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arXiv:1910.01298 · Physical Review A

Dynamics of transient cat states in degenerate parametric oscillation with and without nonlinear Kerr interactions

Run Yan Teh, Feng-Xiao Sun, Rodney Polkinghorne, Qiongyi He, Qihuang Gong, P. D. Drummond, M. D. Reid

Published Apr 7, 2020• 32 citations
arXivHTMLPDF

Abstract

A cat state is formed as the steady-state solution for the signal mode of an ideal degenerate parametric oscillator, in the limit of negligible single-photon signal loss. In the presence of signal loss, this is no longer true over timescales much longer than the damping time. However, for sufficient parametric nonlinearity, a cat state can still exist as a transient state. In this paper we study the dynamics of the creation and decoherence of cat states in degenerate parametric oscillation, both with and without the Kerr nonlinearity found in recent superconducting-circuit experiments that generate cat states in microwave cavities. We determine the time of formation and the lifetime of a cat state of fixed amplitude in terms of three dimensionless parameters $\ensuremath{\lambda}$, $g$, and $\ensuremath{\chi}$. These relate to the driving strength, the parametric nonlinearity relative to signal damping, and the Kerr nonlinearity, respectively. We find that the Kerr nonlinearity has little effect on the threshold parametric nonlinearity ($g>1$) required for the formation of cat states and does not significantly alter the decoherence time of the cat state, but can reduce the time of formation. The quality of the cat state increases with the value of $g$. To verify the existence of the cat state, we consider several signatures, including interference fringes and negativity. We emphasize the importance of taking into account more than one of these signatures. We simulate a superconducting-circuit experiment using published experimental parameters and find good agreement with experimental results, indicating that a nonclassical catlike state with a small Wigner negativity is generated in the experiment. Interference fringes, however, are absent, requiring higher $g$ values. Finally, we explore the feasibility of creating large cat states with a coherent amplitude of 20, corresponding to 400 photons, and study finite-temperature reservoir effects.

