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arXiv:2001.06000 · Physical Review Research

Characterizing spin-one Kitaev quantum spin liquids

Ilia Khait, P. Peter Stavropoulos, Hae-Young Kee, Yong Baek Kim

Published Feb 18, 2021• 48 citations
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Abstract

The authors study the $S$=1 Kitaev model using the density matrix renormalization group, and characterize the magnetic phase diagram of cylindric ladder geometries to find evidence for an intermediate phase for antiferromagnetic Kitaev couplings.

DOI
10.1103/physrevresearch.3.013160

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The authors study the SSS=1 Kitaev model using the density matrix renormalization group, and characterize the magnetic phase diagram of cylindric ladder geometries to find evidence for an intermediate phase for antiferromagnetic Kitaev couplings.
This paper studies the phase diagram for the SSS=1 Kitaev model using a density renormalization group method. The authors find a gapped Kitaev spin liquid with topological nature for both ferromagnetic and antiferromagnetic Kitaev couplings. Further, the the antiferromagnetic Kitaev coupling hosts a more robust topological spin liquid with an additional nonmagnetic intermediate phase
We study an extended Kitaev-Heisenberg model including additional anisotropic couplings by using the two-dimensional density-matrix renormalization group method. Calculating the ground-state energy, entanglement entropy, and spin-spin correlation functions, we make a phase diagram of the extended Kitaev-Heisenberg model around the spin-liquid phase. We find a zigzag antiferromagnetic phase, a ferromagnetic phase, a ${120}^{\ensuremath{\circ}}$ antiferromagnetic phase, and two kinds of incommensurate phases around the Kitaev spin-liquid phase. Furthermore, we study the entanglement spectrum of the model, and we find that entanglement levels in the Kitaev spin-liquid phase are degenerate forming pairs, but those in the magnetically ordered phases are nondegenerate. The Schmidt gap defined as the energy difference between the lowest two levels changes at the phase boundary adjacent to the Kitaev spin-liquid phase. However, we find that phase boundaries between magnetically ordered phases do not necessarily agree with the change of the Schmidt gap.
Recently, it has been proposed that higher-spin analogs of the Kitaev interactions K>0K>0K>0 may also occur in a number of materials with strong Hund's and spin-orbit coupling. In this work, we use Lanczos diagonalization and density matrix renormalization group methods to investigate numerically the S=1S=1S=1 Kitaev-Heisenberg model. The ground-state phase diagram and quantum phase transitions are investigated by employing local and nonlocal spin correlations. We identify two ordered phases at negative Heisenberg coupling J<0J<0J<0: a ferromagnetic phase with $\ensuremath{\langle}{S}_{i}^{z}{S}_{i+1}^{z}\ensuremath{\rangle}>0$ and an intermediate left-left-right-right phase with $\ensuremath{\langle}{S}_{i}^{x}{S}_{i+1}^{x}\ensuremath{\rangle}\ensuremath{\ne}0$. A quantum spin liquid is stable near the Kitaev limit, while a topological Haldane phase is found for J>0J>0J>0.
The Kitaev model, whose ground state is a quantum spin liquid (QSL), was originally conceived for spin S=1/2S=1/2S=1/2 moments on a honeycomb lattice. In recent years, the model has been extended to higher SSS from both theoretical and experimental interests, but the stability of the QSL ground state has not been systematically clarified for general SSS, especially in the presence of other additional interactions, which inevitably exist in candidate materials. Here we study the spin-SSS Kitaev-Heisenberg models by using an extension of the pseudofermion functional renormalization group method to general SSS. We show that, similar to the S=1/2S=1/2S=1/2 case, the phase diagram for higher SSS contains the QSL phases in the vicinities of the pristine ferromagnetic and antiferromagnetic Kitaev models, in addition to four magnetically ordered phases. We find, however, that the QSL phases shrink rapidly with increasing SSS, becoming vanishingly narrow for $S\ensuremath{\ge}2$, whereas the phase boundaries between the ordered phases remain almost intact. Our results provide a reference for the search for higher-SSS Kitaev materials.
Abstract Doped quantum magnets, especially spin liquids with fractionalized excitations, have long attracted attention as a promising path towards unconventional superconductivity. We investigate the hole-doped Kitaev-Heisenberg ( t – J – K ) model on a two-leg ladder geometry using the density-matrix renormalization group (DMRG). We consider the behavior of the antiferromagnetic Kitaev spin-liquid phase as a function of hopping strength t and doping level. This reveals intriguing pairing tendencies only for tK≲0.65\frac{t}{K}\lesssim 0.65Kt​≲0.65 t K ≲ 0.65 , consistent with prior results on three-leg ladders, and firmly supports the emerging picture that the physics of doped Kitaev spin liquids strongly depends on the kinetic energy of the doped holes. Analysis of one- and two-hole doping uncovers close links between spatial profiles of the plaquette operator and the charge density. We also construct a doping-dependent phase diagram for antiferromagnetic Heisenberg interactions and intermediate hopping t = 1. Upon doping, the rung-singlet region develops dominant superconducting correlations. Spin-density wave-like behavior is found in the Kitaev limits, and in the stripy phase.