Realizing quantum materials with Helium: Helium films at ultralow temperatures, from strongly correlated atomically layered films to topological superfluidity
This article provides an overview, primarily from an experimental perspective, of recent progress and future prospects in using helium to realize a range of quantum materials of generic interest, by "top-down" and "bottom-up" nanotechnology. We can grow model systems to realise new quantum states of matter, and explore key issues in condensed matter physics. In the language of cold atomic gases, two dimensional and confined 3He and 4He provide "quantum simulators", with the potential to uncover new emergent quantum states. These include: strictly 2D Fermi system with Mott-Hubbard transition; interacting coupled 2D fermion-boson system; heavy fermion quantum criticality; ideal 2D frustrated ferromagnetism; 2D quantum spin liquid; intertwined superfluid and density wave order with emergent large symmetry; topological mesoscopic superfluidity (new materials and emergent excitations).
This article provides an overview, primarily from an experimental perspective, of recent progress and future prospects in using helium to realize a range of quantum materials of generic interest, by "top-down" and "bottom-up" nanotechnology. We can grow model systems to realise new quantum states of matter, and explore key issues in condensed matter physics. In the language of cold atomic gases, two dimensional and confined 3He and 4He provide "quantum simulators", with the potential to uncover new emergent quantum states. These include: strictly 2D Fermi system with Mott-Hubbard transition; interacting coupled 2D fermion-boson system; heavy fermion quantum criticality; ideal 2D frustrated ferromagnetism; 2D quantum spin liquid; intertwined superfluid and density wave order with emergent large symmetry; topological mesoscopic superfluidity (new materials and emergent excitations).
The Landau Fermi liquid theory and the Ginzburg-Landau phase transition theory stand as two pivotal cornerstones in traditional condensed matter physics, achieving significant success in addressing crucial physical phenomena such as BCS superconductors and liquid helium superfluids. However, marked by the discoveries of the quantum Hall effect and high-temperature superconductivity in the 1980s, it gradually became evident that for a broad class of novel quantum states, such as fractional quantum Hall states and quantum spin liquids, their properties transcend the Landau Fermi liquid theory and Ginzburg-Landau phase transition theory. Topological order and its related concepts of long-range many-body quantum entanglement and fractionalized excitation have become the key concepts to understand these exotic quantum states. Designing and identifying topologically ordered states of matter in quantum materials and quantum simulation systems, and probing and manipulating their fractionalized excitations, are important research directions in modern condensed matter physics. In recent years, great progress has been made in the quantum simulation and manipulation of topological order on highly controllable quantum simulation platforms, such as Rydberg atomic systems, superconducting quantum processors, and two-dimensional moiré superlattices. This article provides a brief overview of recent research advances and challenges in the study of topological order in traditional condensed matter systems and quantum simulation experimental platforms. It also provides prospects for the future developments of this field.
Abstract Atoms deposited on 2D electronic materials, such as graphene, can exhibit unconventional many‐body correlations, not accessible in other settings. All of these are driven by van der Waals forces: between the atoms themselves and atom‐material interactions. For example 4He atoms on 2D materials can potentially form a variety of exotic quantum states of matter, such as 2D supersolids and superfluids, in addition to solid phases. For the “most quantum” case of a single helium layer we discuss, from a theoretical perspective, how the effective low‐energy (Bose–Hubbard) description can take advantage of the extreme sensitivity of this unique system to the interplay between the atomic (helium) and solid‐state (graphene) components. Due to the extraordinary variety and tunability of 2D electronic materials, it is envisaged that a wide range of correlated atomic phases can be realized under favorable conditions. Exciting possibilities in the opposite extreme of many atomic layers forming a liquid on top of graphene are also outlined —in this case a so‐called “spinodal dewetting” pattern can form at the liquid–vapor interface which reflects the presence and electronic properties of graphene underneath. Such patterns could be manipulated by choosing different atoms and materials, with potential technological applications.
Superfluid and superconducting phase transitions of interacting bosons are observed in diverse physical systems such as helium, superconducting materials, ultra-cold atomic gases, etc. For all these systems one-, two-, and three-dimensional (1D, 2D, and 3D) realizations are experimentally accessible. However, the current experimental focus is shifting to the low dimensional systems (e.g., films and wires) due to facilitated measurement techniques and a constant demand of technological applications. From a theoretical standpoint large fluctuations in 1D and 2D systems make them a challenging problem, especially when disorder is present. Here we study peculiarities associated with disorder in low-dimensional cases. Specifically, we are interested in the class of the systems where superfluid or superconducting transitions can be mapped to the finite temperature 2D superfluid-normal Kosterlitz-Thouless (KT) transition: (a) 2D bosonic system with a strong diagonal disorder, (b) 1D system of lattice bosons with off-diagonal disorder in the limit of large integer filling factor at zero temperature, and (c) 3D layered superconductors with no tunnelling between layers in zero external magnetic field.
