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arXiv:2004.02485 · Science Advances

Two-level systems in superconducting quantum devices due to trapped quasiparticles

S. E. de Graaf, Lara Faoro, L. B. Ioffe, S. Mahashabde, Jonathan Burnett, T. Lindström, S. E. Kubatkin, A. V. Danilov, A. Ya. Tzalenchuk

Published Dec 18, 2020• 108 citations
arXivHTMLPDF

Abstract

A major issue for the implementation of large-scale superconducting quantum circuits is the interaction with interfacial two-level system (TLS) defects that lead to qubit parameter fluctuations and relaxation. Another major challenge comes from nonequilibrium quasiparticles (QPs) that result in qubit relaxation and dephasing. Here, we reveal a previously unexplored decoherence mechanism in the form of a new type of TLS originating from trapped QPs, which can induce qubit relaxation. Using spectral, temporal, thermal, and magnetic field mapping of TLS-induced fluctuations in frequency tunable resonators, we identify a highly coherent subset of the general TLS population with a low reconfiguration temperature ∼300 mK and a nonuniform density of states. These properties can be understood if the TLS are formed by QPs trapped in shallow subgap states formed by spatial fluctutations of the superconducting order parameter. This implies that even very rare QP bursts will affect coherence over exponentially long time scales.

DOI
10.1126/sciadv.abc5055

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A major issue for the implementation of large-scale superconducting quantum circuits is the interaction with interfacial two-level system (TLS) defects that lead to qubit parameter fluctuations and relaxation. Another major challenge comes from nonequilibrium quasiparticles (QPs) that result in qubit relaxation and dephasing. Here, we reveal a previously unexplored decoherence mechanism in the form of a new type of TLS originating from trapped QPs, which can induce qubit relaxation. Using spectral, temporal, thermal, and magnetic field mapping of TLS-induced fluctuations in frequency tunable resonators, we identify a highly coherent subset of the general TLS population with a low reconfiguration temperature ∼300 mK and a nonuniform density of states. These properties can be understood if the TLS are formed by QPs trapped in shallow subgap states formed by spatial fluctutations of the superconducting order parameter. This implies that even very rare QP bursts will affect coherence over exponentially long time scales.
A major issue for the implementation of large scale superconducting quantum circuits is the interaction with interfacial two-level system defects (TLS) that leads to qubit relaxation and impedes qubit operation in certain frequency ranges that also drift in time. Another major challenge comes from non-equilibrium quasiparticles (QPs) that result in qubit dephasing and relaxation. In this work we show that such QPs can also serve as a source of TLS. Using spectral and temporal mapping of TLS-induced fluctuations in frequency tunable resonators, we identify a subset of the general TLS population that are highly coherent TLS with a low reconfiguration temperature ∼\sim∼ 300 mK, and a non-uniform density of states. These properties can be understood if these TLS are formed by QPs trapped in shallow subgap states formed by spatial fluctutations of the superconducting order parameter Δ\DeltaΔ. Magnetic field measurements of one such TLS reveals a link to superconductivity. Our results imply that trapped QPs can induce qubit relaxation.
Temporal fluctuations in the superconducting qubit lifetime, T1{T}_{1}T1​, present additional challenges in the pursuit of fault-tolerant quantum computing. Although the exact mechanisms remain unclear, T1{T}_{1}T1​ fluctuations are generally attributed to strong coupling between the qubit and a few near-resonant two-level systems (TLSs), which can exchange energy with an ensemble of thermally fluctuating two-level fluctuators (TLFs) at low frequencies. Here, we report T1{T}_{1}T1​ measurements of qubits with varying geometrical footprints and surface dielectrics as a function of temperature. By analyzing the noise spectrum of the qubit depolarization rate, ${\mathrm{\ensuremath{\Gamma}}}_{1}=1/{T}_{1}$, we disentangle the contributions of TLSs, nonequilibrium quasiparticles (QPs), and equilibrium (thermally excited) QPs to the variance in ${\mathrm{\ensuremath{\Gamma}}}_{1}$. We find that the ${\mathrm{\ensuremath{\Gamma}}}_{1}$ variance in qubits with smaller footprints is more susceptible to QP and TLS fluctuations than that in larger-footprint qubits. Furthermore, the QP-induced variances in all qubits align with the theoretical framework of QP diffusion and fluctuation. These findings offer valuable insights for future qubit design and engineering optimization.
