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arXiv:2004.02303 · Physical Review Letters

Imaging and Localizing Individual Atoms Interfaced with a Nanophotonic Waveguide

Yijian Meng, Christian Liedl, Sebastian Pucher, Arno Rauschenbeutel, Philipp Schneeweiß

Published Jul 31, 2020• 32 citations
arXivHTMLPDF

Abstract

Single particle-resolved fluorescence imaging is an enabling technology in cold-atom physics. However, so far, this technique has not been available for nanophotonic atom-light interfaces. Here, we image single atoms that are trapped and optically interfaced using an optical nanofiber. Near-resonant light is scattered off the atoms and imaged while counteracting heating mechanisms via degenerate Raman cooling. We detect trapped atoms within 150 ms and record image sequences of given atoms. Building on our technique, we perform two experiments which are conditioned on the number and position of the nanofiber-trapped atoms. We measure the transmission of nanofiber-guided resonant light and verify its exponential scaling in the few-atom limit, in accordance with Beer-Lambert's law. Moreover, depending on the interatomic distance, we observe interference of the fields that two simultaneously trapped atoms emit into the nanofiber. The demonstrated technique enables postselection and possible feedback schemes and thereby opens the road toward a new generation of experiments in quantum nanophotonics.

DOI
10.1103/physrevlett.125.053603

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Single particle-resolved fluorescence imaging is an enabling technology in cold-atom physics. However, so far, this technique has not been available for nanophotonic atom-light interfaces. Here, we image single atoms that are trapped and optically interfaced using an optical nanofiber. Near-resonant light is scattered off the atoms and imaged while counteracting heating mechanisms via degenerate Raman cooling. We detect trapped atoms within 150 ms and record image sequences of given atoms. Building on our technique, we perform two experiments which are conditioned on the number and position of the nanofiber-trapped atoms. We measure the transmission of nanofiber-guided resonant light and verify its exponential scaling in the few-atom limit, in accordance with Beer-Lambert's law. Moreover, depending on the interatomic distance, we observe interference of the fields that two simultaneously trapped atoms emit into the nanofiber. The demonstrated technique enables postselection and possible feedback schemes and thereby opens the road toward a new generation of experiments in quantum nanophotonics.
Cold atom-nanophotonic systems constitute a powerful research platform for the exploration of new regimes of light-matter interaction. The guided light in nanophotonic systems are tightly confined, and often used to trap and manipulate cold atoms at subwavelength distance away from the surface. While the initialization of atomic internal degrees of freedom in these systems has been achieved, a full control of the atomic quantum state also requires manipulating and preparing the atomic motional state at the quantum level. In this thesis, we explore and characterize the coupling between motional and spin degrees of freedom in nanofiber-trapped atoms. This coupling originates from the strong polarization gradient which occurs naturally in spatially confined light fields, i.e., the guided light field in a nanophotonic system. We demonstrate that the spin-motion coupling can be utilized to implement degenerate Raman cooling and prepare atoms close to the three-dimensional motional ground state.We obtain mean numbers of motional quanta of nanofiber-trapped atoms using heterodyne fluorescence spectroscopy. Building on this work, we then use the spin-motion coupling for nanofiber-trapped atoms to realize a mechanical analogue of the Dicke model. We infer the energy spectrum of the system from transitions observed in the fluorescence spectrum. We show that our system reaches the ultrastrong coupling regime. Moreover, we demonstrate that the coupling strength can be readily tuned using an additional nanofiber-guided light field. Furthermore, we achieve imaging of single nanofiber-trapped atoms. Taking advantage of degenerate Raman cooling, we cool atoms near the motional ground state while collecting atomscattered light using a camera. We show single atoms can be detected by imaging at an integration time far less than the trapping lifetime. To demonstrate the potential of this technique, we perform two proof of principle experiments. First, we measure the extinction of a nanofiberguided light atom by atom, and verify the Beer-Lambert Law in the few atoms regime. Second, we detect the atom-scattered light that is coupled to the nanofiber. We observe interference of scattered light fields as a function of the distance between two trapped atoms. By controlling atomic motional states and imaging single atoms, our work in this thesis adds to the toolbox for manipulating and detecting cold atoms interfaced to nanophotonic systems, and paves the way for realizing the bottom-up approach to explore new regimes of light-matter interaction atom by atom.
