The addition of a weak oscillating field modifying strongly dressed spins enhances and enriches the system quantum dynamics. Through low-order harmonic mixing, the bichromatic driving generates additional rectified static field acting on the spin system. The secondary field allows for a fine tuning of the atomic response and produces effects not accessible with a single dressing field, such as a spatial triaxial anisotropy of the spin coupling constants and acceleration of the spin dynamics. This tuning-dressed configuration introduces an extra handle for the system full engineering in quantum control applications. Tuning amplitude, harmonic content, spatial orientation, and phase relation are control parameters. A theoretical analysis, based on perturbative approach, is experimentally tested by applying a bichromatic radiofrequency field to an optically pumped Cs atomic vapour. The theoretical predictions are precisely confirmed by measurements performed with tuning frequencies up to the third harmonic.
The addition of a weak oscillating field modifying strongly dressed spins enhances and enriches the system quantum dynamics. Through low-order harmonic mixing, the bichromatic driving generates additional rectified static field acting on the spin system. The secondary field allows for a fine tuning of the atomic response and produces effects not accessible with a single dressing field, such as a spatial triaxial anisotropy of the spin coupling constants and acceleration of the spin dynamics. This tuning-dressed configuration introduces an extra handle for the system full engineering in quantum control applications. Tuning amplitude, harmonic content, spatial orientation, and phase relation are control parameters. A theoretical analysis, based on perturbative approach, is experimentally tested by applying a bichromatic radiofrequency field to an optically pumped Cs atomic vapour. The theoretical predictions are precisely confirmed by measurements performed with tuning frequencies up to the third harmonic.
Controlled modifications of the quantum magnetic response are produced in dressed systems by a high frequency, strong and not-resonant electromagnetic field. This quantum control is greatly enhanced and enriched by the harmonic, commensurable and orthogonally oriented dual dressing theoretically discussed here. The secondary field enables a fine tuning of the qubit response, with control parameters amplitude, harmonic content, spatial orientation and phase relation. Our analysis is based on a perturbative approach and includes few numerical solutions. The long-time dynamics is described in terms of an anisotropic effective static magnetic field representing the handle for the system full engineering. Through a low-order harmonic mixing the bichromatic driving generates a rectified static field acting on the spin. The Zeeman response becomes anisotropic in a triaxial geometry and includes a quadratic contribution. Our dressing increases the two-level energy splitting, improving the spin detection sensitivity. On the low field direction it compensates the static fields applied in different geometries. A resonant spin exchange between two species having very different magnetic response as electron and nucleus is allowed by the dressing. The spin temporal evolution includes a micromotion at harmonics of the driving frequency whose role in the spin detection is examined and can be exploited in quantum information. The results presented here lay a foundation for additional applications to be harnessed in quantum simulations.
Controlled modifications of the magnetic response of a two-level system are produced in dressed systems by one high-frequency, strong, and nonresonant electromagnetic field. This quantum control is greatly enhanced and enriched by a harmonic, commensurable, and orthogonally oriented dual dressing, as discussed here. The secondary field enables a fine tuning of the qubit response, with control parameter amplitude, harmonic content, spatial orientation, and phase relation. Our analysis, mainly based on a perturbative approach with respect to the driving strength, includes also nonperturbative numerical solutions. The Zeeman response becomes anisotropic in a triaxial geometry and includes a nonlinear quadratic contribution. The long-time dynamics is described by an anisotropic effective magnetic field representing the handle for the system full engineering. Through the low-order harmonic mixing, the bichromatic driving generates a synthetic static field modifying the system dynamics. The spin temporal evolution includes a micromotion at harmonics of the driving frequency whose role in the spin detection is examined. Our dressing increases the two-level energy splitting, improving the spin detection sensitivity. In the weak-field direction it compensates the static fields applied in different geometries. The results presented here lay a foundation for additional applications to be harnessed in quantum simulations.