DOI
10.1103/physreva.101.043807

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A cat state is formed as the steady-state solution for the signal mode of an ideal degenerate parametric oscillator, in the limit of negligible single-photon signal loss. In the presence of signal loss, this is no longer true over timescales much longer than the damping time. However, for sufficient parametric nonlinearity, a cat state can still exist as a transient state. In this paper we study the dynamics of the creation and decoherence of cat states in degenerate parametric oscillation, both with and without the Kerr nonlinearity found in recent superconducting-circuit experiments that generate cat states in microwave cavities. We determine the time of formation and the lifetime of a cat state of fixed amplitude in terms of three dimensionless parameters \ensuremathλ\ensuremath{\lambda}\ensuremathλ, ggg, and \ensuremathχ\ensuremath{\chi}\ensuremathχ. These relate to the driving strength, the parametric nonlinearity relative to signal damping, and the Kerr nonlinearity, respectively. We find that the Kerr nonlinearity has little effect on the threshold parametric nonlinearity (g>1g>1g>1) required for the formation of cat states and does not significantly alter the decoherence time of the cat state, but can reduce the time of formation. The quality of the cat state increases with the value of ggg. To verify the existence of the cat state, we consider several signatures, including interference fringes and negativity. We emphasize the importance of taking into account more than one of these signatures. We simulate a superconducting-circuit experiment using published experimental parameters and find good agreement with experimental results, indicating that a nonclassical catlike state with a small Wigner negativity is generated in the experiment. Interference fringes, however, are absent, requiring higher ggg values. Finally, we explore the feasibility of creating large cat states with a coherent amplitude of 20, corresponding to 400 photons, and study finite-temperature reservoir effects.
A cat-state is a superposition of two coherent states with amplitudes α0α_{0}α0​ and −α0-α_{0}−α0​. Recent experiments create cat states in a microwave cavity field using superconducting circuits. As with degenerate parametric oscillation (DPO) in an adiabatic and highly nonlinear limit, the states are formed in a signal cavity mode via a two-photon dissipative process induced by the down conversion of a pump field to generate pairs of signal photons. The damping of the signal and the presence of thermal fluctuations rapidly decoheres the state, and the effect on the dynamics is to either destroy the possibility of a cat state, or else to sharply reduce the lifetime and size of the cat-states that can be formed. In this paper, we study the effect on both the DPO and microwave systems of a squeezed reservoir coupled to the cavity. While the threshold nonlinearity is not altered, we show that the use of squeezed states significantly lengthens the lifetime of the cat states. This improves the feasibility of generating cat states of large amplitude and with a greater degree of quantum macroscopic coherence, which is necessary for many quantum technology applications. Using current experimental parameters for the microwave set-up, which requires a modified Hamiltonian, we further demonstrate how squeezed states enhance the quality of the cat states that could be formed in this regime. Squeezing also combats the significant decoherence due to thermal noise, which is relevant for microwave fields at finite temperature. By modeling a thermal squeezed reservoir, we show that the thermal decoherence of the dynamical cat states can be inhibited by a careful control of the squeezing of the reservoir. To signify the quality of the cat state, we consider different signatures including fringes and negativity, and the Cl1C_{l_{1}}Cl1​​ measure of quantum coherence.
We discuss general properties of the equilibrium state of parametric down-conversion in superconducting quantum circuits with detunings and Kerr anharmonicities, in the strongly nonlinear regime. By comparing moments of the steady state and those of a Schr\"odinger cat, we show that true Schr\"odinger cats cannot survive in the steady state if there is any single-photon loss. A delta-function ``catlike'' steady-state distribution can be formed, but this only exists in the limit of an extremely large nonlinearity. The steady state is a mixed state, which is more complex than a mixture or linear combination of delta functions, and the purity of which is reduced by driving. We expect this general behavior to occur in other driven, dissipative quantum subharmonic nonequilibrium open systems.
Abstract The quantum to classical transition is determined by the interplay of a trio of parameters: dissipation, nonlinearity, and macroscopicity. Why is nonlinearity needed to see quantum effects? And, is not an ordinary pendulum quite nonlinear already? In this manuscript, we discuss the parameter regime where the dynamics of a massive oscillator should be quantum mechanical in the presence of dissipation. We review the outstanding challenge of the dynamical generation of highly quantum mechanical cat states of a massive ‘pendulum’, known as Kerr-cats. We argue that state-of-the-art cold atom experiments may be in a position to reach such a nonlinear regime, which today singles out superconducting quantum circuits. A way to stabilize Schrödinger cat superpositions of a mechanical atomic oscillator via parametric squeezing and further protected by an unusual form of quantum interference is discussed. The encoding of a neutral atom Kerr-cat qubit is proposed.
