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arXiv:2006.06228 · Physical Review Research

Observation of a strongly ferromagnetic spinor Bose-Einstein condensate

SeungJung Huh, Kyungtae Kim, Kiryang Kwon, Jae-yoon Choi

Published Sep 23, 2020• 45 citations
arXivHTMLPDF

Abstract

We report the observation of strongly ferromagnetic F = 1 spinor Bose-Einstein condensates of 7 Li atoms.The condensates are generated in an optical dipole trap without using magnetic Feshbach resonances, so that the condensates have internal spin degrees of freedom.Studying the nonequilibrium spin dynamics, we have measured the ferromagnetic spin interaction energy and determined the s-wave scattering length difference among total spin f channels to be a f =2a f =0 = -18(3) Bohr radius.This strong collision-channel dependence leads to a large variation in the condensate size with different spin composition.We were able to excite a radial monopole mode after a spin-flip transition between the |m F = 0 and |m F = 1 spin states.From the experiments, we estimated the scattering length ratio a f =2 /a f =0 = 0.27(6), and determined a f =2 = 7(2) and a f =0 = 25(5) Bohr radii, respectively.The results indicate the spin-dependent interaction energy of our system is as large as 46% of the condensate chemical potential.

DOI
10.1103/physrevresearch.2.033471

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We report the observation of strongly ferromagnetic F = 1 spinor Bose-Einstein condensates of 7 Li atoms.The condensates are generated in an optical dipole trap without using magnetic Feshbach resonances, so that the condensates have internal spin degrees of freedom.Studying the nonequilibrium spin dynamics, we have measured the ferromagnetic spin interaction energy and determined the s-wave scattering length difference among total spin f channels to be a f =2a f =0 = -18(3) Bohr radius.This strong collision-channel dependence leads to a large variation in the condensate size with different spin composition.We were able to excite a radial monopole mode after a spin-flip transition between the |m F = 0 and |m F = 1 spin states.From the experiments, we estimated the scattering length ratio a f =2 /a f =0 = 0.27(6), and determined a f =2 = 7(2) and a f =0 = 25(5) Bohr radii, respectively.The results indicate the spin-dependent interaction energy of our system is as large as 46% of the condensate chemical potential.
Bose-Einstein condensation (BEC) is a phenomenon in which identical bosons occupy the same quantum state below a certain critical temperature. A hallmark of BEC is the coherence between particles every particle shares the same quantum wavefunction and phase. This coherence has been demonstrated for the external (motional) degrees of freedom of the atomic condensates by interfering two condensates. In this thesis, the coherence is shown to extend to the internal spin degrees of freedom of a spin-1 Bose gas evidenced by the observed coherent and reversible spin-changing collisions. The observed coherent dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. Control of the coherent evolution of the system using magnetic fields is also demonstrated. The studies on spinor condensates begin by creating spinor condensates directly using all-optical approaches that were first developed in our laboratory. All-optical formation of Bose-Einstein condensates (BEC) in 1D optical lattice and single focus trap geometries are developed and presented. These techniques offer considerable flexibility and speed compared to magnetic trap approaches, and the trapping potential can be essentially spin-independent and are ideally suited for studying spinor condensates. Using condensates with well-defined initial non-equilibrium spin configuration, spin mixing of F = 1 and F = 2 spinor condensates of rubidium-87 atoms confined in an optical trap is observed. The equilibrium spin configuration in the F = 1 manifold confirms that 87Rb is ferromagnetic. The coherent spinor dynamics are demonstrated by initiating spin mixing deterministically with a non-stationary spin population configuration. Finally, the interplay between the coherent spin mixing and spatial dynamics in spin-1 condensates with ferromagnetic interactions is investigated.
