Abstract Unravelling superradiance, also known as superfluorescence, relies on an ensemble of phase-matched dipole oscillators and the suppression of inhomogeneous broadening. Here we report a superradiance platform that combines an optical lattice free from the ac Stark shift and a hollow-core photonic crystal fibre, enabling an extended atom-light interaction over 2 mm free from the Doppler effect. This system allows control of the atom spatial distribution and spectral homogeneity whilst efficiently coupling the radiation field to an optical fibre. The experimentally-observed and theoretically-corroborated temporal, spectral and spatial dynamic behaviours of the superradiance, e.g., superradiance ringing and density-dependent frequency shift, demonstrate a unique interplay between the trapped atoms and the fibre-guided field with multiple transverse modes. Our theory indicates that the resulting temporal evolution of the guided light shows a minimal beam radius of 3.1 µm which is three times smaller than that of the lowest-loss fibre mode.
Abstract Unravelling superradiance, also known as superfluorescence, relies on an ensemble of phase-matched dipole oscillators and the suppression of inhomogeneous broadening. Here we report a superradiance platform that combines an optical lattice free from the ac Stark shift and a hollow-core photonic crystal fibre, enabling an extended atom-light interaction over 2 mm free from the Doppler effect. This system allows control of the atom spatial distribution and spectral homogeneity whilst efficiently coupling the radiation field to an optical fibre. The experimentally-observed and theoretically-corroborated temporal, spectral and spatial dynamic behaviours of the superradiance, e.g., superradiance ringing and density-dependent frequency shift, demonstrate a unique interplay between the trapped atoms and the fibre-guided field with multiple transverse modes. Our theory indicates that the resulting temporal evolution of the guided light shows a minimal beam radius of 3.1 µm which is three times smaller than that of the lowest-loss fibre mode.
Unlike photons, which are conveniently handled by mirrors and optical fibres without loss of coherence, atoms lose their coherence via atom–atom and atom–wall interactions. This decoherence of atoms deteriorates the performance of atomic clocks and magnetometers, and also hinders their miniaturization. Here we report a novel platform for precision spectroscopy. Ultracold strontium atoms inside a kagome-lattice hollow-core photonic crystal fibre are transversely confined by an optical lattice to prevent atoms from interacting with the fibre wall. By confining at most one atom in each lattice site, to avoid atom–atom interactions and Doppler effect, a 7.8-kHz-wide spectrum is observed for the 1S0−3P1(m=0) transition. Atoms singly trapped in a magic lattice in hollow-core photonic crystal fibres improve the optical depth while preserving atomic coherence time. Atoms lose coherence via interactions with each other and the walls of their environment, which degrades the performance of atomic systems. As a route to minimize such effects, Okaba et al.use kagome-lattice hollow-core photonic crystal fibres to confine atoms, preventing them interacting with the wall.
Our goal is to study quantum optical phenomena in a strong nonlinear optical system. For this purpose, we create a hollow-core photonic-crystal (HCPC) fiber-based platform that confines photons and atomic ensembles together. This enables strong light-matter interactions which are crucial for implementing optical nonlinearities at single-photon levels [1]. We use an optical dipole trap at cesium's magic wavelength to guide laser cooled cesium atoms into and inside the fiber core. This approach will allow us to perform experiments with the dipole trap continuously on as opposed to the previously reported fiber-loading systems [2,3] in which the dipole trap was rapidly amplitude-modulated to avoid the effect from the spatially dependent AC Stark shift. In this system, we perform experiments on electromagnetically induced transparency (EIT) and demonstrate slow light and all optical switch. We also aim to observe large cross-phase modulation (XPM) using a three-level ladder scheme [4,5]. Lastly, the approaches to integrate a cavity into HCPCFs to increase light-matter interactions, thus the optical nonlinearities, will be described.