The application of nonresonant electromagnetic fields, a technique known as 'dressing', provides critical control over the properties of fundamental quantum systems. We investigate the time evolution of a dressed-atom coherent spin ensemble, effectively representing a qubit, driven by a non-resonant electromagnetic field with two components, one along the quantisation static magnetic field and the other one orthogonal to it. While this second component produces a Larmor precession of the spin, the longitudinal dressing modifies the instantaneous field value, leading to a frequency modulated temporal evolution of the spin. This dual-dressing configuration represents an extension of the Landau-Zener multipassage interferometry in the presence of an additional dressing field controlling the tunneling process by its amplitude and phase. Our measurement of the qubit coherence introduces additional features to the transition probability readout of standard interferometry. The coherence time evolution is characterized by oscillations at several frequencies, each of them produced by a different quantum contribution. Such frequency description introduces a new picture of the qubit multipassage evolution. Our tuning-dressed configuration expands the toolbox for quantum state manipulation and quantum control applications. The experiments are performed in rubidium and caesium atomic magnetometers, confined in a magneto-optical trap and in a vapour cell, respectively. Static fields in the μT range and kHz oscillating fields with large Rabi frequencies are applied. Because the present low-frequency dressing operation does not fall within the standard Floquet engineering paradigm based on the high-frequency expansion, we develop an ad-hoc dressing perturbation treatment. Numerical simulations support the adiabatic and non-adiabatic qubit evolution.
The application of a periodic nonresonant drive to a system allows the Floquet engineering of effective fields described by a broad class of quantum simulated Hamiltonians. The Floquet evolution is based on two different elements. The first one is a time-independent or stroboscopic evolution with an effective Hamiltonian corresponding to the quantum simulation target. The second element is the time evolution at the frequencies of the nonresonant driving and of its harmonics, denoted as micromotion. We examine experimentally and theoretically the harmonic dual-dressing Floquet engineering of a cold atomic two-level sample. Our focus is the dressing operation with small bare energies and large Rabi frequencies, where frequencies and amplitudes of the stroboscopic/micromotion time evolutions are comparable. At the kHz range of our dressed atom oscillations, we probe directly both the stroboscopic and micromotion components of the qubit global time evolution. We develop ad-hoc monitoring tools of the Floquet space evolution. The direct record of the time evolution following a pulsed excitation demonstrates the interplay between the two components of the spin precession in the Floquet space. From the resonant pumping of the dressed system at its evolution frequencies, Floquet eigenenergy spectra up to the fifth order harmonic of the dressing frequency are precisely measured as function of dressing parameters. Dirac points of the Floquet eigenenergies are identified and, correspondingly, a jump in the dynamical phase shift is measured. The stroboscopic Hamiltonian eigenfrequencies are measured also from the probe of the micromotion sidebands.These monitoring tools are appropriate for quantum simulation/computation investigations. Our results evidence that the stroboscopic phase shift of the qubit wavefunction contains an additional information that opens new simulation directions.
We report the observation of electron spin interactions between Rydberg atoms, which are driven by spin-orbit coupling through second-order dipole perturbation and exhibit a spatial anisotropy governed by the atomic configuration. Specifically, we observe coherent electron spin exchange dynamics, with the measured coupling strength agreeing well with both numerical calculations and theoretical models. Furthermore, we show that global microwave dressing enables active engineering and dynamical freezing of the spin exchange by introducing a differential AC Stark shift between the participating states. Additionally, we achieve tunability of the interaction by applying a stronger magnetic field, which effectively modifies the energy contributions of the underlying spin-orbit coupling channels. Finally, measuring spin dynamics in one-dimensional multi-atom chains aligned parallel or perpendicular to the magnetic field provides a self-consistent validation of the anisotropic XXZ framework. This electron spin interaction natively features spin-position coupling and enables a natural mapping onto the Heisenberg-Kitaev model. Our findings reveal a new class of electron spin-spin interactions among Rydberg atoms, expanding the scope of quantum simulation with Rydberg atom arrays.
Quantum systems with multiharmonic dressing have been extensively investigated and exhibited various novel phenomena and technologies by virtue of their robust electromagnetic response. Here we mainly investigate the self-generated longitudinal Floquet modulation phenomenon of an alignment-based magnetic-resonance system with pump-probe structure dressed by two different transverse radio-frequency (rf) fields in a warm atomic cesium ensemble, both theoretically and experimentally. The self-generated Floquet modulation includes first and second harmonics, which are contributed to by linear and nonlinear processes from the weak-dressed field, respectively. The self-generated Floquet modulation dresses the alignment absorption spectra into two continua. The asymmetry of each dressed continuum is due to the generalized parity symmetry of the system being broken by the second harmonic modulation. Moreover, the nonlinear modification effect of the weak rf field on the probe verifies the existence of the four-wave mixing process in the rf band. The analytical expression, establishment process, and asymmetry analysis of the continua are given concisely. Our results can be applied to the fields of precision magnetic-field measurement, quantum control, quantum simulation, and so on. In addition, because the physical mechanism is universal, it can be applied not only to an atomic ensemble, but also to solid-state devices.