Abstract Spatial modes of light directly give the most easily accessible degree of freedom that span an infinite dimensional Hilbert space. The higher dimensional spatial mode entanglement realized using spontaneous parametric down conversion (SPDC) process is generally restricted to the subspace defined by a single spatial mode in pump. Access to other modal subspaces can be realized by pumping beams carrying several easily tunable transverse modes. As a proof of principle experiment, we generate twin-photon states in an SPDC process with pump as a superposition of first order Laguerre–Gaussian (or Hermite–Gaussian) modes. We show that the generated states can be easily tuned between different subspaces by controlling the respective modal content in the pump superposition.
Abstract Spatial modes of light directly give the most easily accessible degree of freedom that span an infinite dimensional Hilbert space. The higher dimensional spatial mode entanglement realized using spontaneous parametric down conversion (SPDC) process is generally restricted to the subspace defined by a single spatial mode in pump. Access to other modal subspaces can be realized by pumping beams carrying several easily tunable transverse modes. As a proof of principle experiment, we generate twin-photon states in an SPDC process with pump as a superposition of first order Laguerre–Gaussian (or Hermite–Gaussian) modes. We show that the generated states can be easily tuned between different subspaces by controlling the respective modal content in the pump superposition.
Spontaneous parametric downconversion (SPDC) in quantum optics is an invaluable resource for the realization of high-dimensional qudits with spatial modes of light. One of the main open challenges is how to directly generate a desirable qudit state in the SPDC process. This problem can be addressed through advanced computational learning methods; however, due to difficulties in modeling the SPDC process by a fully differentiable algorithm, progress has been limited. Here, we overcome these limitations and introduce a physically constrained and differentiable model, validated against experimental results for shaped pump beams and structured crystals, capable of learning the relevant interaction parameters in the process. We avoid any restrictions induced by the stochastic nature of our physical model and integrate the dynamic equations governing the evolution under the SPDC Hamiltonian. We solve the inverse problem of designing a nonlinear quantum optical system that achieves the desired quantum state of downconverted photon pairs. The desired states are defined using either the second-order correlations between different spatial modes or by specifying the required density matrix. By learning nonlinear photonic crystal structures as well as different pump shapes, we successfully show how to generate maximally entangled states. Furthermore, we simulate all-optical coherent control over the generated quantum state by actively changing the profile of the pump beam. Our work can be useful for applications such as novel designs of high-dimensional quantum key distribution and quantum information processing protocols. In addition, our method can be readily applied for controlling other degrees of freedom of light in the SPDC process, such as spectral and temporal properties, and may even be used in condensed-matter systems having a similar interaction Hamiltonian.
Spontaneous parametric down-conversion in quantum optics is an invaluable resource for the realization of high-dimensional qudits with spatial modes of light. One of the main open challenges is how to directly generate a desirable qudit state in the SPDC process. This problem can be addressed through advanced computational learning methods; however, due to difficulties in modeling the SPDC process by a fully differentiable algorithm that takes into account all interaction effects, progress has been limited. Here, we overcome these limitations and introduce a physically-constrained and differentiable model, validated against experimental results for shaped pump beams and structured crystals, capable of learning every interaction parameter in the process. We avoid any restrictions induced by the stochastic nature of our physical model and integrate the dynamic equations governing the evolution under the SPDC Hamiltonian. We solve the inverse problem of designing a nonlinear quantum optical system that achieves the desired quantum state of down-converted photon pairs. The desired states are defined using either the second-order correlations between different spatial modes or by specifying the required density matrix. By learning nonlinear volume holograms as well as different pump shapes, we successfully show how to generate maximally entangled states. Furthermore, we simulate all-optical coherent control over the generated quantum state by actively changing the profile of the pump beam. Our work can be useful for applications such as novel designs of high-dimensional quantum key distribution and quantum information processing protocols. In addition, our method can be readily applied for controlling other degrees of freedom of light in the SPDC process, such as the spectral and temporal properties, and may even be used in condensed-matter systems having a similar interaction Hamiltonian.
