Interactions in an ultracold boson-fermion mixture are often manifested by elastic collisions. In a mixture of a condensed Bose gas (BEC) and spin polarized degenerate Fermi gas (DFG), fermions can mediate spin-spin interactions between bosons, leading to an effective long-range magnetic interaction analogous to Ruderman-Kittel-Kasuya-Yosida [Phys. Rev. 96, 99 (1954); Prog. Theor. Phys. 16, 45 (1956); Phys. Rev. 106, 893 (1957)] interaction in solids. We used Ramsey spectroscopy of the hyperfine clock transition in a ^{87}Rb BEC to measure the interaction mediated by a ^{40}K DFG. By controlling the boson density we isolated the effect of mediated interactions from mean-field frequency shifts due to direct collision with fermions. We measured an increase of boson spin-spin interaction by a factor of η=1.45±0.05^{stat}±0.13^{syst} in the presence of the DFG, providing clear evidence of spin-spin fermion mediated interaction. Decoherence in our system was dominated by inhomogeneous boson density shift, which increased significantly in the presence of the DFG, again indicating mediated interactions. We also measured a frequency shift due to boson-fermion interactions in accordance with a scattering length difference of a_{bf_{2}}-a_{bf_{1}}=-5.36±0.44^{stat}±1.43^{syst}a_{0} between the clock-transition states, a first measurement beyond the low-energy elastic approximation [R. Côté, A. Dalgarno, H. Wang, and W. C. Stwalley, Phys. Rev. A 57, R4118 (1998); A. Dalgarno and M. Rudge, Proc. R. Soc. A 286, 519 (1965)] in this mixture. This interaction can be tuned with a future use of a boson-fermion Feshbach resonance. Fermion-mediated interactions can potentially give rise to interesting new magnetic phases and extend the Bose-Hubbard model when the atoms are placed in an optical lattice.
Interactions in an ultracold boson-fermion mixture are often manifested by elastic collisions. In a mixture of a condensed Bose gas (BEC) and spin polarized degenerate Fermi gas (DFG), fermions can mediate spin-spin interactions between bosons, leading to an effective long-range magnetic interaction analogous to Ruderman-Kittel-Kasuya-Yosida [Phys. Rev. 96, 99 (1954); Prog. Theor. Phys. 16, 45 (1956); Phys. Rev. 106, 893 (1957)] interaction in solids. We used Ramsey spectroscopy of the hyperfine clock transition in a ^{87}Rb BEC to measure the interaction mediated by a ^{40}K DFG. By controlling the boson density we isolated the effect of mediated interactions from mean-field frequency shifts due to direct collision with fermions. We measured an increase of boson spin-spin interaction by a factor of η=1.45±0.05^{stat}±0.13^{syst} in the presence of the DFG, providing clear evidence of spin-spin fermion mediated interaction. Decoherence in our system was dominated by inhomogeneous boson density shift, which increased significantly in the presence of the DFG, again indicating mediated interactions. We also measured a frequency shift due to boson-fermion interactions in accordance with a scattering length difference of a_{bf_{2}}-a_{bf_{1}}=-5.36±0.44^{stat}±1.43^{syst}a_{0} between the clock-transition states, a first measurement beyond the low-energy elastic approximation [R. Côté, A. Dalgarno, H. Wang, and W. C. Stwalley, Phys. Rev. A 57, R4118 (1998); A. Dalgarno and M. Rudge, Proc. R. Soc. A 286, 519 (1965)] in this mixture. This interaction can be tuned with a future use of a boson-fermion Feshbach resonance. Fermion-mediated interactions can potentially give rise to interesting new magnetic phases and extend the Bose-Hubbard model when the atoms are placed in an optical lattice.
