The recent experimental observation of dissipation-induced structural instability provides new opportunities for exploring the competition mechanism between stationary and nonstationary dynamics [N. Dogra et al., Science 366, 1496 (2019)]. In that study, two orthogonal quadratures of cavity field were coupled to two different Zeeman states of a spinor Bose-Einstein condensate (BEC). Here we propose a scheme to couple two density-wave degrees of freedom of a BEC to two quadratures of the cavity field. Different from previous studies, the light-matter quadratures coupling in our model is endowed with a tunable coupling angle. Apart from the uniform and self-organized phases, we unravel a dynamically unstable state induced by the cavity dissipation. Interestingly, the dissipation defines a particular coupling angle, across which the instabilities disappear. Moreover, at this critical coupling angle, one of the two atomic density waves can be independently excited without affecting one another. It is also found that our system can be mapped into a reduced three-level model under the commonly used low-excitation-mode approximation. However, the effectiveness of this approximation is shown to be broken by the dissipative nature of some special system parameters, hinting that the low-excitation-mode approximation is insufficient in capturing some dissipation-sensitive physics. Our work enriches the quantum simulation toolbox in the cavity-quantum-electrodynamics system and broadens the frontiers of light-matter interaction.
The recent experimental observation of dissipation-induced structural instability provides new opportunities for exploring the competition mechanism between stationary and nonstationary dynamics [N. Dogra et al., Science 366, 1496 (2019)]. In that study, two orthogonal quadratures of cavity field were coupled to two different Zeeman states of a spinor Bose-Einstein condensate (BEC). Here we propose a scheme to couple two density-wave degrees of freedom of a BEC to two quadratures of the cavity field. Different from previous studies, the light-matter quadratures coupling in our model is endowed with a tunable coupling angle. Apart from the uniform and self-organized phases, we unravel a dynamically unstable state induced by the cavity dissipation. Interestingly, the dissipation defines a particular coupling angle, across which the instabilities disappear. Moreover, at this critical coupling angle, one of the two atomic density waves can be independently excited without affecting one another. It is also found that our system can be mapped into a reduced three-level model under the commonly used low-excitation-mode approximation. However, the effectiveness of this approximation is shown to be broken by the dissipative nature of some special system parameters, hinting that the low-excitation-mode approximation is insufficient in capturing some dissipation-sensitive physics. Our work enriches the quantum simulation toolbox in the cavity-quantum-electrodynamics system and broadens the frontiers of light-matter interaction.
Dissipative and unitary processes define the evolution of a many-body system. Their interplay gives rise to dynamical phase transitions and can lead to instabilities. In this study, we observe a nonstationary state of chiral nature in a synthetic many-body system with independently controllable unitary and dissipative couplings. Our experiment is based on a spinor Bose gas interacting with an optical resonator. Orthogonal quadratures of the resonator field coherently couple the Bose-Einstein condensate to two different atomic spatial modes, whereas the dispersive effect of the resonator losses mediates a dissipative coupling between these modes. In a regime of dominant dissipative coupling, we observe the chiral evolution and relate it to a positional instability.
We study a transversely pumped atomic Bose-Einstein condensate coupled to a single-mode optical cavity, where effective atom-atom interactions are mediated by pump and cavity photons. A number of experiments and theoretical works have shown the formation of a superradiant state in this setup, where interference of pump and cavity light leads to an optical lattice in which atoms self-consistently organize. This self-organization has been extensively studied using the approximate Dicke model (truncating to two momentum states), as well as through numerical Gross-Pitaevskii simulations in one and two dimensions. Here, we perform a full mean-field analysis of the system, including all relevant atomic momentum states and the cavity field. We map out the steady-state phase diagram vs pump strength and cavity detuning, and provide an in-depth understanding of the instabilities that are linked to the emergence of spatiotemporal patterns. We find and describe parameter regimes where the mean field predicts bistability, regimes where the dynamics form chaotic trajectories, instabilities caused by resonances between normal mode excitations, and states with atomic dynamics but vanishing cavity field.
