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arXiv:1911.00255 · Physical Review A

Ground-state phase diagram and excitation spectrum of a Bose-Einstein condensate with spin-orbital-angular-momentum coupling

Ke-Ji Chen, Fan Wu, Jianshen Hu, Lianyi He

Published Jul 16, 2020• 20 citations
arXivHTMLPDF

Abstract

We investigate the ground-state phase diagram and excitation spectrum of an interacting spinor Bose-Einstein condensate with spin-orbital-angular-momentum (SOAM) coupling realized in recent experiments by introducing atomic Raman transition with a pair of copropagating Laguerre-Gaussian laser beams that carry different orbital angular momenta (OAM) [Chen et al., Phys. Rev. Lett. 121, 113204 (2018) and Zhang et al., Phys. Rev. Lett. 122, 110402 (2019)]. Because of the ground-state degeneracy of the single-particle Hamiltonian at vanishing detuning, several angular-stripe phases, which are the superposition of states with different angular quantum numbers, appear in the phase diagram. However, these phases normally exist at small detuning, which makes them hard to be probed in experiments. We show that for a large OAM difference of the laser beams, an asymmetric kind of angular-stripe phase can exist even at large detuning. The excitation spectra in different phases exhibit distinct features: In the angular-stripe phase there exist two gapless bands corresponding to the broken $\mathrm{U}(1)$ and rotational symmetries, while in the half-skyrmion phase the gapless band exhibits a rotonlike structure. Our predictions of the angular-stripe phases and the low-energy excitations can be examined in recently realized Bose-Einstein condensates with SOAM coupling.