We describe recent theoretical and experimental developments on mediated interactions in mixtures of bosonic and fermionic atoms. We discuss how particle-hole excitations of a Fermi sea can induce long-range interactions between heavy impurities or atoms in a Bose-Einstein condensate. Conversely, phonon excitations of a Bose-Einstein condensate induce interactions between fermionic atoms. These mediated interactions exhibit different short-range and long-range scaling regimes with distance and, if strong enough, can induce fermion superfluidity. We discuss the prospects for observing new phenomena that could arise from mediated interactions. Experimentally, we outline recent studies of the 133Cs-6Li Bose-Fermi mixture, a platform well-suited for investigating fermion-mediated interactions. A Cs Bose-Einstein condensate immersed in a degenerate Li Fermi gas is prepared with tunable interspecies interactions. In the weak-coupling regime, precision measurements of condensate properties reveal fermion-mediated attractions between bosons, matching theoretical predictions. In the strong-coupling regime, we observe suppression and revival of sound modes and novel many-body resonances. Altogether, we aim to highlight both instances where experiment and theory agree well, and promising prospects to engineer long-range interactions in atomic quantum gases.
The work described in this thesis can be divided into two parts. The first part is concerned with the production of degenerate Fermi gases and Bose-Fermi mixtures. The second part of the thesis describes studies of strongly interacting spin-mixtures of ultracold fermions. We have cooled a magnetically trapped spin-polarized 6Li Fermi gas into quantum degeneracy by sympathetic cooling with bosonic 23Na. In order to do this, we have converted our previously developed apparatus for Bose-Einstein condensation of 23Na into a two-species cooling facility. We have produced 6Li samples with up to 7 × 107 atoms at temperatures below 0.5TF , and up to 3× 107 atoms at temperatures as low as 0.05TF . Further, we have also produced stable quantum degenerate mixtures of 23Na and 6Li, with several million atoms of each species. In a second set of experiments, we have studied strongly interacting spin-mixtures of 6Li. The strength of interactions was resonantly controlled by applying a magnetic field and tuning to “Feshbach resonances”, which occur when the total energy of the colliding particles coincides with the energy of a bound molecular state. These studies are relevant for the continuing quest for a superfluid transition in a Fermi gas. By studying the inelastic decay of the cloud, we have experimentally identified two Feshbach resonances for the inter-state interactions of the two lowest ground states of 6Li. Most importantly, we found that the lifetime of the strongly interacting system is long enough to observe a superfluid transition in the future. The effects of the coherent collisions in 6Li spin-mixtures were studied using radiofrequency (RF) spectroscopy. We demonstrated the absence of mean field “clock shifts” in a two-state mixture of fermions, and have introduced a three-level method to observe the interaction energy shifts. In the strongly interacting regime, near a Feshbach resonance, we have observed universal behavior of the interaction energy, independent of the value of the scattering length. Finally, we have theoretically studied the effects of Pauli blocking during a free expansion of a degenerate Fermi gas. We have concluded that a strongly interacting normal gas will undergo a hydrodynamic expansion even at zero temperature, due to inefficiency of the Pauli suppression of collisions. Therefore, the already observed hydrodynamic expansion cannot be conclusively interpreted as a signature of superfluidity. Thesis Supervisor: Wolfgang Ketterle Title: John D. MacArthur Professor of Physics
In the strong-coupling Bose-Einstein condensation (BEC) region where a Feshbach resonance gives rise to tightly bound dimer molecules, we show that a spin-polarized Fermi superfluid reduces to a simple Bose-Fermi mixture of Bose-condensed dimers and the leftover unpaired fermions. Using a many-body functional integral formalism, the Gaussian fluctuations give rise to an induced dimer-dimer interaction mediated by the unpaired fermions, with the dimer-fermion vertex being given by the (mean-field) Born approximation. Treating the pairing fluctuations to quartic order, we show how the action for a spin-polarized Fermi superfluid reduces to one for a Bose-Fermi mixture. This Bose-Fermi action includes an expression for the effective dimer-unpaired fermion interaction in a spin-polarized Fermi superfluid beyond the Born approximation, in the BEC limit. In the low-density limit, we show how this dimer-fermion interaction gives the s-wave scattering length aBF=1.18aF (aF is the s-wave fermion scattering length), a result first derived by Skorniakov and Ter-Martirosian in 1957 for three interacting fermions.