Present-day experiments have started to couple traditional simulations of ultracold atom experiments with quantum light-fields in cavities. This has provided a wealth of op- portunities to enlarge the number of interaction potentials: cavity mediated long-range interactions compete with kinetic energies, longitudinal fields, short-ranged collisional or magnetic spin-spin interactions. The intracavity many-body lattice models often have to be maintained far from equilibrium through the presence of external driving lasers that help to boost and engineer the various interaction potentials. The steady influx of energy is compensated by a steady stream of energy out of the atom-cavity system for example by photon losses or atomic spontaneous emission. Several experiments have demonstrated that such environments can give rise to new competing quantum phases. \nBut this long-standing ambition to push for models with tailorable interaction potentials can bring with it also considerable challenges in their theoretical description, since sponta- neous symmetry breaking transitions in many body lattice systems coupled to dynamical light-fields with single-photon character occur in the presence of drive and dissipation for the photonic force carriers. This clearly calls for model systems where the above men- tioned interplay of interactions, drive, dissipation and cooperative many-body behaviour can be theoretically studied to provide simple, experimentally verifiable predictions. \nThe Dicke model is, through its simplicity (an exactly solved ferromagnet with infinite range atom-atom interactions mediated by a single cavity mode), an exceptionally well- suited candidate. As the generic model for atom-light interactions, it has been experimen- tally realized in a variety of modern quantum optical systems, highlighting its relevance for present-day research. The Dicke model is also highly versatile itself. It has been extended into the dissipative realm, was promoted to account for multiple optical light modes and was used to describe multiple, coupled single-mode cavity structures. It was adapted to treat spin-selective coupling to a cavity to describe superradiance phase tran- sitions in multi-level atomic systems. Moreover, it was realised in electronic circuits where the dipole coupling of real atoms to single mode fields is replaced by a capacitive cou- pling of artificial atoms to a resonator mode. This illustrates that the Dicke model and its extended variants are ’future-proof’ and continue to be of relevance for fundamental light-matter interactions and for driven-dissipative phase transitions. \nIn this thesis, we investigate magnetic phase transitions in driven-dissipative atomic en- sembles interacting with quantum light. We present three research projects on variants of cooperative radiation of an ensemble of laser driven two-level atoms in a single mode optical cavity, as described by the Dicke model. \nThroughout the chapters 2,3 and 4 that contain the main body of research of this thesis, we investigate phase transitions between non-equilibrium stationary states in engineered quantum-optical systems each of which extends the conventional Dicke model physics. As a starting point, we map the quantum equations of motion onto a set of semiclassical nonlinear stochastic equations and analyse their stationary states and instabilities with master equations for atomic spin and photon mean-field amplitudes. These are used to obtain experimentally relevant parameters such as critical atom-light couplings for phase transitions, phase diagrams and properties of stationary non-equilibrium states in addition to cavity output spectra that identify the imprint of magnetic correlations in the light-field. \nIn chapter 2, we help resolve a discrepancy between earlier experimental investigations of the critical atom-light coupling strength for the superradiance transition in the Dicke model: higher external pumping strengths than theoretically predicted were needed to observe a coherent, superradiant state of the light field in an optical cavity. By including incoherent spontaneous emission of atomic excitations, we extend the dissipative Dicke model to a two loss channel variant containing both photon leakage and atomic decay that reproduces the experimentally observed critical atom-light coupling. \nRecent experiments have started to interface quantum many body lattice models with coherent cavity fields, thereby allowing to realize new quantum phases through competing atom-cavity and atom-atom interactions. In chapter 3, we consider a simplified model for such a set-up where a single quantized mode of the light-field interacts with an ensemble of Rydberg-dressed atoms inside a high finesse optical cavity. This model provides a base case for further studies of quantum magnets in optical cavities. At the heart of this model is a competition of short- (dipolar atom-atom) and long-range (atom-light) interactions at the Hamiltonian level in the presence of both spontaneous emission and photon leak- age through the cavity mirrors. We show that different magnetic phases can coexist with coherent atomic radiation and provide clear experimental signatures to identify the mag- netic structure and intra-cavity dynamics. We suggest an experimental level-scheme for a quantum optical implementation of our model. \nIn chapter 4 we consider a generic, collective decay for many-body excitations in the paradigmatic Dicke model. This extension drastically enriches the dynamics as it induces a bicritical point and a bistable regime dominated by true non-equilibrium fluctuations that induce a dissipative first-order phase transition that can only be resolved by including finite fluctuation corrections with the help of stochastic Langevin equations. We investigate the hysteretic response to time-dependent ramps of the atom-light coupling. Discontinuous first-order phase transitions where metastable states coexist in a hysteresis domain have been investigated in recent dissipative quantum-optical experiments. We review noise- activation far from thermal equilibrium in chapter 5.
