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arXiv:2004.00040

The paraxial approximation fails to describe the interaction of atoms with general vortex light fields

G. F. Quinteiro, Christian Tomás Schmiegelow, Ferdinand Schmidt‐Kaler

Published Mar 31, 2020• 3 citations
arXivHTMLPDF

Abstract

Neglecting the electric field component along the light's propagation direction is a common practice, known as paraxial approximation. However, experimental evidence and theory on the head-on excitation of atoms by Laguerre-Gaussian beams reveal that the full vector character of the light field has to be taken into account. Optical vortices are a large family of fields, being Laguerre-Gaussian only one particular case. Now we extend the study of the applicability of the paraxial approximation to a broader set of optical vortices by considering the interaction of atoms with generalized Laguerre-Gaussian and generalized Bessel beams. We demonstrate that all vortex beams here considered look the same close to the beam axis, where the atom is placed. From this, we conclude that the paraxial approximation fails for the large set of vortex beams, and that a full understanding of the interaction of optical vortices with atoms requires the inclusion of all vector components of the electric field.

DOI
10.48550/arxiv.2004.00040

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Neglecting the electric field component along the light's propagation direction is a common practice, known as paraxial approximation. However, experimental evidence and theory on the head-on excitation of atoms by Laguerre-Gaussian beams reveal that the full vector character of the light field has to be taken into account. Optical vortices are a large family of fields, being Laguerre-Gaussian only one particular case. Now we extend the study of the applicability of the paraxial approximation to a broader set of optical vortices by considering the interaction of atoms with generalized Laguerre-Gaussian and generalized Bessel beams. We demonstrate that all vortex beams here considered look the same close to the beam axis, where the atom is placed. From this, we conclude that the paraxial approximation fails for the large set of vortex beams, and that a full understanding of the interaction of optical vortices with atoms requires the inclusion of all vector components of the electric field.
Experimental evidence and theory on the head-on excitation of atoms by paraxial Laguerre–Gaussian beams revealed that the longitudinal component of the field has to be taken into account. Optical vortices are in fact a large family of fields, Laguerre–Gaussian being only one particular case. Here, we extend the previous study to a broader set of vortex fields. We demonstrate that, in general, paraxial optical vortices that have opposite orbital and spin angular momenta exhibit a longitudinal component that cannot be disregarded in the light–matter interaction.
The exchange of orbital angular momentum (OAM) between paraxial optical vortex and a Bose-Einstein condensate (BEC) of atomic gases is well known. In this paper, we develop a theory for the microscopic interaction between matter and an optical vortex beyond paraxial approximation. We show how superposition of vortex states of BEC can be created with a focused optical vortex. Since the polarization or spin angular momentum (SAM) of the optical field is coupled with OAM of the field, in this case, these angular momenta can be transferred to the internal electronic and external center-of-mass motion of atoms provided both the motions are coupled. We propose a scheme for producing the superposition of matter-wave vortices using Gaussian and a focused Laguerre-Gaussian beam. We study how two-photon Rabi frequencies of stimulated Raman transitions vary with focusing angles for different combinations of OAM and SAM of optical states. We demonstrate the formation of vortex-antivortex structure and discuss interference of three vortex states in a BEC.
Recent studies have confirmed the coupling of optical vortices, such as Laguerre-Gaussian and Bessel-Gaussian modes, to quadrupole-active atomic transitions. This interaction has been shown to be enhanced considerably in the case of Laguerre-Gaussian beams due to the gradient coupling, particularly, in the case of a relatively large winding number. Here, we consider the trapping and the dynamics of atoms in the optical quadrupole potential generated by two coaxial counterpropagating optical vortex beams. We focus on the atomic transition $6{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}\ensuremath{\rightarrow}5{\phantom{\rule{0.16em}{0ex}}}^{2}{D}_{5/2}$ in Cs which is a dipole-forbidden but a quadrupole-allowed transition. We show how this atomic transition engages with the optical vortex fields at near resonance, leading to atom trapping in the optical quadrupole potential well accompanied by translational motion. We show how the optical forces generate the motion of the atoms trapped within the quadrupole potential, illustrating the results using typical experimentally accessible parameters.
We examine the applicability and limitations of several established measures of paraxiality in the context of electric quadrupole interactions between light and trapped atoms. Focusing on Laguerre–Gaussian beams, we compare analytical predictions—particularly transition amplitudes and selection rules—derived under the paraxial assumption with full numerical solutions obtained via diffraction integrals that account for the complete vectorial field structure. This comparison allows us to assess the validity and relevance of these measures across a range of beam parameters. We also investigate the role of the power-series expansion in the paraxial parameter in bridging paraxial and nonparaxial regimes.
In this work, the paraxial approximation of the free Dirac equation is examined. The results are first obtained by constructing superpositions of exact solutions with suitable profiles, which are borrowed from paraxial optics. In this manner, the paraxial Dirac beams are obtained in four cases: as Gaussian, Bessel-Gaussian, modified Bessel-Gaussian and elegant Laguerre-Gaussian beams. In the second part of the work, the paraxial Dirac equation is derived, and then its solutions in the aforementioned cases are directly obtained. All the resulting wave functions conform to those derived formerly by virtue of superpositions, except for terms that are negligible upon the assumption that the paraxial functions along the propagation axis vary only slightly over a distance equal to the de Broglie wavelength, which is the standard paraxial requirement.
The propagation of light beams is well described using the paraxial approximation, where field components along the propagation direction are usually neglected. For strongly inhomogeneous or shaped light fields, however, this approximation may fail, leading to intriguing variations of the light-matter interaction. This is the case of twisted light having opposite orbital and spin angular momenta. We compare experimental data for the excitation of a quadrupole transition in a single trapped ^{40}Ca^{+} ion from Schmiegelow et al. [Nat. Commun. 7, 12998 (2016)NCAOBW2041-172310.1038/ncomms12998] with a complete model where longitudinal components of the electric field are taken into account. Our model matches the experimental data and excludes by 11 standard deviations the approximation of a complete transverse field. This demonstrates the relevance of all field components for the interaction of twisted light with matter.