Abstract Exponential decay laws describe systems ranging from unstable nuclei to fluorescent molecules, in which the probability of jumping to a lower-energy state in any given time interval is static and history-independent. These decays, involving only a metastable state and fluctuations of the quantum vacuum, are the most fundamental nonequilibrium process and provide a microscopic model for the origins of irreversibility. Despite the fact that the apparently universal exponential decay law has been precisely tested in a variety of physical systems, it is a surprising truth that quantum mechanics requires that spontaneous decay processes have nonexponential time dependence at both very short and very long times. Cold-atom experiments have proven to be powerful probes of fundamental decay processes; in this article, we propose the use of Bose condensates in Floquet–Bloch bands as a probe of long-time nonexponential decay in single isolated emitters. We identify a range of parameters that should enable observation of long-time deviations and experimentally demonstrate a key element of the scheme: tunable decay between quasi-energy bands in a driven optical lattice.
Abstract Exponential decay laws describe systems ranging from unstable nuclei to fluorescent molecules, in which the probability of jumping to a lower-energy state in any given time interval is static and history-independent. These decays, involving only a metastable state and fluctuations of the quantum vacuum, are the most fundamental nonequilibrium process and provide a microscopic model for the origins of irreversibility. Despite the fact that the apparently universal exponential decay law has been precisely tested in a variety of physical systems, it is a surprising truth that quantum mechanics requires that spontaneous decay processes have nonexponential time dependence at both very short and very long times. Cold-atom experiments have proven to be powerful probes of fundamental decay processes; in this article, we propose the use of Bose condensates in Floquet–Bloch bands as a probe of long-time nonexponential decay in single isolated emitters. We identify a range of parameters that should enable observation of long-time deviations and experimentally demonstrate a key element of the scheme: tunable decay between quasi-energy bands in a driven optical lattice.
The most important law of radioactivity is that of the exponential decay. In the realm of quantum mechanics, however, this decay law is neither rigorous nor fundamental. The deviations from the exponential decay have been observed experimentally at the early stage of a decay process, but there is little evidence for nonexponential behavior at long times. Yet such long-term nonexponentiality is expected theoretically to probe the nonresonant background components of the initial wave function which preserve the structural interference and the memory of how the state was created. In this paper, we propose new observables that can be used for experimental investigations of the post-exponential decay regime, including the decay of threshold resonances, particle correlations in three-body decays, and interference between near-lying resonances. While the specific examples presented in this work pertain to atomic nuclei, the properties of nonexponential decay are generic, i.e., they apply to other many-body open quantum systems, such as hadrons, atoms, molecules, and nanostructures.
Summary form only given.We report the observation of short-time deviation from exponential decay in a quantum tunneling experiment. Our system consists of ultracold sodium atoms that are trapped in an accelerating periodic optical potential created by a standing wave of light. Atoms can escape the wells via quantum tunneling, and the number that remain is measured as a function of interaction time for a fixed value of the well depth and acceleration. To study tunneling in this system, sodium atoms are first trapped and cooled in a magneto-optical trap. The trapping beams as well as the magnetic field gradient are then turned off, and an accelerating far-detuned standing wave of light is turned on. A three-step acceleration is implemented to measure the loss due to tunneling. Once the final velocity is reached, the potential is turned off and the atomic fluorescence is imaged after a free drift time. We have measured the survival probability and found that the initial survival probability is flat and then crosses over to an exponential decay. The intermediate stage is characterized by a time-dependent loss rate. To analyze the short-time tunneling probability and the approach to exponential decay, we use a simple model of the band structure with a single (trapped) band separated by a bandgap from a free particle state. We find an analytic expression for the survival probability that is quadratic for the first few microseconds of evolution, with a crossover to exponential decay at long times. We show that this crossover time is related to the tunneling time. We also identify a new parameter regime where coherent oscillations of the survival probability are seen.
We report Floquet band engineering of long-range transport and direct imaging of Floquet-Bloch bands in an amplitude-modulated optical lattice. In one variety of Floquet-Bloch bands we observe tunable rapid long-range high-fidelity transport of a Bose condensate across thousands of lattice sites. Quenching into an opposite-parity Floquet-hybridized band allows Wannier-Stark localization to be controllably turned on and off using modulation. A central result of this work is the use of transport dynamics to demonstrate direct imaging of a Floquet-Bloch band structure. These results demonstrate that transport in dynamical Floquet-Bloch bands can be mapped to transport in quasistatic effective bands, opening a path to cold atom quantum emulation of ultrafast multiband electronic dynamics.
Quantum emulation of extreme non-equilibrium phenomena is a natural application of the precision and control of ultracold atomic physics experiments. In particular, ``Floquet engineering" with an explicitly time-dependent Hamiltonian enables the creation of states of matter that can only exist in the presence of strong driving. In this work, we create and study such tunable strongly driven quantum systems. We use quantum degenerate lithium as a platform because of its light mass, fast tunneling rates, and broadly tunable Feshbach resonance, which allow the study of a wide variety of systems: noninteracting Bosons, strongly interacting many body systems, and bright solitons, to name a few. We describe the experimental setup used to create a 7Li Bose-Einstein condensate as an archetypal quantum platform, and then discuss three key results: the first direct measurement of position-space Bloch oscillations in a cold atom system, the creation of a massive relativistic harmonic oscillator, and finally the demonstration of a new method for controlled long-range quantum coherent transport enabled by Floquet band engineering.
The decay profile of a metastable quantum state decaying in isolation is predicted to depart from exponential behaviour after many lifetimes, and in typical cases to adopt algebraic behaviour as the late-time limit. The effect of environmental interactions, including measurement, is quite different from that of the familiar Zeno (and anti-Zeno) effects that have been observed at very early times. Instead of arresting the decay (or hastening it), the late-time interactions tend to enforce the exponential decay law, without substantially changing the decay constant intrinsic to the isolated system. The experimental challenge is to prevent these interactions and observe the crossover to the nonexponential regime.
Strong periodic driving of cavity-quantum electrodynamics (QED) in the ultrastrong-coupling regime creates nonequilibrium states whose dissipation is governed by Floquet quasienergies rather than undriven dressed resonances. However, modeling such a regime is a significant theoretical challenge, including a number of subtle problems such as the need to ensure gauge invariance for truncated matter-cavity systems with time-dependent driving. To fill this theoretical gap, we introduce a nonsecular Floquet generalized master equation framework for strongly driven open cavity-QED systems, formulated in the dressed basis of the quantum Rabi model and applicable to structured reservoirs without rotating-wave approximations. Our theory can thus model Floquet-driven dynamics in open ultrastrong-coupling cavity-QED, and demonstrates a wide range of quantum state control. Using strong optical pumping and parametric mechanical modulation, we compute long-time populations, fluorescence spectra, and the Floquet-Liouville eigenspectra, resolving observable resonances into hybridized quasienergy channels and decay rates. By systematically comparing with conventional time-independent dressed-basis generalized master equations, we show that static approaches only reproduce steady-state populations in restricted excitation regimes, and fail for frequency-resolved observables and break down under appropriate Floquet engineering, surprisingly, even for spectrally flat baths. Structured environments, such as Lorentzian-Ohmic reservoirs, further amplify these discrepancies through sideband-selective decay. Our results demonstrate that dissipation in driven ultrastrong cavity-QED is intrinsically quasienergy resolved and we establish Floquet-dissipative theory as an accurate and powerful framework for predicting spectra, controlling decay pathways, and engineering nonequilibrium quantum states and reservoirs.