Driven-dissipative Kerr cavities serve as a versatile platform for generating nonclassical states, such as quantum cat states and high-photon-number Fock states, which are essential for quantum information processing. Building on the quantized Lugiato-Lefever equation (QLLE), which predicts steady-state coherent state superpositions in multi-mode Kerr resonators, and the framework for engineering Kerr nonlinearity ratios to mitigate spectral crowding in coupled oscillators, we propose an integrated approach for precise quantum control. By engineering the Kerr ratio K1/K2 to approximate an incommensurate value using complex rational approximations, we eliminate parasitic degeneracies and enable selective addressing of transitions in the QLLE steady state. Employing a Magnus expansion, we derive an effective Hamiltonian that incorporates Stark-shift corrections, facilitating deterministic synthesis of entangled cat states and Fock states with fidelities exceeding 99.9%. Numerical simulations using QuTiP validate robustness against dissipation and thermal noise, demonstrating quantum hysteresis and Wigner negativity in multi-mode configurations. This synthesis bridges dissipative phase transitions with architectural control, offering a blueprint for scalable bosonic quantum processors in circuit QED. The Wigner function plays a pivotal role in characterizing these nonclassical states, providing a phase-space representation that reveals quantum interference effects. In our framework, the emergence of negative values in the Wigner function for the central mode confirms the non-Gaussian nature of the cat states, as dictated by Hudson’s theorem, which states that only Gaussian pure states have non-negative Wigner functions everywhere [21]. This negativity arises from the interference term in the cat-state Wigner expression, quantifying macroscopic quantum coherence and serving as a witness for entanglement in multi-mode systems.For instance, our simulations at F = 2.0 yield a minimum Wigner value of approximately -0.006, highlighting the system’s departure from classical behavior and its utility for bosonic error correction, where cat codes leverage phase-space separation to suppress bit-flip errors exponentially with cat size. Furthermore, the relation to Wigner functions extends to dynamical properties: the steady-state Wigner negativity is robust against thermal noise due to the dissipative stabilization mechanism, aligning with results from driven Bose-Hubbard models where two-mode cat states maintain negativity under loss [46]. In the QLLE context, the multi-mode extension introduces spatial localization, where the Wigner function’s negative regions correspond to soliton-like structures, as evidenced by photon population distributions [0.33, 0.90, 0.33]. This negativity is not merely a feature but a consequence of fundamental limits on classical simulability, relating to the Gottesman-Knill theorem’s extension to continuous variables, where non-Gaussian operations are necessary for universal quantum computation. Quantum hysteresis, observed in our hysteresis plots, is intimately linked to the Wigner representation through the bifurcation dynamics. Near the codimension-2 point, the system’s bistability manifests as distinct paths in phase space, with Wigner functions switching between Gaussian-like (low-photon) and cat-like (high-photon) forms, supported by spectral theory of Liouvillians that guarantees metastable states in dissipative phase transitions [30]. The forward and backward sweeps in our simulations demonstrate this path dependence, with the Wigner negativity peaking in the high-drive regime, underscoring the role of Kerr nonlinearity in engineering quantum resources. Overall, the Wigner function’s negativity serves as a diagnostic tool for the efficacy of our engineered ratios, directly tying to experimental verifiability in circuit QED setups, where homodyne measurements can reconstruct Wigner distributions to confirm cat-state fidelity. This work not only advances control protocols but also highlights the profound interplay between phase-space quasi-probabilities and dissipative quantum engineering, paving the way for fault-tolerant bosonic qubits.
The optical parametric oscillator is one of the most well-characterized devices in nonlinear optics, with many useful applications, especially as a frequency converter and as a wide-band amplifier. Novel discoveries made with these devices in the quantum domain include demonstrations of large amounts of both single-mode and two-mode squeezing, and, in the two-mode case, significant quantum intensity correlations between the two modes and quadrature correlations, which provided the first experimental demonstration of the original Einstein–Podolsky–Rosen (EPR) paradox. In this chapter, a systematic theory is developed of quantum fluctuations in the degenerate parametric oscillator. The quantum statistical effects produced by the degenerate parametric amplifier and oscillator have been intensely studied. As we have seen, the amount of transient squeezing produced in an ideal lossless parametric amplifier was calculated using asymptotic methods by Crouch and Braunstein. It was found to scale inversely with the square root of the initial pump photon number. When the system is put into a cavity, and driving and dissipation are introduced, we find that the steady state of a driven degenerate parametric oscillator bifurcates. There is a single steady state at low driving strengths, but, as the driving field increases, a threshold value is reached and the single state splits and forms two stable states. Below the threshold, a linearized analysis of squeezing in the quantum quadratures is possible; while above this threshold, or critical point, the tunneling time between the two states due to quantum fluctuations can be calculated.
Generation of Schrödinger cat-like states via degenerate dual pump spontaneous four-wave mixing in a χ(3)χ^{(3)}χ(3) microring resonator
We theoretically investigate the generation of non-Gaussian quantum states, specifically Schrödinger cat-like states (SCLSs), via degenerate dual-pump spontaneous four-wave mixing in a χ(3)χ^{(3)}χ(3)-based microring resonator. By introducing a unitary transformation that exactly decouples the self-phase modulation (SPM) and cross-phase modulation (XPM) terms, we reduce the full nonlinear Hamiltonian to an effective three-mode interaction. The resulting dynamics (decoupled and full Hamiltonians) are studied using the Lindblad master equation, accounting for cavity losses. Unlike semiclassical or parametric approximations, our full quantum mechanical approach explicitly includes quantum pump depletion, which enables the emergence and observation of non-Gaussian features. We compute the Wigner function, photon number distributions, quadrature variances, Fano factor, Schmidt number, and fidelity to characterize the generated states. For the non-dissipative case, we find that the signal mode b^3\hat{b}_3b^3​ or a^3\hat{a}_3a^3​ exhibits clear non-Gaussian features with a structured Wigner function and even-dominated photon number distribution, characteristic of an even coherent state. In the presence of dissipation (γj=0.2γ_j = 0.2γj​=0.2), the interference fringes become faint, odd photon numbers appear, and the fidelity with the ideal state remains high (>0.9>0.9>0.9), indicating robustness. The pump mode b^1\hat{b}_1b^1​ or a^1\hat{a}_1a^1​ remains Gaussian, while both modes display super-Poissonian statistics and entanglement (>2>2>2). Our results demonstrate that degenerate dual-pump spontaneous four-wave mixing in microring resonators is a promising platform for generating and controlling cat-like states under dissipative conditions.