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arXiv:2003.00797 · Journal of Physics B Atomic Molecular and Optical Physics

Generation of third-order parametric down-conversion photons via weak nonlinearities

Ying-Qiu He, Dong Ding, Feng-Li Yan, Ting Gao

Published Feb 12, 2021• 0 citations
arXivHTMLPDF

Abstract

Abstract A higher-order parametric down-conversion (PDC) photon state is amazingly different from the states involving independent photon pairs. We focus on the third-order PDC photons. Firstly, we present a symmetry detector which is capable of analyzing twin-beam six-photon symmetric states in the regime of weak nonlinearities. By cascading symmetry detectors, then, it is shown that one can generate third-order PDC photons from a class of twin-beam six-photon symmetric states. Finally, as an example, we describe an application of third-order PDC photons for exploring six-mode-photon entangled states with linear optics.

DOI
10.1088/1361-6455/abe5c8

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Abstract A higher-order parametric down-conversion (PDC) photon state is amazingly different from the states involving independent photon pairs. We focus on the third-order PDC photons. Firstly, we present a symmetry detector which is capable of analyzing twin-beam six-photon symmetric states in the regime of weak nonlinearities. By cascading symmetry detectors, then, it is shown that one can generate third-order PDC photons from a class of twin-beam six-photon symmetric states. Finally, as an example, we describe an application of third-order PDC photons for exploring six-mode-photon entangled states with linear optics.
We describe a method to detect twin-beam multiphoton entanglement based on a beam splitter and weak nonlinearities. For the twin-beam four-photon entanglement, we explore a symmetry detector. It works not only for collecting two-pair entangled states directly from the spontaneous parametric down-conversion process, but also for generating them by cascading these symmetry detectors. Surprisingly, by calculating the iterative coefficient and the success probability we show that with a few iterations the desired two-pair can be obtained from a class of four-photon entangled states. We then generalize the symmetry detector to n-pair emissions and show that it is capable of determining the number of the pairs emitted indistinguishably from the spontaneous parametric down-conversion source, which may contribute to explore multipair entanglement with a large number of photons.
Nowadays, the nonlinear optical process of spontaneous parametric down-conversion is considered as the canonical approach for creating entangled-photon pairs. We consider three pairs of entangled photons emitted by the parametric down-conversion source, and introduce a setup for evolving these photons based on linear optics, which is composed of several polarizing beam splitters, beam splitters, and half wave plates. By using the parametric down-conversion source and the setup, we carefully design an efficient scheme for preparing six-photon hyperentangled states in both the polarization and the spatial degrees of freedom. Because we use almost all possible behaviors of the three pairs of entangled photons, the present scheme is efficient for creating six-photon hyperentangled states. Next, in the regime of weak nonlinearity we design a quantum nondemolition detection to distinguish the two cases of photons in two special spatial modes. It is worth pointing out that our scheme is much easier to realize, since the strength of the nonlinearities in the process of quantum nondemolition detection can be restricted to the scalable orders of magnitude in practicality.
The generation of multi-photon quantum states in integrated waveguiding structures provides a route to the creation of quantum optical chips. In particular, the simultaneous generation of photons through spontaneous parametric down-conversion (SPDC) and their quantum walks in nonlinear waveguide arrays (WGAs) can be used to produce strongly spatially entangled biphoton states [1] with applications for quantum search algorithms [2]. Whereas up to now only arrays of single-mode nonlinear waveguides have been considered for SPDC, in general the waveguides may support several guided modes, which were demonstrated to strongly affect nonlinear wave mixing in the classical regime [3]. Here we show that using higher order modes for SPDC has a significant influence on the generated two-photon states and gives additional means to control them. In particular, we employ the symmetry of the modes to engineer effectively nonlocal photon pair generation by SPDC.
Parametric down-conversion (PDC) is one of the most widely used methods to create pure single-photon states for quantum information applications. However, little attention has been paid to higher-order photon components in the PDC process, yet these ultimately limit the prospects of generating single photons of high quality. In this paper we investigate the impact of higher-order photon components and multiple frequency modes on the heralding rates and single-photon fidelities. This enables us to determine the limits of PDC sources for single-photon generation. Our results show that a perfectly single-mode PDC source in conjunction with a photon-number-resolving detector is ultimately capable of creating single-photon Fock states with unit fidelity and a maximal state creation probability of 25%. Hence, an array of 17 switched sources is required to build a deterministic ($>999999%$ emission probability) pure single-photon source.
We investigate production of three-photon states in cascaded parametric down-conversion (PDC). The analysis includes preparation of Greenberger-Horne-Zeilinger polarization-entangled states in cascaded type-II and type-I PDC in the framework of considering the dual-grid structure that involves two periodically poled crystals. Considering cascaded optical parametric oscillator (OPO) driven by a sequence of laser pulses with Gaussian time-dependent envelopes, we investigate quantum statistical properties of high intensity mode generated in intracavity three-photon splitting. Calculating the normalized third-order correlation function below-and at the generation threshold, we demonstrate that in the pulsed regime, depending on the duration of pulses and the time-interval separations between them, the degree of three-photon-number correlation essentially exceed the analogous one for the case of continuous pumping.
Parametric down-conversion (PDC) is mostly known in the low-gain (spontaneous) regime, in which the correlated photon pairs are produced. Spontaneous PDC (SPDC) plays a very important role for quantum optics as a variety of quantum states is produced via SPDC. In the high-gain case PDC leads to generation of bright states having up to hundreds mW mean power. With such states almost any nonlinear optical interaction or light-matter interaction becomes more efficient. Even being macroscopically bright, the produced states maintain nonclassical properties as, for example, the fluctuations of electric field quadratures are squeezed below the shot-noise level. The high-gain PDC could be used not only in the same applications as SPDC, it also can provide new ones. Apart from that the high-gain PDC has many remarkable spectral and statistical properties, which are in the focus of this work. The description starts from the PDC generation in normal and anomalous group velocity dispersion ranges. The spectrum and mode content of high-gain PDC is considered as well as their change with the parametric gain are demonstrated. Then, there are the interference effects emerging from the PDC correlations presented, namely the macroscopic analogue of the Hong-Ou-Mandel interference. In addition, it is shown how spatial and temporal walk-off matching could be used for the generation of giant narrowband twin beams. Finally, the statistical properties of high-gain PDC are reviewed as well as their use for multiphoton effects is demonstrated. Photon-number fluctuations of PDC are studied via normalized correlation functions and probability distributions. These fluctuations enhance the generation efficiency for multiphoton effects by orders of magnitude and lead to tremendously fluctuating light described by heavy-tailed photon-number probability distributions.