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arXiv:2002.01480 · New Journal of Physics

Precise high-fidelity electron–nuclear spin entangling gates in NV centers via hybrid dynamical decoupling sequences

Wenzheng Dong, F A Calderon-Vargas, Sophia E Economou

Published Jun 11, 2020• 14 citations
arXivHTMLPDF

Abstract

Abstract Color centers in solids, such as the nitrogen-vacancy center in diamond, offer well-protected and well-controlled localized electron spins that can be employed in various quantum technologies. Moreover, the long coherence time of the surrounding spinful nuclei can enable a robust quantum register controlled through the color center. We design pulse sequence protocols that drive the electron spin to generate robust entangling gates with these nuclear memory qubits. We find that compared to using Carr-Purcell-Meiboom-Gill (CPMG) alone, Uhrig decoupling sequence and hybrid protocols composed of CPMG and Uhrig sequences improve these entangling gates in terms of fidelity, spin control range, and spin selectivity. We provide analytical expressions for the sequence protocols and also show numerically the efficacy of our method on nitrogen-vacancy centers in diamond. Our results are broadly applicable to color centers weakly coupled to a small number of nuclear spin qubits.

DOI
10.1088/1367-2630/ab9bc0

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Abstract Color centers in solids, such as the nitrogen-vacancy center in diamond, offer well-protected and well-controlled localized electron spins that can be employed in various quantum technologies. Moreover, the long coherence time of the surrounding spinful nuclei can enable a robust quantum register controlled through the color center. We design pulse sequence protocols that drive the electron spin to generate robust entangling gates with these nuclear memory qubits. We find that compared to using Carr-Purcell-Meiboom-Gill (CPMG) alone, Uhrig decoupling sequence and hybrid protocols composed of CPMG and Uhrig sequences improve these entangling gates in terms of fidelity, spin control range, and spin selectivity. We provide analytical expressions for the sequence protocols and also show numerically the efficacy of our method on nitrogen-vacancy centers in diamond. Our results are broadly applicable to color centers weakly coupled to a small number of nuclear spin qubits.
Color centers in diamond provide a possible hardware for quantum computation, where the most basic quantum information processing unit are nitrogen-vacancy (NV) centers, each in contact with adjacent carbon nuclear spins. With specifically tailored dynamical decoupling sequences, it is possible to execute selective, high-fidelity two-body gates between the electron spin of the NV center and a targeted nuclear spin. In this work, we present a method to determine the optimal execution time that balances the trade-off between fidelity and execution speed for gates generated by adaptive XY sequences. With these optimized gates, we use the nuclear spin environment as a code space for quantum error correction within a color center register.
Abstract A nitrogen-vacancy (NV) center in a diamond enables the access to an electron spin, which is expected to present highly sensitive quantum sensors. Although exploiting a nitrogen nuclear spin improves the sensitivity, manipulating it using a resonant pulse requires a long gate time owing to its small gyromagnetic ratio. Another technique to control nuclear spins is a conditional rotation gate based on dynamical decoupling, which is faster but unavailable for nitrogen spins owing to the lack of transverse hyperfine coupling with the electron spin. In this study, we generated effective transverse coupling by applying a weak off-axis magnetic field. An effective coupling depends on the off-axis field; the conditional rotation gate on the nitrogen-14 spins of an NV center was demonstrated within 4.2 μs under an 1.8% off-axis field and a longitudinal field of approximately 280 mT. We estimated that a population transfer from the electron to nitrogen spins can be implemented with 8.7 μs. Our method is applicable to an ensemble of NV centers, in addition to a single NV center.
Selective control of qubits in a quantum register for the purposes of quantum information processing represents a critical challenge for dense spin ensembles in solid-state systems. Here we present a protocol that achieves a complete set of selective electron-nuclear gates and single nuclear rotations in such an ensemble in diamond facilitated by a nearby nitrogen-vacancy (NV) center. The protocol suppresses internuclear interactions as well as unwanted coupling between the NV center and other spins of the ensemble to achieve quantum gate fidelities well exceeding 99%. Notably, our method can be applied to weakly coupled, distant spins representing a scalable procedure that exploits the exceptional properties of nuclear spins in diamond as robust quantum memories.
Nitrogen-vacancy (NV) centers in diamond provide room-temperature electron-nuclear spin registers for quantum sensing and quantum information processing, with surrounding 13C nuclear spins serving as long-lived quantum memories. However, coherent control of large nuclear-spin registers is limited by finite electron-spin coherence and spectral addressability. Existing approaches follow two complementary strategies: dynamical-decoupling (DD) gates exploit filter-function resonances to realize selective conditional evolution but permit only discrete rotation angles, whereas dynamical-decoupling radio-frequency (DDrf) control restores continuous tunability at the cost of stringent hyperfine-geometry and RF-power requirements. Here, we introduce hybrid dynamical-decoupling and radio-frequency (H-DDrf) control, which preserves the DD-induced conditional evolution and employs a geometrically phase-matched RF drive to complete the target operation. This approach reduces both RF power and gate duration while maintaining high-fidelity control, thereby expanding the accessible 13C nuclear-spin register for room-temperature NV-based quantum memories and quantum processors.
The electron spin of a nitrogen-vacancy center in diamond lends itself to the control of proximal 13C^{13}\mathrm{C}13C nuclear spins via dynamical decoupling methods, possibly combined with radio-frequency driving. Long-lived single-qubit states and high-fidelity electron-nuclear gates required for the realization of a multiqubit register have already been demonstrated. Towards the goal of a scalable architecture, linking multiple such registers in a photonic network represents an important step. Multiple pairs of remotely entangled qubits can enable advanced algorithms or error correction protocols. We investigate how a photonic architecture can be extended from the intrinsic nitrogen spin to multiple 13C^{13}\mathrm{C}13C spins per node. Applying decoherence-protected gates sequentially, we simulate the fidelity of creating multiple pairs of remotely entangled qubits. Even though the currently achieved degree of control of 13C^{13}\mathrm{C}13C spins might not be sufficient for large-scale devices, the two schemes are compatible in principle. One requirement is the correction of unconditional phases acquired by unaddressed nuclear spins during a decoupling sequence.
Motivated by the recent experimental progress in exploring the use of a nitrogen-vacancy (NV) center in diamond as a quantum computing platform, we propose schemes for fast and high-fidelity entangling gates on this platform. Using both analytical and numerical calculations, we demonstrate that synchronization effects between resonant and off-resonant transitions may be exploited such that spin-flip errors due to strong driving may be eliminated by adjusting the gate time or the driving field. This allows for fast, high-fidelity entangling operations between the electron spin and one or several nuclear spins. We investigate a two-qubit system where the NV center comprises a N 15 atom and a qubit-qutrit system for the case of a N 14 atom. In both cases, we predict a complete suppression of off-resonant driving errors for two-qubit gates when addressing the NV electron spin conditioned on states of nuclear spins of the nitrogen atom of the defect. Additionally, we predict fidelities > 0.99 for multiqubit gates when including the surrounding C 13 atoms in the diamond lattice in the conditioned logic.