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arXiv:2004.09003 · Physical Review Letters

Probing Spin Correlations in a Bose-Einstein Condensate Near the Single-Atom Level

An Qu, Bertrand Evrard, Jean Dalibard, Fabrice Gerbier

Published Jul 17, 2020• 46 citations
arXivHTMLPDF

Abstract

Using parametric conversion induced by a Shapiro-type resonance, we produce and characterize a two-mode squeezed vacuum state in a sodium spin 1 Bose-Einstein condensate. Spin-changing collisions generate correlated pairs of atoms in the m=±1 Zeeman states out of a condensate with initially all atoms in m=0. A novel fluorescence imaging technique with sensitivity ΔN∼1.6 atom enables us to demonstrate the role of quantum fluctuations in the initial dynamics and to characterize the full distribution of the final state. Assuming that all atoms share the same spatial wave function, we infer a squeezing parameter of 15.3 dB.

DOI
10.1103/physrevlett.125.033401

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Using parametric conversion induced by a Shapiro-type resonance, we produce and characterize a two-mode squeezed vacuum state in a sodium spin 1 Bose-Einstein condensate. Spin-changing collisions generate correlated pairs of atoms in the m=±1 Zeeman states out of a condensate with initially all atoms in m=0. A novel fluorescence imaging technique with sensitivity ΔN∼1.6 atom enables us to demonstrate the role of quantum fluctuations in the initial dynamics and to characterize the full distribution of the final state. Assuming that all atoms share the same spatial wave function, we infer a squeezing parameter of 15.3 dB.
Using parametric conversion induced by a Shapiro-type resonance, we produce and characterize a two-mode squeezed vacuum state in a sodium spin 1 Bose-Einstein condensate. Spin changing collisions generate correlated pairs of atoms in the m=±1m=\pm 1m=±1 Zeeman states out of a condensate with initially all atoms in m=0m=0m=0. A novel fluorescence imaging technique with sensitivity ΔN∼1.6\Delta N \sim 1.6ΔN∼1.6 atom enables us to demonstrate the role of quantum fluctuations in the initial dynamics and to characterize the full distribution of the final state, which reaches a squeezing level of 16.8 16.8\,16.8dB.
A major challenge in quantum metrology is the generation of entangled states with a macroscopic atom number. Here, we demonstrate experimentally that atomic squeezing generated via nonlinear dynamics in Bose-Einstein condensates, combined with suitable trap geometries, allows scaling to large ensemble sizes. We achieve a suppression of fluctuations by 5.3(5) dB for 12,300 particles, from which we infer that similar squeezing can be obtained for more than 10(7) atoms. With this resource, we demonstrate quantum-enhanced magnetometry by swapping the squeezed state to magnetically sensitive hyperfine levels that have negligible nonlinearity. We find a quantum-enhanced single-shot sensitivity of 310(47) pT for static magnetic fields in a probe volume as small as 90 μm3.
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The quantum properties of matter waves, in particular quantum correlations and entanglement are an important frontier in atom optics with applications in quantum metrology and quantum information. In this thesis, we report the first observation of sub-Poissonian fluctuations in the magnetization of a spinor 87Rb condensate. The fluctuations in the magnetization are reduced up to 10 dB below the classical shot noise limit. This relative number squeezing is indicative of the predicted pair-correlations in a spinor condensate and lay the foundation for future experiments involving spin-squeezing and entanglement measurements. We have investigated the limits of the imaging techniques used in our lab, absorption and fluorescence imaging, and have developed the capability to measure atoms numbers with an uncertainly < 10 atoms. Condensates as small as ≈ 10 atoms were imaged and the measured fluctuations agree well with the theoretical predictions. Furthermore, we implement a reliable calibration method of our imaging system based on quantum projection noise measurements. We have resolved the individual lattice sites of a standing-wave potential created by a CO2 laser, which has a lattice spacing of 5.3 µm. Using microwaves, we site-selectively address and manipulate the condensate and therefore demonstrate the ability to perturb the lattice condensate of a local level. Interference between condensates in adjacent lattice sites and lattice sites separated by a lattice site are observed.
Bose-Einstein condensates of atoms with non-zero spin are known to constitute an ideal system to investigate fundamental properties of magnetic superfluids. More recently it was realized that they also provide the fascinating opportunity to investigate the macroscopic amplification of quantum and classical fluctuations. This is strikingly manifested in a sample initially prepared in the m F = 0 state, where spin-changing collisions triggered by quantum fluctuations may lead to the creation of correlated pairs in m F = ±1. We show that the pair creation efficiency is strongly influenced by the interplay between the external trapping potential and the Zeeman effect. It thus reflects the confinement-induced magnetic field dependence of elementary spin excitations of the condensate. Remarkably, pair production in our experiments is therefore characterized by a multi-resonant dependence on the magnetic field. Pair creation at these resonances acts as strong parametric matter-wave amplifier. Depending on the resonance condition, this amplification can be extremely sensitive or insensitive to the presence of seed atoms. We show that pair creation at a resonance which is insensitive to the presence of seed atoms is triggered purely by quantum fluctuations and thus the system acts as a matter-wave amplifier for the vacuum state.
Spin changing collisions in alkaline Bose-Einstein condensates can be employed to generate highly entangled atomic quantum states. Here, we will report on the generation of two classes of entangled states. Firstly, we demonstrate the generation of two-mode squeezed vacuum states and record their characteristic quadrature correlations by atomic homodyning. We prove that the correlations fulfill Reid’s criterion [1] for continuous-variable Einstein-Podolsky-Rosen entanglement. The homodyne measurements allow for a full tomographic reconstruction, yielding a two-mode squeezed state with a 78% fidelity. The created state can be directly applied to atom interferometry, as is exemplified by an atomic clock measurement beyond the Standard Quantum Limit. Secondly, we demonstrate entanglement between two spatially separated atomic modes. The entangled state is obtained by spatially splitting a Twin Fock state of indistinguishable atoms along a line of zero density. This structure of two separated atomic modes is obtained by utilizing an excited trap mode. The non-classical correlations between these atomic modes are verified by applying a novel entanglement criterion especially sensitive for our case. The method opens a path to exploit the recent success in the creation of many-particle entanglement in ultracold atoms for the field of quantum information, where individually addressable subsystems are required. Finally, we will show how the measurement protocol can be extended to perform a Bell test of quantum nonlocality. [1] M. Reid, Phys. Rev. A 40, 913-923 (1989)