The achievement of a Bose-Einstein condensate of cesium in the lowest internal state (F=3, m/sub F/=3) by evaporative cooling in an optical trap is reported. The corresponding scattering length shows a strong dependence on magnetic field, varying from large negative to large positive values in a conveniently accessible magnetic field range due to a unusual combination of broad and narrow Feshbach resonances. The inelastic processes resulting from this complex scattering behavior in thermal ensembles is studied. These measurements have been of crucial importance for identifying a suitable path in phase space towards condensation. In first experiments, the strong dependence of the condensate mean-field energy on the magnetic field is demonstrated. By briefly switching to different scattering lengths just before releasing the sample from the trap, imploding, exploding, and non-interacting 'frozen' condensates are produced. We will employ the tunable interaction in further experiments by looking at molecule formation on Feshbach resonances and exploring condensate dynamics at extreme values of the scattering length.
The achievement in cooling alkali atomic gases, such as 87^{87}87Rb, 23^{23}23Na and 7^{7}7Li, to quantum degeneracy opens up a way to study magnetism in spinor bosons, because these constituent atoms usually have a hyperfine spin degree of freedom. This article reviews several basic problems related to the ferromagnetic phase transition in spinor atomic Bose gases from a theoretical perspective. After a brief discussion on various possible origins of the ferromagnetic interaction, the phase diagram of the ferromagnetically coupled spinor bosons is investigated. It is found that the ferromagnetic transition occurs always above Bose-Einstein condensation and the Bose condensate is fully polarized. The low-lying collective excitations of the spinor condensate, including spin and density modes, are discussed. The spectrum of the density mode is of the Bogliubov form and the spin wave spectrum has a k2k^2k2-formed dispersion relation at long wavelengths. The spin-wave stiffness coefficient contains contribut
We describe a compact, robust and versatile system for studying the macroscopic spin dynamics in a spinor Bose–Einstein condensate. Condensates of are produced by all-optical evaporation in a 1560 nm optical dipole trap, using a non-standard loading sequence that employs an ancillary 1529 nm beam for partial compensation of the strong differential light-shift induced by the dipole trap itself. We use near-resonant Faraday rotation probing to non-destructively track the condensate magnetization, and demonstrate few-Larmor-cycle tracking with no detectable degradation of the spin polarization. In the ferromagnetic F = 1 ground state, we observe the spin orientation between atoms in the condensate is preserved, such that they precess all together like one large spin in the presence of a magnetic field. We characterize this dynamics in terms of the single-shot magnetic coherence times and , and observe them to be of several seconds, limited only by the residence time of the atoms in the trap. At the densities used, this residence is restricted only by one-body losses set by the vacuum conditions.
We use a Feshbach resonance to tune the scattering length a of a Bose-Einstein condensate of 7Li in the |F=1,mF=1> state. Using the spatial extent of the trapped condensate, we extract a over a range spanning 7 decades from small attractive interactions to extremely strong repulsive interactions. The shallow zero crossing in the wing of the Feshbach resonance enables the determination of a as small as 0.01 Bohr radii. Evidence of the weak anisotropic magnetic dipole interaction is obtained by comparison with different trap geometries for small a.
We report the observation of matter-wave jet emission in a strongly ferromagnetic spinor Bose-Einstein condensate of ^{7}Li atoms. Directional atomic beams with |F=1,m_{F}=1⟩ and |F=1,m_{F}=-1⟩ spin states are generated from |F=1,m_{F}=0⟩ state condensates or vice versa. This results from collective spin-mixing scattering events, where spontaneously produced pairs of atoms with opposite momentum facilitates additional spin-mixing collisions as they pass through the condensates. The matter-wave jets of different spin states (|F=1,m_{F}=±1⟩) can be a macroscopic Einstein-Podolsky-Rosen state with spacelike separation. Its spin-momentum correlations are studied by using the angular correlation function for each spin state. Rotating the spin axis, the inter- and intraspin-momentum correlation peaks display a high-contrast oscillation, indicating collective coherence of the atomic ensembles. We provide numerical calculations that describe the experimental results at a quantitative level. Our Letter paves the way to generating macroscopic quantum entanglement with the spin and motional degree of freedom with massive particles. It has a wide range of applications from quantum information science to the fundamental studies of quantum entanglement.