We study the formation and collision-aided decay of an ultracold atomic Bose-Einstein condensate in the first excited band of a double-well two-dimensional optical lattice with weak harmonic confinement in the perpendicular
z direction. This lattice geometry is based on an experiment by Wirth et al. [Nat. Phys. 7, 147 (2010)]. The double well is asymmetric, with the local ground state in the shallow well nearly degenerate with the first excited state of the adjacent deep well. We compare the band structure obtained from a tight-binding model with that obtained numerically using a plane-wave basis. We find the tight-binding model to be in quantitative agreement for the lowest two bands, in qualitative agreement for the next two bands, and inadequate for even higher excited bands. The bandwidths of the excited bands are much larger than the harmonic-oscillator energy spacing in the
z direction. We then study the thermodynamics of a noninteracting Bose gas in the first excited band. We estimate the condensate fraction and critical temperature
Tc as functions of the lattice parameters. For typical atom numbers, the critical energy
kBTc, with
kB the Boltzmann constant, is larger than the excited bandwidths and harmonic-oscillator energy. Using conservation of total energy and atom number, we show that the temperature increases after the lattice transformation. Finally, we estimate the time scale for a two-body collision-aided decay of the condensate as a function of the lattice parameters. The decay involves two processes, the dominant one in which both colliding atoms decay to the ground band, and the second involving excitation of one atom to a higher band. For this estimate, we have used tight-binding wave functions for the lowest four bands and numerical estimates for higher bands. The decay rate rapidly increases with lattice depth, but close to the critical temperature, it stays smaller than the tunneling rate between the
s and
p orbitals in adjacent wells.
The kinetics of the formation of coherent correlation properties associated with Bose condensation is studied in detail. The evolution of a nonequilibrium state with no “condensate-seed” is related to a hierarchy of relaxation times. At the first stage, a particle flux in energy space toward low energies sets in. The evolution in this case is described by a nonlinear Boltzmann equation, with a characteristic time given by interparticle collisions. When the particles which will later form the condensate have a kinetic energy which is less than the potential energy, a quasicondensate starts to form. In this stage, fluctuations of the density (but not of the phase) are suppressed and short-range coherent correlation properties are governed by the equation of motion for a quasiclassical complex field. The next stage is connected with the formation of the long-range order. The time for forming topological order and therefore genuine superfluidity proves to be dependent on the system size. The off-diagonal long-range order, arising after the attenuation of long-wave phase fluctuations, has a size-dependent relaxation time as well. Introduction The problem of Bose–Einstein Condensation (BEC) kinetics, being interesting in itself, has acquired a special significance in connection with experimental efforts to observe this condensation in a number of systems with particles with a finite lifetime. Such systems include spin-polarized atomic hydrogen [1], excitons [2] and biexcitons [3] in semiconductors and, more recently, laser-cooled atomic systems [4].
Abstract This article provides a synopsis of our recent experimental work exploring Bose–Einstein condensation in metastable higher Bloch bands of optical lattices. Bipartite lattice geometries have allowed us to implement appropriate band structures, which meet three basic requirements: the existence of metastable excited states sufficiently protected from collisional band relaxation, a mechanism to excite the atoms initially prepared in the lowest band with moderate entropy increase, and the possibility of cross-dimensional tunneling dynamics, necessary to establish coherence along all lattice axes. A variety of bands can be selectively populated and a subsequent thermalization process leads to the formation of a condensate in the lowest energy state of the chosen band. As examples the 2nd, 4th and 7th bands in a bipartite square lattice are discussed. The geometry of the 2nd and 7th bands can be tuned such that two inequivalent energetically degenerate energy minima arise at the X ± -points at the edge of the 1st Brillouin zone. In this case even a small interaction energy is sufficient to lock the phase between the two condensation points such that a complex-valued chiral superfluid order parameter can emerge, which breaks time reversal symmetry. In the 4th band a condensate can be formed at the Γ-point in the center of the 1st Brillouin zone, which can be used to explore topologically protected band touching points. The new techniques to access orbital degrees of freedom in higher bands greatly extend the class of many-body scenarios that can be explored with bosons in optical lattices.
We study the nonequilibrium dynamics of a Bose-Einstein condensate that is split in a harmonic trap by turning up a periodic optical lattice potential. We evaluate the dynamical evolution of the phase coherence along the lattice and the number fluctuations in individual lattice sites within the stochastic truncated Wigner approximation when several atoms occupy each site. We show that the saturation of the number squeezing at high lattice strengths, which was observed in recent experiments by Orzel et al. [Science 291, 2386 (2001)] can be explained by the nonadiabaticity of the splitting.
We study the dynamics of a Bose-Einstein condensate in a double-well potential in the two-mode approximation. The dissipation of energy from the condensate is described by the coupling to a thermal reservoir of noncondensate modes. As a consequence of the coupling, the self-locked population imbalance in the macroscopic quantum self-trapping decays away. We show that a coherent state predicted by spontaneous symmetry breaking is not robust and decoheres rapidly into a statistical mixture due to the interactions between condensate and noncondensate atoms. However, via stochastic simulations we find that with a sufficiently fast measurement rate of the relative phase between the two wells the matter wave coherence is established even in the presence of the decoherence.
Photo-excited excitons, i.e. closely bound electron-hole pairs, are in the low-density regime approximately bosons. For sufficiently low temperatures and sufficiently high densities of the exciton gas, a nonequilibrium phase transition in the form of a Bose-Einstein condensation (BEC) can be expected. Various levels of the description of the kinetics of relaxation and condensation due to the coupling of the excitons to a cold reservoir of acoustic phonons are discussed. For noninteracting excitons a rate equation approach with the exciton Boltzmann equation can be used. For interacting excitons the nonmarkovian quantum kinetics is required for the description of the BEC in order to incorporate the changes of the energy spectrum during the condensation self-consistently. Finally colored Langevin fluctuations can be used to calculate the phase diffusion of the condensate.