with increasing frequency Ω and vanishes beyond a threshold value of Ω at T → 0. Furthermore, we predict that SΩ may depend non-monotonously on temperature due to quantum coherent nature of QPS noise. The results of our theoretical analysis can be directly tested in future experiments with superconducting nanowires.