In this thesis, I am intending to understand the cooperative effect of an ensemble of quantum emitters, which constitutes the preliminary elements of our current experimental investigations towards realization of an ultra-narrow linewidth superriant laser. In the first part of the thesis, I investigate the basics of the theory of superradiance (SR), which includes the full derivation of the Hamiltonian and the Lindblad equation for an ensemble of two-level atoms in both free-space and a single-mode waveguide. In addition, I construct the simulations for observing the transition from single-atom uncorrelated spontaneous emission to superradiance in various physical settings, as well as a simulation for the understanding of the cooperative effects of an ensemble of two-level atoms inside an optical cavity. Then, in the second part of the thesis, I introduce the experimental progress we have been making to observe SR with an ensemble of laser-cooled Cs atoms inside a hollow-core photonic crystal fiber (HCPCF). In our experiment, the Cs atoms, initially cooled using a magneto-optical trap (MOT), are guided and confined inside a short piece of HCPCF with a magic-wavelength dipole trap. Currently we have successfully implemented a novel detection methods for studying superradiance.
Recent demonstrations of light-matter interactions with atoms and molecules confined to hollow waveguides offer great promise for ultralow-light-level applications. The use of waveguides allows for tight optical confinement over interaction lengths much greater than what could be achieved in bulk geometries. However, the combination of strong atom-photon interactions and nonuniformity of guided light modes gives rise to spectroscopic features that must be understood in order to take full advantage of the properties of such systems. We use light-induced atomic desorption to generate an optically dense Rb vapor at room temperature inside a hollow-core photonic band-gap fiber. Saturable-absorption spectroscopy and passive slow-light experiments reveal large ac Stark shifts, power broadening, and transit-time broadening, that are present in this system even at nanowatt powers.
In this thesis I describe experimental work and present data on the guiding of \nRubidium atoms along free-space propagating light beams as well as within hollow \ncore glass fibres, namely photonic crystal fibres. I describe experiments, laser systems \nand vacuum trap assemblies designed to facilitate this guiding. \nThese experiments are intended to aid progression within the field of cold \natom guidance wherein narrow diameter, long distance hollow-fibre guides are a \ncurrent goal. Realisation of these guides could lead to promising applications such as \natom interferometers and spatially accurate, multi-source, atom depositors. \nHerein, guided fluxes are observed in free-space guiding experiments for \ndistances up to 50mm and up to 10GHz red-detuning from resonance. Additionally \nhollow-core, Kagome structured, quasi- and true-photonic crystal fibres are \ncharacterised. Finally a number of detailed fibre-guiding magneto-optic traps are \ndeveloped. \nBoth cold atomic-beams and cold atomic clouds are reliably positioned above \nfibre entrance facets in conjunction with a guiding laser beam coupled into the fibre \ncore. \nIssues regarding optical flux detection outwith fibre confinement appear to \nhave hindered observation of guided atoms. A far more sensitive detection system has \nbeen developed for use in current, ongoing fibre-guide experiments.
[Truncated] This thesis concerns a new photonic technology based on hollow-core photonic-crystal fibre (HC-PCF) that has been loaded with an atomic vapour. It was demonstrated that this technology may have important applications in the fields of metrology and quantum optics. Furthermore, the small size and robustness of HC-PCF allows these devices to potentially be miniaturised for possible commercial and industrial applications. By filling the HC-PCF with an atomic vapour, excellent light-atom coupling can be attained as both the atoms and light are confined within the same volume. The small transverse dimensions of the fibre’s optical mode leads to high intensities at low input powers, enabling efficient driving of non-linear transitions which would otherwise be difficult with free-space optical systems. Additionally, long interaction lengths, obtained through an arbitrary length of HC-PCF, lead to large optical depths on these typically weak non-linear transitions. The non-linear transition employed here is the 5S1/2 → 5D5/2 rubidium (Rb) two-photon transition. This system is of great interest due to its non-linearity, long excited state lifetime, efficient excitation and large optical depth attained within the HC-PCF. A number of methods for loading a HC-PCF with Rb are discussed, along with proposed ideas for making this process more efficient. Spectroscopic techniques were used to investigate the effect of the fibre’s confined geometry upon the atomic spectra. Extensive theoretical modelling was employed to confirm the observed spectra and give insight to the mechanisms behind the observations. Using this experimental and theoretical knowledge, two applications were targeted: optical atomic frequency standards; and cross phase modulation for quantum logic gates.