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arXiv:1910.06131 · Physical Review A

Generation of atomic spin orientation with a linearly polarized beam in room-temperature alkali-metal vapor

Patrick Bevington, R. Gartman, Witold Chałupczak

Published Jan 30, 2020• 9 citations
arXivHTMLPDF

Abstract

Traditionally, atomic spin orientation is achieved by the transfer of angular momentum from polarized light to an atomic system. We demonstrate the mechanism of orientation generation in room-temperature caesium vapors that combines three elements: optical pumping, nonlinear spin dynamics, and spin-exchange collisions. Through the variation of the spin-exchange relaxation rate, the transition between an aligned and an oriented atomic sample is presented. The observation is performed by monitoring the atomic radio-frequency spectra. The measurement configuration discussed paves the way to simple and robust radio-frequency atomic magnetometers that are based on a single low-power laser diode that approach the performance of multilaser pump-probe systems.

DOI
10.1103/physreva.101.013436

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Traditionally, atomic spin orientation is achieved by the transfer of angular momentum from polarized light to an atomic system. We demonstrate the mechanism of orientation generation in room-temperature caesium vapors that combines three elements: optical pumping, nonlinear spin dynamics, and spin-exchange collisions. Through the variation of the spin-exchange relaxation rate, the transition between an aligned and an oriented atomic sample is presented. The observation is performed by monitoring the atomic radio-frequency spectra. The measurement configuration discussed paves the way to simple and robust radio-frequency atomic magnetometers that are based on a single low-power laser diode that approach the performance of multilaser pump-probe systems.
An effect is demonstrated where off-resonant optical pumping is enhanced by spin-exchange collisions, which enables a high degree of spin orientation to be obtained in alkali-metal atoms. The experiment with room-temperature cesium vapor employs radio-frequency spectroscopy under conditions of the nonlinear Zeeman effect that allow the populations of the individual Zeeman sublevels to be determined. The improved efficiency of atomic orientation leads to a significant reduction of population relaxation out of the state with maximum magnetic quantum number mmm (stretched state), which is observed as a narrowing of radio-frequency resonances. Spin-exchange collisions play a crucial role in this effect although the applied atomic density $\ensuremath{\sim}101010{}^{11}$ cm${}^{\ensuremath{-}3}$ corresponds to collision rates not greater than several tens of Hz. A simplified theoretical model has been developed to reproduce the measurement results numerically.
We explore the role of the linearly polarized probe beam in the radio-frequency atomic magnetometer. Two regimes of coupling of the linearly polarized light to the atomic ensemble, near and off-resonant, are demonstrated and discussed. Our studies cover three types of interaction between the atomic spin system and the linearly polarized beam, i.e., absorptive production of spin polarization, dispersive spin state readout, and nonlinear spin couplings. The work is performed with the outlook of optimization and simplification of magnetometer operation. Operation of a magnetometer with a single beam, generating and probing the atomic orientation, is presented. This single-beam configuration, which combines optical pumping, nonlinear spin couplings, and spin-exchange collisions, creates the option for a portable device with simple instrumentation.
A recently demonstrated technique of continuous indirect pumping enables a high level of atomic spin polarization to be generated in thermal alkali-metal vapors, without compromising the coherence lifetime through power broadening from the pump laser. The indirect pumping process combines optical excitation and spin-exchange collisions. Here we describe the pumping process and the role of spin-exchange collisions for the case of amplitude-modulated optical excitation. We demonstrate that effective spin-exchange decoherence is modified by the measurement geometry and dynamics. Decoherence changes are studied through magneto-optical-rotation signals. The studies presented here are particularly important for optimizing the performance of an atomic magnetometer operating in the quantum nondemolition configuration in a nonzero-magnetic-field environment.
We have developed a simple heuristic method for determining the polarization of an optically pumped alkali-metal vapor. A linearly polarized probe beam traverses a vapor cell perpendicular to the pump-beam propagation direction, and the transmitted beam intensity is monitored for orthogonal linear polarizations. As the probe beam is scanned in frequency across the D1{D}_{1}D1​ transition, its linear-polarization-dependent transmission can be used as a measure of the atomic orientation of the vapor. We analyze these transmission differences and their dependence on the alkali-metal number density in the vapor.
A variation of the usual method of atomic orientation of alkali metal vapors by optical pumping is proposed. This variation consists of employing a single circularly polarized D1{D}_{1}D1​ line as pumping radiation, instead of a mixture of the two DDD lines. Under these conditions, one magnetic substate of the ground state is transparent to the pumping radiation. It is shown that for a sufficiently intense light source and relatively weak relaxation, the entire population of the vapor will tend to be pumped into this single state, resulting in nearly one-hundred percent atomic orientation. The pumping process is analyzed in detail for sodium vapor illuminated with $3{P}_{\frac{1}{2}}\ensuremath{-}3{S}_{\frac{1}{2}}$ radiation, and the time dependence of the populations of the eight magnetic sublevels of the ground state is computed. It is shown that in the steady state, the light absorption by the vapor is linear rather than exponential with distance. A simple method of measuring relaxation times based on this observation is suggested. The conditions under which the imprisonment of resonance radiation limits the size of the oriented sample are discussed, and it is suggested that the proposed technique will allow the alignment of larger samples than is possible by the usual method of optical pumping.
Spin-exchange relaxation free alkali-metal magnetometers typically operate in the regime of high optical density, presenting challenges for simple and efficient optical pumping and detection. We describe a high-sensitivity Rb magnetometer using a single elliptically polarized off-resonant laser beam. Circular component of the light creates relatively uniform spin polarization while the linear component is used to measure optical rotation generated by the atoms. Modulation of the atomic spin direction with an oscillating magnetic field shifts the detected signal to high frequencies. Using a fiber-coupled distributed feedback laser, we achieve magnetic field sensitivity of 7 fT/Hz7\text{ }\text{fT}/\sqrt{\text{Hz}}7 fT/Hz​ with a miniature $5\ifmmode\times\else\texttimes\fi{}5\ifmmode\times\else\texttimes\fi{}5\text{ }\text{mm}\text{ }\text{Rb}$ vapor cell.