Ultracold atomic gases provide a fantastic platform to implement quantum simulators and investigate a variety of models initially introduced in condensed matter physics or other areas. One of the most promising applications of quantum simulation is the study of strongly correlated Fermi gases, for which exact theoretical results are not always possible with state-of-the-art approaches. Here, we review recent progress of the quantum simulation of the emblematic Fermi–Hubbard model with ultracold atoms. After introducing the Fermi–Hubbard model in the context of condensed matter, its implementation in ultracold atom systems, and its phase diagram, we review landmark experimental achievements, from the early observation of the onset of quantum degeneracy and superfluidity to the demonstration of the Mott insulator regime and the emergence of long-range anti-ferromagnetic order. We conclude by discussing future challenges, including the possible observation of high- T c superconductivity, transport properties, and the interplay of strong correlations and disorder or topology.
The physics of strongly interacting particles is often extraordinarily rich, leading to the \textit{emergence} of fundamentally new phases and phenomena that cannot exist in the absence of correlations. This thesis is devoted to the study of different classes of quantum systems with such strong correlations. Programmable quantum simulators based on Rydberg atom arrays have recently emerged as versatile platforms to probe quantum many-body phases and their dynamics. In Chapter 2, we start with theories of quantum phase transitions (QPTs) in one-dimensional chains of Rydberg atoms. We demonstrate the existence of a novel QPT in the universality class of the Z3 chiral clock model, calculate its critical exponents, and discuss their measurement with the quantum Kibble-Zurek mechanism. Proceeding to two dimensions, Chapter 3 describes the zero-temperature phase diagram of a square-lattice Rydberg atom array, revealing several experimentally realizable density-wave-ordered phases and QPTs. For a different geometry, namely, the kagome lattice studied in Chapter 4, we identify a regime that constitutes a likely candidate for hosting a phase with long-range quantum entanglement and topological order. Based on mappings to dimer models and gauge theories, we argue for the existence of a quantum spin liquid phase that has proved elusive in solid-state materials. In the next part of this thesis, we focus on similarly strongly correlated phases in the realm of quantum materials. Motivated by recent observations of an enhanced thermal Hall response in the high-temperature cuprate superconductors, in Chapter 5, we study the thermal Hall conductivity, κxy, of chiral spin-liquid ans\"{a}tze on the square lattice, focusing on the contribution from neutral (bosonic or fermionic) spinons. Thereafter, going beyond mean-field theory, we consider the corrections due to emergent gauge fields, which yield a response of opposite sign to that of the fermionic matter. We additionally consider the contribution of phonons to κxy and establish its relation to the spinon Hall viscosity. Thermal Hall measurements also leave intriguing fingerprints in Kitaev materials like α-RuCl3, and in this context, Chapter 6 investigates the unquantized κxy obtained in a gapless spinon Fermi surface state.