Ultracold atomic gases loaded into optical cavities constitute one of the most versatile platforms for the study of out-of-equilibrium dynamics and quantum simulation of many- body systems. In this thesis, we explore these two possibilities, motivated by current state-of-the-art atom-cavity experiments, uncovering novel phenomena and opening up new theoretical and experimental avenues into the intriguing world of quantum many- body physics. First, we study a gas of ultracold atoms coupled to three optical resonators. We show that the inherent Z2 symmetries, associated with each atom-cavity coupling, can be combined into a global SO(3) rotational symmetry which can be spontaneously broken. We determine the phase diagram of the system, which shows the emergence and breaking of the continuous symmetries and displays first- and second-order phase transitions. We argue that by coupling the atoms equally to n different modes, it will in general be possible to generate a global SO(n) symmetry. Second, we investigate the dynamics of a spinor BEC inside an optical cavity. We focus on a two-component Dicke model with complex light-matter couplings, accounting for photon losses. We compute the steady-state phase diagram and find dynamical in- stabilities in the form of limit cycles, heralded by the presence of exceptional points and level attraction. We show that the instabilities are induced by dissipative processes that generate nonreciprocal couplings between the two collective spins. Lastly, we explore the dynamics of a BEC inside an optical cavity in the presence of an optical lattice. We derive an effective master equation by adiabatically eliminating the cavity field. In the bad-cavity regime, we find an infinite-temperature steady state, but with relaxation dynamics that can be highly nontrivial. For small hopping, the interplay between dissipation and strong interactions leads to an algebraic relaxation of the system, whereas for large hopping, the approach to the steady state is exponential. In the good- cavity regime, we show that the system allows for optical pumping between momentum modes, enabling cavity cooling.
Motivated by recent experiments on light-matter interacting systems, we investigate a dilute Bose gas and self-bound quantum droplets in a one-dimensional optical lattice coupled to a lossy cavity mode. Using a classical-field approach, we determine the stationary states and collective excitations of this non-equilibrium system. Apart from the usual Bogoliubov modes, we identify a polariton-like gapped excitation, the frequency of which softens as a precursor of the density ordering transition. Moreover, its relaxation time diverges as the critical point is approached, signaling the non-equilibrium nature of this transition. Dynamically, this polariton-like mode can be probed by inducing cavity field fluctuations, which in turn generates spatio-temporal oscillations of both the condensate and droplet states. In the droplet regime, we also analyze the bound modes which bear the characteristics of such non-equilibrium self-bound state. In addition, we uncover solitonic non-equilibrium states, including condensate with kink-like configuration and double-droplet state, and investigate their robustness following a sudden quench. Remarkably, although these states become unstable beyond a critical coupling, they continue to manifest in the dynamics, akin to the scarring phenomena. Our results demonstrate that dissipative cavity coupling provides a versatile route for exploring rich non-equilibrium dynamics of condensates and quantum droplets within experimentally accessible settings.
The coupled nonlinear dynamics of ultracold quantum matter and electromagnetic field modes in an optical resonator exhibits a wealth of intriguing collective phenomena. Here we study a Λ-type, three-component Bose–Einstein condensate coupled to four dynamical running-wave modes of a ring cavity, where only two of the modes are externally pumped. However, the unpumped modes play a crucial role in the dynamics of the system due to coherent backscattering of photons. On a mean- field level we identify three fundamentally different steady-state phases with distinct characteristics in the density and spatial spin textures: a combined density and spin-wave, a continuous spin spiral with a homogeneous density, and a spin spiral with a modulated density. The spin-spiral states, which are topological, are intimately related to cavity-induced spin–orbit coupling emerging beyond a critical pump power. The topologically trivial density-wave–spin-wave state has the characteristics of a supersolid with two broken continuous symmetries. The transitions between different phases are either simultaneously topological and first-order, or second-order. The proposed setup allows the simulation of intriguing many-body quantum phenomena by solely tuning the pump amplitudes and frequencies, with the cavity output fields serving as a built-in nondestructive observation tool.