Integrating the scalability of individually addressable arrays of optical-tweezer-trapped single atoms with the efficient light-matter interface provided by nanophotonic waveguides has been a long-standing challenge in quantum technologies based on atoms and photons. Here we realize a quantum interface between photons guided in an optical nanofiber with a diameter of 310 nm and an array of on average 155 individually addressable atoms. Using a spatial light modulator and an objective lens with NA = 0.45, single cesium atoms are trapped in a one-dimensional array of 200 optical tweezer spots with micrometer-scale trap sizes on the nanofiber. Individual atoms are addressed by spatially scanning an excitation laser beam, focused to a spot size comparable to that of the traps through the same objective lens, along the nanofiber. We confirm the single-atom nature of the individual trapping sites through photon-correlation measurements of the guided fluorescence, observing strong photon antibunching with g(2)(0)≈0.26g^{(2)}(0) \approx 0.26g(2)(0)≈0.26. We measure trap lifetimes of a few hundred milliseconds, with a maximum value of 460 ms, at an atom-surface separation of 670 nm without active cooling, representing an order-of-magnitude improvement over previous nanofiber traps. This platform opens a new regime for atom-photon interfaces, paving the way for scalable distributed quantum computing and quantum networks, as well as for the exploration of collective radiative effects in waveguide QED with individually addressable atoms.
Near-fields around nanophotonic structures and waveguides can be used to optically interface particles ranging from atoms and molecules to microscopic biological and synthetic particles. Due to the strong, non-linear dependence of the near-field coupling strength on the particles' position, a change of the spread of the particles' position will change their mean coupling strength. When the particles are trapped, this position spread depends on their temperature, generally leading to temperature-dependent coupling. Here, we experimentally demonstrate that this effect renders optical probing of trapped particles with near fields an inherently transient process. Specifically, we trap cold atoms in a two-color dipole trap surrounding an optical nanofiber and probe them with the evanescent field of guided, resonant light. The scattering of this probe light heats up the atoms, leading to a decrease of the coupling strength as well as loss of atoms. We observe both effects via a concurrent decrease of the absorption signal. In addition, we demonstrate that the coupling strength can be recovered by cooling the atoms back to their initial temperature. Our findings are relevant for numerous situations where stable coupling of trapped particles to a nanophotonic structure is required.
Laser-cooled atoms coupled to nanophotonic structures constitute a powerful research platform for the exploration of new regimes of light-matter interaction.While the initialization of the atomic internal degrees of freedom in these systems has been achieved, a full preparation of the atomic quantum state also requires controlling the center-of-mass motion of the atoms at the quantum level.Obtaining such control is not straightforward because of the close vicinity of the atoms to the photonic system at ambient temperature.Here, we demonstrate cooling of individual neutral cesium atoms that are optically interfaced with light in an optical nanofiber, preparing them close to their three-dimensional motional ground state.The atoms are localized less than 300 nm away from the hot fiber surface.Ground-state preparation is achieved by performing degenerate Raman cooling, and the atomic temperature is inferred from the analysis of heterodyne fluorescence spectroscopy signals.Our cooling method can be implemented either with externally applied or guided light fields.Moreover, it relies on polarization gradients, which naturally occur for strongly confined guided optical fields.Thus, this method can be implemented in any trap based on nanophotonic structures.Our results provide an ideal starting point for the study of novel effects such as light-induced self-organization, the measurement of novel optical forces, and the investigation of heat transfer at the nanoscale using quantum probes.
Abstract Near-fields around nanophotonic structures and waveguides can be used to optically interface particles ranging from atoms and molecules to microscopic biological and synthetic particles. Due to the strong, nonlinear dependence of the near-field coupling strength on the particles’ position, a change of the spread of the particles’ position will change their mean coupling strength. When the particles are trapped, this position spread depends on their temperature, generally leading to temperature-dependent coupling. Here, we experimentally demonstrate that this effect renders optical probing of trapped particles with near fields an inherently transient process. Specifically, we trap cold atoms in a two-color dipole trap surrounding an optical nanofiber and probe them with the evanescent field of guided, resonant light. The scattering of this probe light heats up the atoms, leading to a decrease of the coupling strength as well as loss of atoms. We observe both effects via a concurrent decrease of the absorption signal. In addition, we demonstrate that the coupling strength can be recovered by cooling the atoms back to their initial temperature. Our findings are relevant for numerous situations where stable coupling of trapped particles to a nanophotonic structure is required.
We demonstrate efficient interfacing of individually trapped single atoms to a nanofiber cavity. The cavity is formed by fabricating photonic crystal structures directly on the nanofiber using femtosecond laser ablation. The single atoms are interfaced to the nanofiber cavity using an optical tweezer based side-illumination trapping scheme. We show that the fluorescence of individual single atoms trapped on the nanofiber cavity can be readily observed in real-time through the fiber guided modes. From the photon statistics measured for different cavity decay rates, the effective coupling rate of the atom-cavity interface is estimated to be 34±2 MHz. This yields a cooperativity of 5.4±0.6 (Purcell factor=6.4±0.6) and a cavity enhanced channeling efficiency as high as 85±2% for a cavity mode with a finesse of 140. The trap lifetime is measured to be 52±5 ms. These results may open new possibilities for deterministic preparation of single atom events for quantum photonics applications on an all-fiber platform.