Precise measurement of the angular deviation of an object is a common task in science and technology. Many methods use light for this purpose. Some of these exploit interference effects to achieve technological advantages, such as amplification effects, or simplified measurement devices. However, all of these schemes require phase stability to be useful. Here we show theoretically and experimentally that this drawback can be lifted by utilizing two-photon interference, which is known to be less sensitive to phase fluctuations. Our results show that nonclassical interference can provide a path towards robust interferometric sensing, allowing for increased metrological precision in the presence of phase noise.
Precise measurement of the angular deviation of an object is a common task in science and technology. Many methods use light for this purpose. Some of these exploit interference effects to achieve technological advantages, such as amplification effects, or simplified measurement devices. However, all of these schemes require phase stability to be useful. Here we show theoretically and experimentally that this drawback can be lifted by utilizing two-photon interference, which is known to be less sensitive to phase fluctuations. Our results show that nonclassical interference can provide a path towards robust interferometric sensing, allowing for increased metrological precision in the presence of phase noise.
Optical quantum metrology uses specially-prepared states of light to probe sensitive samples. Choosing a suitable probe state allows one to extract more information per probe photon about an unknown parameter than is possible using any classical technique. In effect, these techniques improve the sensitivity of the measurement whenever the number of probe photons is constrained in some way. This thesis presents experimental and theoretical results on the use of pairs of time-frequency entangled photons in precision measurements. It begins with an overview of necessary background knowledge about quantum optics and quantum information. This is followed by a theoretical discussion on the estimation of a single delay using two-photon interference. We show that constraints on the probe photon's bandwidth complicate the measurement problem, requiring suitable optimization of the two-photon quantum state to avoid losing precision. We then consider the use of two-photon interference for linear spectroscopic measurements. Linear spectroscopy relates the absorption and phase spectrum of a sample to unknown electronic parameters. We describe a proof-of-principle experiment demonstrating that two-photon interferometric spectroscopy can be used for simultaneously measurement of both absorption and phase. This is followed by an information-theoretic discussion of the precision of this technique. For low losses, we show that the method provides phase sensitivity similar to classical interferometry while approaching the optimal absorption precision of any possible measurement. If the absorption and phase values are both related to a single unknown parameter, then our technique provides improved sensitivity to this parameter compared to both classical measurements and other quantum techniques in the presence of realistic levels of loss. We conclude with a discussion of quantum-optical coherence tomography, which is a two-photon interferometric method for determining the material structure of a sample. We present an ongoing experiment which aims to apply the method to tissue-like samples, where the quantum measurement is limited by a poor signal-to-noise ratio. Preliminary results demonstrate that this noise can be largely reduced by suitable frequency-domain filtering. This allows us to precisely determine the position of a scattering center using a few hundred detected photon pairs despite the presence of large amounts of noise. We follow this with a theoretical discussion of signal artifacts which are known to complicate the measured interferogram. We show these artifacts are due to a distinct interferometric effect, which can be distinguished from the signal of interest using the relative time delay between detected photons. We conclude with a brief discussion on possible techniques for artifact removal.
Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realizing this experimentally is technologically demanding, as it requires coincident single-photon detection proportional to the number of photons involved, which represents a severe challenge for achieving a practical quantum advantage over classical methods. Here, we exploit advanced quantum state engineering based on superposing two photon-pair creation events to realize a new approach that bypasses this issue. In particular, optical phase shifts are probed with a two-photon quantum state whose information is subsequently effectively transferred to a single-photon state. Notably, without any multiphoton detection, we infer phase shifts by measuring the average intensity of the single-photon beam on a photodiode, in analogy to standard classical measurements. Importantly, our approach maintains the quantum advantage: twice as many interference fringes are observed for the same phase shift, corresponding to N = 2 path-entangled photons. Our results demonstrate that the advantages of quantum-enhanced phase sensing can be fully exploited in standard intensity measurements, paving the way toward resource-efficient and practical quantum optical metrology.