DOI
10.1103/physreva.102.013316

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We investigate the ground-state phase diagram and excitation spectrum of an interacting spinor Bose-Einstein condensate with spin-orbital-angular-momentum (SOAM) coupling realized in recent experiments by introducing atomic Raman transition with a pair of copropagating Laguerre-Gaussian laser beams that carry different orbital angular momenta (OAM) [Chen et al., Phys. Rev. Lett. 121, 113204 (2018) and Zhang et al., Phys. Rev. Lett. 122, 110402 (2019)]. Because of the ground-state degeneracy of the single-particle Hamiltonian at vanishing detuning, several angular-stripe phases, which are the superposition of states with different angular quantum numbers, appear in the phase diagram. However, these phases normally exist at small detuning, which makes them hard to be probed in experiments. We show that for a large OAM difference of the laser beams, an asymmetric kind of angular-stripe phase can exist even at large detuning. The excitation spectra in different phases exhibit distinct features: In the angular-stripe phase there exist two gapless bands corresponding to the broken U(1)\mathrm{U}(1)U(1) and rotational symmetries, while in the half-skyrmion phase the gapless band exhibits a rotonlike structure. Our predictions of the angular-stripe phases and the low-energy excitations can be examined in recently realized Bose-Einstein condensates with SOAM coupling.
Motivated by recent experiments [Chen et al., Phys. Rev. Lett. 121, 113204 (2018); Chen et al., Phys. Rev. Lett. 121, 250401 (2018)], we investigate the low-lying excitation spectrum of the ground-state phases of spin-orbital-angular-momentum-coupled (SOAM-coupled) spin-1 condensates. At vanishing detuning, a ferromagnetic SOAM-coupled spin-1 Bose-Einstein condensate (BEC) can have two ground-state phases, namely, coreless and polar-core vortex states, whereas an antiferromagnetic BEC supports only polar-core vortex solution. The angular momentum per particle, longitudinal magnetization, and excitation frequencies display discontinuities across the phase boundary between the coreless vortex and polar-core vortex phases. The low-lying excitation spectrum evaluated by solving the Bogoliubov--de Gennes equations is marked by avoided crossings and hence the hybridization of the spin and density channels. The spectrum is further confirmed by the dynamical evolution of the ground state subjected to a perturbation suitable to excite a density or a spin mode and a variational analysis for the density-breathing mode.
By inducing a Raman transition using a pair of Gaussian and Laguerre-Gaussian laser beams, we realize a ^{87}Rb condensate whose orbital angular momentum (OAM) and its internal spin states are coupled. By varying the detuning and the coupling strength of the Raman transition, we experimentally map out the ground-state phase diagram of the system for the first time. The transitions between different phases feature a discontinuous jump of the OAM and the spin polarization, and hence are of first order. We demonstrate the hysteresis loop associated with such first-order phase transitions. The role of interatomic interaction is also elucidated. Our work paves the way to explore exotic quantum phases in the spin-orbital-angular-momentum coupled quantum gases.
We present a theoretical study of the collective excitations of the supersolid annular stripe phase of a spin-orbital-angular-momentum-coupled (SOAM-coupled) spin-1 Bose-Einstein condensate. The annular stripe phase simultaneously breaks two continuous symmetries, namely rotational and U(1)U(1)U(1) gauge symmetry, and is more probable in the condensates with a larger orbital angular momentum transfer imparted by a pair of Laguerre-Gaussian beams than what has been considered in the recent experiments. Accordingly, we consider a SOAM-coupled spin-1 condensate with a $4\ensuremath{\hbar}$ orbital angular momentum transferred by the lasers. Depending on the values of the Raman coupling strength and quadratic Zeeman term, the condensate with realistic antiferromagnetic interactions supports three ground-state phases: the annular stripe, the vortex necklace, and the zero angular momentum phase. We numerically calculate the collective excitations of the condensate as a function of coupling and quadratic Zeeman field strengths for a fixed ratio of spin-dependent and spin-independent interaction strengths. At low Raman coupling strengths, we observe a direct transition from the zero angular momentum to the annular stripe phase, characterized by the softening of a double symmetric roton mode, which serves as a precursor to supersolidity.
The experimental realization of emergent spin-orbit coupling through laser-induced Raman transitions in ultracold atoms paves the way for exploring novel superfluid physics and simulating exotic many-body phenomena. A recent proposal with the use of Laguerre-Gaussian lasers enables another fundamental type of coupling between spin and orbital angular momentum (SOAM) in ultracold atoms. We hereby study quantum phases of a realistic Bose-Einstein condensate (BEC) with this synthetic SOAM coupling in a disk-shaped geometry, respecting radial inhomogeneity of the Raman coupling. We find that the experimental system naturally resides in a strongly interacting regime in which the phase diagram significantly deviates from the single-particle picture. The interplay between SOAM coupling and interaction leads to rich structures in spin-resolved position and momentum distributions, including a stripe phase and various types of immiscible states. Our results would provide a guide for an experimental investigation of SOAM-coupled BECs.
Theoretical study is presented for a spinor Bose-Einstein condensate, whose two components are coupled by copropagating Raman beams with different orbital angular momenta. The investigation is focused on the behavior of the ground state of this condensate, depending on the atom-light coupling strength. By analyzing the ground state, we have identified a number of quantum phases, which reflect the symmetries of the effective Hamiltonian and are characterized by the specific structure of the wave function. In addition to the well-known stripe, polarized, and zero-momentum phases, our results show that the system can support phases whose wave functions contain a complex vortex molecule. Such a molecule plays an important role in the continuous phase transitions of the system. The predicted behavior of vortex-molecule phases can be examined in cold-atom experiments using currently existing techniques.
We propose a simple model with spin and orbit angular momentum coupling in a spin-1 Bose-Einstein condensate, where three internal atomic states are Raman coupled by a pair of copropagating Laguerre-Gaussian beams. The resulting Raman transition imposes a transfer of orbital angular momentum between photons and the condensate in a spin-dependent way. Focusing on a regime where the single-particle ground state is nearly threefold degenerate, we show that the weak interatomic interaction in the condensate produces a rich phase diagram, and that a many-body Rabi oscillation between two quantum phases can be induced by a sudden quench of the quadratic Zeeman shift. We carried out our calculations using both a variational method and a full numerical method, and found excellent agreement.