Abstract In this work, we investigate the orbital angular momentum (OAM) spectrum of photons generated via spontaneous parametric down-conversion (SPDC) and study how shaping the transverse profile of the pump beam influences the resulting spectrum. Using a perfect optical vortex (POV) mode as the pump, we show that the OAM spectrum narrows significantly, leading to purer OAM states. We further examine the entanglement between the down-converted photons in the OAM basis, finding that Laguerre–Gaussian (LG) pumped photons exhibit increased higher-dimensional entanglement at the expense of mode purity.
High-dimensional spatial entanglement generated via spontaneous parametric down-conversion (SPDC) provides a powerful resource for quantum information processing, yet its mode structure becomes increasingly complex when the pump occupies a higher-order Laguerre--Gaussian (LG) mode. Here, we develop an algebraic framework for characterizing biphoton spatial-mode entanglement by factorizing LG-pumped SPDC into a spatial-mode beam-splitter transformation followed by spatial two-mode squeezing. By choosing the biphoton LG basis radius as the geometric mean of the pump-beam radius and the crystal-induced correlation width, we obtain a natural modal basis in which the two operations can be treated separately. When the pump-beam radius matches the correlation width, spatial squeezing vanishes, and the two circular-mode components of the pump are independently conserved across the signal and idler photons, leading to conservation of both orbital angular momentum and the total spatial mode number. We further derive an analytical expression for the Schmidt number for arbitrary LG pump modes and squeezing strengths, revealing how the radial and azimuthal pump indices govern the dimensionality of the spatial entanglement. This algebraic characterization provides a unified description of the mode structure, conservation laws, and entanglement dimensionality of higher-order-LG-pumped SPDC.
Spontaneous parametric down-conversion (SPDC) has been a reliable process for the generation of entangled photon pairs. In this process, a nonlinear quadratic crystal is pumped by a laser field in order to convert (high-energy) photons into correlated photon pairs whose efficient control plays an essential role in various applications of quantum information processing. In particular, the amount of entanglement has been successfully controlled by adjusting the spatial structure of the incident pump field. Here, we theoretically analyze how the entanglement of the down-converted two-photon state can be further enhanced by using Ince-Gaussian beams with well-defined ellipticity $\ensuremath{\epsilon}$, i.e., solutions of the paraxial wave equation in elliptical coordinates. These spatially structured beams are quite universal as they include both the Laguerre-Gaussian beams for $\ensuremath{\epsilon}\ensuremath{\rightarrow}0$ as well as the Hermite-Gaussian beams for $\ensuremath{\epsilon}\ensuremath{\rightarrow}\ensuremath{\infty}$. We demonstrate that the entanglement of the generated photon pairs in SPDC can be maximized by a proper choice of $\ensuremath{\epsilon}$ and that such an enhanced entanglement can be observed experimentally in terms of the Schmidt number.
The two-photon state generated by spontaneous parametric down-conversion (SPDC) exhibit spatial entanglement embedded in the corresponding mode function. The control of the spatial characteristics of the generated two-photon state is an issue of paramount importance. For example, the spatial entanglement of the two down converted photons forms the basis of quantum imaging, and entanglement in orbital angular momentum has opened a new scenario for implementing multidimensional Hilbert spaces. We put forward several techniques to engineer the spatial structure of entangled two-photon states generated in SPDC. The first strategy we consider for spatial control of the quantum state makes use of the direct manipulation of the pump beam. This technique makes feasible to prepare arbitrary engineered entangled states in any d-dimensional Hilbert space. The second strategy is based on the proper preparation of the down-converting crystal itself, namely quantum state manipulation by quasi-phase-matching (QPM) engineering. We use properly designed transversely varying QPM gratings in nonlinear crystals.