From time to time in physics, single technical achievements have spawned an explosion of research activity and have led to the genesis of entirely new avenues of investigation. Precisely this occurred in the field of quantum gases - the topic of this Focus Issue - following the achievement of Bose-Einstein condensation in a dilute alkali gas in 1995. These experiments built on the foundational work on quantum fluids in dense systems, such as superfluid helium, and the technical achievements of laser cooling in atomic physics. Dilute quantum gases have already proved to be an incredibly fertile ground for exploring a wide range of macroscopic quantum phenomena. The rapid pace of experimental discovery and theoretical advance is evident and every year continues to bring significant achievements. A great advantage is that microscopic observations can be made directly and compared with the predictions of many-body theoretical formulations founded on interaction parameters which are completely determined - something which is not possible in their dense fluid counterparts. This Focus Issue brings together papers which cover many of the topical aspects of quantum gases: optical lattices, quantum degenerate fermions, quantum atom optics, molecular Bose-Einstein condensation, vorticity, and quantum fluctuations in systems of reduced dimensionality. One pervasive theme is the flexibility which arises from the ability to control the interactions, even dynamically if necessary. In quantum gases, this can be effected in two ways, either by changing the internal nature of the pairwise potentials by a Feshbach resonance, or by changing the nature of external potentials in which the atoms are confined and supported against gravity. The external potential may be used to spin gases to high vorticity, imprint on the system a periodic optical lattice potential, or even change the effective dimensionality. Optical lattices are particularly well represented in this Focus Issue. This is where there is the strongest connection with the physics of solids and strongly correlated fluids. Interest in optical lattices is partly due to the recent experimental demonstration that in these systems one can study the quantum phase transition from a Mott insulator, where the atoms are localized to individual sites of the optical potential, to a superfluid phase with long-range order. In contrast to a condensed matter system, the transition can be easily dynamically controlled since it is induced by simply varying the depth of the optical potential. Another area of focused interest is in fermionic gases where there is an ongoing effort, both experimentally and theoretically, to observe and characterize the high-temperature superfluid transition that should occur with enhanced pairwise interactions. If realized, this quantum system would allow experimental investigation of the crossover from Bose-Einstein condensation of dilute weakly-interacting composite bosons to the superconducting-like transition that occurs in a system of weakly interacting fermions. The topics of this Focus Issue represent well the building blocks of quantum gas studies which should allow the exploration of a wide range of macroscopic quantum phenomena in a highly controllable and clean system in which the effects of disorder may be completely absent. Given the recent progress, it will be intriguing to see where this field leads in the future. Focus on Quantum Gases Contents Anisotropic dissipation of superfluid flow in a periodically dressed Bose-Einstein condensate D M Stamper-Kurn Rapidly rotating Bose-Einstein condensates in anharmonic potentials G M Kavoulakis and Gordon Baym Feshbach resonances and collapsing Bose-Einstein condensates J N Milstein, C Menotti and M J Holland Three-body recombination of cold fermionic atoms H Suno, B D Esry and Chris H Greene Bogoliubov spectrum and Bragg spectroscopy of elongated Bose-Einstein condensates C Tozzo and F Dalfovo Quantum atom optics with Bose-Einstein condensates Klaus Mølmer Creation of effective magnetic fields in optical lattices: the Hofstadter butterfly for cold neutral atoms D Jaksch and P Zoller The Josephson frequency of resonantly coupled atomic and molecular condensates R A Duine and H T C Stoof Superfluid current disruption in a chain of weakly coupled Bose–Einstein condensates F S Cataliotti, L Fallani, F Ferlaino, C Fort, P Maddaloni and M Inguscio Bright matter wave solitons in Bose–Einstein condensates K E Strecker, G B Partridge, A G Truscott and R G Hulet Spin dynamics for bosons in an optical lattice Juan José García-Ripoll and Juan Ignacio Cirac Mean field ground state of a spin-1 condensate in a magnetic field Wenxian Zhang, Su Yi and Li You Atom resonant tunnelling through a moving barrier M L Chiofalo, M Artoni and G C La Rocca Local correlations in a strongly interacting one-dimensional Bose gas D M Gangardt and G V Shlyapnikov Shift of the molecular bound state threshold in dense ultracold Fermi gases with Feshbach resonance R Combescot Landau damping in trapped Bose condensed gases B Jackson and E Zaremba An exact reformulation of the Bose–Hubbard model in terms of a stochastic Gutzwiller ansatz Iacopo Carusotto and Yvan Castin Chemical potential standard for atomic Bose–Einstein condensates Sigmund Kohler and Fernando Sols The short-distance first-order correlation function of the interacting one-dimensional Bose gas Maxim Olshanii and Vanja Dunjko The relation between the Gross–Pitaevskii and Bogoliubov descriptions of a dilute Bose gas A J Leggett Superfluidity of Bose–Einstein condensate in an optical lattice: Landau–Zener tunnelling and dynamical instability B Wu and Q Niu Density-optimized efficiency for magneto-optical production of a stable molecular Bose–Einstein condensate Matt Mackie, Anssi Collin, Kalle-Antti Suominen and Juha Javanainen A two-atom picture of coherent atom–molecule quantum beats Bogdan Borca, D Blume and Chris H Greene Superfluid dynamics of a Bose–Einstein condensate in a periodic potential C Menotti, A Smerzi and A Trombettoni Phase diagram of two-component bosons on an optical lattice Ehud Altman, Walter Hofstetter, Eugene Demler and Mikhail D Lukin Murray J Holland University of Colorado at Boulder, USA