This work is inspired by recent experimental observations in ultracold atomic Bose-Fermi mixtures [DeSalvo et al., Nature 568 (2019)]. These experiments reveal the emergence of an attractive fermion-mediated interaction between bosons, as well as a stability-instability transition. We give the first mathematical demonstration of this transition by studying the low-energy spectrum of a many-body interspecies Hamiltonian. More precisely, we show the convergence of its eigenvalues towards those of an effective Bose Hamiltonian, which includes fermion-mediated effects. Applying this result to a model with short-range potentials, we derive a stability-instability transition in the bosonic subsystem, driven by the Bose-Fermi coupling strength g. For small ∣g∣, the bosons form a stable Bose-Einstein condensate with the energy per particle uniformly bounded from below. For large ∣g∣, the energy per particle is no longer uniformly bounded from below, signaling the collapse of the condensate.
Interactions between particles play an important role in quantum degenerate gases.\nIn fact, the system’s behavior is usually largely determined by the strength, range, and\nsymmetry of the interactions, even if very weak. For more than two decades after the\nfirst experimental realization of a Bose-Einstein condensate (BEC) in 1995, investigations of ultracold atomic gases have mainly considered contact-type interactions, which\nmodel the short-range van der Waals interactions between the atoms in terms of a single\nparameter, the s-wave scattering length. However, some atomic or molecules species\npossess a magnetic or electric dipole moment and additionally interact among each\nother via the dipole-dipole interaction (DDI), which is long-ranged and anisotropic.\nSignatures of the DDI have been first observed in a BEC of chromium atoms in 2005.\nIn the last several years, a new class of atoms from the lanthanide series, e.g., dysprosium and erbium, with stronger dipolar properties, have come into play. This permits\na more full-fledged study of dipolar effects in BECs. Furthermore, ultracold molecules\nand highly excited Rydberg atoms are other promising examples for futures studies of\nsystems where dipolar interaction will be even more dominant, but they still need experimental efforts to achieve the desired quantum regime. Whereas the weak DDI in a\nchromium BEC is well described with the Gross-Pitaevskii equation, stronger dipolar\ninteractions certainly necessitate a beyond-mean-field description within a Bogoliubov\ntheory.\nIn parallel to research on bosons, cold fermions also trigger great interest because\nthey are actually often found in nature, e.g., within the electron gas of metals, as\nneutrons of heavy stars, or as quarks in plasmas as constituent elements of composite particles. Contrary to Bose systems, quantum degeneracy in experiments is much\nmore difficult to achieve in Fermi systems, since s-wave scattering is absent between\nidentical fermions, due to the Pauli exclusion principle. It was first achieved in 1999\nfor alkali atoms using a technique based on the sympathetic cooling with a second spin\nstate, another species, or a different isotope. For highly magnetic atoms, quantum degeneracy was achieved for dysprosium in 2012 using the standard sympathetic cooling\ntechnique, while in 2014 erbium was cooled deep into the degenerate regime using a\ndirect evaporative cooling mediated by dipolar collisions. This direct cooling scheme\nivallows producing very dense Fermi gas down to 10% of the Fermi temperature.\nFurthermore, a novel kind of strongly dipolar quantum gases became available in\nthe last several years. These are weakly bound polar molecules produced from atoms\nwith large magnetic dipole moments, such as erbium. Only very recently a quantum\ndegenerate dipolar Fermi gas of potassium-rubidium molecules has been experimentally realized. Unlike previously considered magnetic systems, heteronuclear molecules\nsuch as potassium-rubidium possess large electric dipole moments. The next natural\nstep is to polarize this system in a preferential direction by an external electric field,\nsuch that the DDI dominates the behavior of the system, which would open up the\nrealm for experimental investigation of strong dipolar Fermi gases...
Engineering long-range interactions in cold-atom quantum simulators can lead to exotic quantum many-body behavior. Fermionic atoms in ultracold atomic mixtures can act as mediators, giving rise to long-range Ruderman-Kittel-Kasuya-Yosida-type interactions characterized by the dimensionality and density of the fermionic gas. Here, we propose several tuning knobs, accessible in current experimental platforms, that allow one to further control the range and shape of the mediated interactions, extending the existing quantum simulation toolbox. In particular, we include an additional optical lattice for the fermionic mediator, as well as anisotropic traps to change its dimensionality in a continuous manner. This allows us to interpolate between power-law and exponential decays, introducing an effective cutoff for the interaction range, as well as to tune the relative interaction strengths at different distances. Finally, we show how our approach allows one to investigate frustrated regimes that were not previously accessible, where symmetry-protected topological phases as well as chiral spin liquids emerge.