Measuring the phase stability of single photons is essential for evaluating performance in various phase-based quantum applications, yet systematic methodologies for quantitative characterization remain underexplored. In this work, we numerically demonstrate that time-resolved two-photon interference can be effectively utilized to estimate the phase noise of single photons. Our simulations reveal that as phase noise increases, the interference visibility decreases, causing the joint detection probability to approach the non-interfering classical envelope. Furthermore, we verify that the power spectral density (PSD) of the phase noise can be reconstructed using a derived mathematical relationship. This approach establishes a direct quantitative link between measurable interference patterns and the underlying statistical phase fluctuations. This method provides a practical framework for characterizing single-photon phase stability, offering significant potential for enhancing quantum technologies such as quantum key distribution and sensing.
When a photon interferes with itself while traversing a Mach-Zehnder interferometer, the output port where it emerges is influenced by the phase difference between the interferometer arms. This allows for highly precise estimation of the path length difference (delay) but is extremely sensitive to phase noise. By contrast, a delay between the arms of the two-photon Hong-Ou-Mandel interferometer directly affects the relative indistinguishability of the photon pair, affecting the rate of recorded coincidences. This likewise allows for delay estimation, notably less precise but with the advantage of being less sensitive to perturbations of the photons' phase. Focusing on two-photon input states, we here investigate to what degree of noise Mach-Zehnder interferometry retains its edge over Hong-Ou-Mandel interferometry. We also explore the competing benefits of different two-photon inputs for a Mach-Zehnder interferometer and under what parameter regimes each input performs best.
The insights offered by quantum mechanics to the field of optical metrology are many-fold, with non-classical states of light themselves used to make sensors that surpass the sensitivity of sensors using classical states of light. Unfortunately, this advantage, referred to often as "super-sensitivity" is notoriously fragile, and even the slightest experimental imperfections may greatly reduce the efficacy of the non-classical sensors, sometimes completely obviating their advantage. In my thesis I have shown that the performance of an otherwise ideal two-photon interferometer, which exploits entanglement between photons to make super-sensitive measurements of phase, is crippled by the slightest introduction of decoherence between modes of the interferometer. I have shown further that such drastic reduction in sensitivity can also appear in classical measurement problems, specifically that the recently developed methods of estimating the separation between a pair of point sources are rendered less effective when the ideal assumption of complete spatial incoherence is relaxed. Towards overcoming these and other issues, I have designed new configurations that use ancillary optical degrees of freedom, a tool-set that has recently garnered much interest in the field of quantum optics. In the context of two-photon interferometry, I have shown that by coupling polarization to the spatial-structure of the two photon state used to probe phase it is possible to obviate the need for a reference phase, even in the context of decoherence and imperfections in the interferometer. In the context of two-point resolution, I have developed an anisotropic imaging system that performs the function of an image-inversion interferometer and is inherently stable, offering an attractive implementation of recently developed methods of sub-Rayleigh imaging. I have further shown both theoretically and experimentally that the same anisotropic image-inversion interferometer is useful in measuring spatially encoded phases, both in the context of classical illumination as well as quantum-aided two-photon super-sensing. In both cases, the ability to perform interferometric measurements of the spatial structure of an electric field without splitting beam paths forms a bridge between conception and implementation of precision-sensing measurement strategies. Finally, I have shown that binary interferometric method based on the common-path anisotropic imaging system that I introduced, are able to measure both phase gradients and transverse beam tilts with a sensitivity beating conventional systems that are used both commercially and in research laboratories.
Quantum interferences of entangled photons have engendered tremendous intriguing phenomena that lack any counterpart in classical physics. Hitherto, owing to the salient properties of quantum optics, quantum interference has been widely studied and provides useful tools that ultimately broaden the path towards ultra-sensitive quantum metrology, ranging from sub-shot-noise quantum sensing to high-resolution optical spectroscopy. In particular, quantum interferometric metrology is an essential requisite for extracting information about the structure and dynamics of photon-sensitive biological and chemical molecules. This article reviews the theoretical and experimental progress of this quantum interferometric metrology technology along with their advanced applications. The scope of this review includes Hong–Ou–Mandel interferometry with ultrahigh timing resolution, entanglement-assisted absorption spectroscopy based on a Fourier transform, and virtual-state spectroscopy using tunable energy-time entangled photons.