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arXiv:1910.10506 · Light Science & Applications

Nonlinear interference in crystal superlattices

Anna V. Paterova, Leonid A. Krivitsky

Published May 9, 2020• 38 citations
arXivHTMLPDF

Abstract

Nonlinear interferometers with correlated photons hold promise to advance optical characterization and metrology techniques by improving their performance and affordability. These interferometers offer subshot noise phase sensitivity and enable measurements in detection-challenging regions using inexpensive and efficient components. The sensitivity of nonlinear interferometers, defined by the ability to measure small shifts of interference fringes, can be significantly enhanced by using multiple nonlinear elements, or crystal superlattices. However, to date, experiments with more than two nonlinear elements have not been realized, thus hindering the potential of nonlinear interferometers. Here, we build a nonlinear interferometer with up to five nonlinear elements, referred to as superlattices, in a highly stable and versatile configuration. We study the modification of the interference pattern for different configurations of the superlattices and perform a proof-of-concept gas sensing experiment with enhanced sensitivity. Our approach offers a viable path towards broader adoption of nonlinear interferometers with correlated photons for imaging, interferometry, and spectroscopy.

DOI
10.1038/s41377-020-0320-1

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Nonlinear interferometers with correlated photons hold promise to advance optical characterization and metrology techniques by improving their performance and affordability. These interferometers offer subshot noise phase sensitivity and enable measurements in detection-challenging regions using inexpensive and efficient components. The sensitivity of nonlinear interferometers, defined by the ability to measure small shifts of interference fringes, can be significantly enhanced by using multiple nonlinear elements, or crystal superlattices. However, to date, experiments with more than two nonlinear elements have not been realized, thus hindering the potential of nonlinear interferometers. Here, we build a nonlinear interferometer with up to five nonlinear elements, referred to as superlattices, in a highly stable and versatile configuration. We study the modification of the interference pattern for different configurations of the superlattices and perform a proof-of-concept gas sensing experiment with enhanced sensitivity. Our approach offers a viable path towards broader adoption of nonlinear interferometers with correlated photons for imaging, interferometry, and spectroscopy.
Nonlinear interferometers with quantum correlated photons have been demonstrated to improve optical characterization and metrology. These interferometers can be used in gas spectroscopy, which is of particular interest for monitoring greenhouse gas emissions, breath analysis and industrial applications. Here, we show that gas spectroscopy can be further enhanced via the deployment of crystal superlattices. This is a cascaded arrangement of nonlinear crystals forming interferometers, allowing the sensitivity to scale with the number of nonlinear elements. In particular, the enhanced sensitivity is observed via the maximum intensity of interference fringes that scales with low concentration of infrared absorbers, while for high concentration the sensitivity is better in interferometric visibility measurements. Thus, a superlattice acts as a versatile gas sensor since it can operate by measuring different observables, which are relevant to practical applications. We believe that our approach offers a compelling path towards further enhancements for quantum metrology and imaging using nonlinear interferometers with correlated photons.
We describe an all-fiber nonlinear interferometer based on four-wave mixing in highly nonlinear fiber. Our configuration realizes phase-sensitive interference with 97% peak visibility and >90% visibility over a broad 554 GHz optical band. By comparing the output noise power to the shot-noise level, we confirm noise cancellation at dark interference fringes, as required for quantum-enhanced sensitivity. Our device extends nonlinear interferometry to the important platform of highly nonlinear optical fiber and could find applications in a variety of fiber-based sensors.
A nonlinear interferometer uses nonlinear elements as beam splitters to split and to recombine optical waves for interference. As a result, the interference fringe size has a nonlinear dependence on the intensity of the field for phase sensing and leads to an enhanced phase signal. In this paper, a practical scheme of nonlinear interferometry for precision phase measurement is analyzed with parametric amplifiers as the nonlinear beam splitters. It is found that the signal due to phase shift is enhanced by a factor of the amplification gain as compared to a linear interferometer with the same phase-sensing light intensity while the quantum noise is kept at the vacuum level, thus, effectively increasing the signal-to-noise ratio (SNR) beyond the standard quantum limit. Furthermore, the scheme is not as sensitive to the detection loss as the linear scheme with a squeezed state for noise reduction. However, losses inside the interferometer limit the enhancement factor in SNR. We apply the concept to a Michelson interferometer but with parametric amplifiers involved for gravitational-wave detection. We find that effective power is increased by the gain of the amplifiers without actually increasing the cycling power inside the interferometer. Furthermore, the full benefits with squeezed input and variational output or the combination of a quantum nondemolition interferometer for sensitivity beyond the standard quantum limit apply here with even better results. Such a nonlinear interferometer will find wide applications in precision measurements.
Quantum metrology promises greater sensitivity for optical phase measurements than could ever be achieved classically. Here, we present a theory of the phase sensitivity for the general case where the detection probability is given by an N photon interference fringe. We find that the phase sensitivity has a complicated dependence on both the intrinsic efficiency of detection η and the interference fringe visibility V . Most importantly, the phase that gives maximum phase sensitivity is in general not the same as the phase at which the slope of the interference fringe is a maximum, as has previously been assumed. We determine the parameter range where quantum enhanced sensitivity can be achieved. In order to illustrate these theoretical results, we perform a four-photon experiment with η=3/4 and V =82±6% (an extension of our previous work (Nagata et al 2007 Science 316 726)) and find a phase sensitivity 1.3 times greater than the standard quantum limit at a phase different to that which gives maximum slope of the interference fringe.
Interferometers are widely used as sensors in precision measurement. Compared with a conventional Mach–Zehnder interferometer, the sensitivity of a correlation-enhanced nonlinear interferometer can break the standard quantum limit. Phase sensitivity plays a significant role in the enhanced performance. In this paper, we review improvement in phase estimation technologies in correlation-enhanced nonlinear interferometers, including SU(1,1) interferometer and SU(1,1)-SU(2) hybrid interferometer, and so on, and the applications in quantum metrology and quantum sensing networks.