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Microscopic two-level systems (TLS) -- ubiquitous atomic-scale defects in solid-state quantum devices -- are a dominant source of qubit decoherence, yet their role is often considered local and short-memoried. Here, we report the observation of a coherent TLS that couples simultaneously to two spatially distant superconducting qubits. The TLS is identified to reside within the tunable coupler linking the qubits, enabling controllability of the TLS-qubit coupling strength via coupler frequency -- a capability absent in earlier studies. This tunability allows us to systematically probe how TLS distorts qubit dynamics, revisiting the decoherence model in the presence of non-Markovian TLS dephasing noise. This is corroborated by the reconstructed 1/f1/f1/f noise spectrum of TLS frequency fluctuation spanning more than ten orders of magnitude (0.1\,mHz -- 1\,MHz) that reveals discrete fluctuator signatures. Quantum process tomography further unveils TLS-induced correlated qubit dynamics, highlighting the long-lived TLS as an effective source of non-Markovianity. Our findings expose a previously overlooked interaction mechanism in scalable quantum architectures: defects embedded in coupling elements can simultaneously affect multiple qubits with variable impact. Beyond immediate implications for system characterization and calibration, this situation provides a powerful testbed for studying defect-driven quantum dynamics, refining error suppression strategies, and advancing architecture design for scalable quantum technologies.
Recent progress with microfabricated quantum devices has revealed that an ubiquitous source of noise originates in tunneling material defects that give rise to a sparse bath of parasitic two-level systems (TLSs). For superconducting qubits, TLSs residing on electrode surfaces and in tunnel junctions account for a major part of decoherence and thus pose a serious roadblock to the realization of solid-state quantum processors. Here, we utilize a superconducting qubit to explore the quantum state evolution of coherently operated TLSs in order to shed new light on their individual properties and environmental interactions. We identify a frequency-dependence of TLS energy relaxation rates that can be explained by a coupling to phononic modes rather than by anticipated mutual TLS interactions. Most investigated TLSs are found to be free of pure dephasing at their energy degeneracy points, around which their Ramsey and spin-echo dephasing rates scale linearly and quadratically with asymmetry energy, respectively. We provide an explanation based on the standard tunneling model, and identify interaction with incoherent low-frequency (thermal) TLSs as the major mechanism of the pure dephasing in coherent high-frequency TLS.
Two-level systems (TLS) are widely recognized as a dominant source of energy relaxation in superconducting qubits, limiting coherence times and device performance. While TLS-induced dissipation is often modeled as independent channels, interacting TLS can form finite many-body environments whose dynamical role in qubit relaxation remains insufficiently understood. Building on the information-erasure-based framework for irreversible thermalization developed in our previous work, we present a microscopic model and numerical simulations of a superconducting qubit coupled to a finite interacting many-body TLS environment as a concrete physical realization of this mechanism. We show that effective irreversible energy relaxation can emerge from intrinsic many-body dynamics without invoking external baths or phenomenological dissipation. The introduction of information erasure drives a transition from coherent oscillatory energy exchange to nonoscillatory exponential relaxation of the qubit. The relaxation times exhibit the scaling T1,T2∝Jq,τ−2T_1, T_2 \propto J_{q,τ}^{-2}T1​,T2​∝Jq,τ−2​ with respect to the qubit-TLS coupling strength, consistent with Fermi's golden rule and Lindblad-type descriptions. Importantly, both exponential decay and its scaling behavior arise directly from microscopic many-body dynamics. These results provide quantitative insight into TLS-induced decoherence mechanisms and establish a microscopic link between information erasure, many-body thermalization, and irreversible relaxation in superconducting quantum systems.