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arXiv:1910.00598 · Physical Review Letters

Direct Generation of Tailored Pulse-Mode Entanglement

Francesco Graffitti, Peter Barrow, Alexander Pickston, Agata M. Brańczyk, Alessandro Fedrizzi

Published Feb 4, 2020• 47 citations
arXivHTMLPDF

Abstract

Photonic quantum technology increasingly uses frequency encoding to enable higher quantum information density and noise resilience. Pulsed time-frequency modes (TFM) represent a unique class of spectrally encoded quantum states of light that enable a complete framework for quantum information processing. Here, we demonstrate a technique for direct generation of entangled TFM-encoded states in single-pass, tailored down-conversion processes. We achieve unprecedented quality in state generation-high rates, heralding efficiency, and state fidelity-as characterized via highly resolved time-of-flight fiber spectroscopy and two-photon interference. We employ this technique in a four-photon entanglement swapping scheme as a primitive for TFM-encoded quantum protocols.

DOI
10.1103/physrevlett.124.053603

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•Jan 1, 2015•1 citation
Photonic quantum technology increasingly uses frequency encoding to enable higher quantum information density and noise resilience. Pulsed time-frequency modes (TFM) represent a unique class of spectrally encoded quantum states of light that enable a complete framework for quantum information processing. Here, we demonstrate a technique for direct generation of entangled TFM-encoded states in single-pass, tailored down-conversion processes. We achieve unprecedented quality in state generation-high rates, heralding efficiency, and state fidelity-as characterized via highly resolved time-of-flight fiber spectroscopy and two-photon interference. We employ this technique in a four-photon entanglement swapping scheme as a primitive for TFM-encoded quantum protocols.
Quantum photonics is increasingly making use of the energy-time degree of freedom (DoF) to encode information. Its inherently high-dimensionality offers higher information capacity and robustness against noise. Most frequently, the energy-time DoF is exploited in the form of time bins and frequency bins, with direct applications in both quantum information processing tasks and quantum communication protocols. More recently, it has been used also in its pulse modes (or temporal modes) form, sets of states overlapping in time and frequency but kept orthogonal considering their temporal and spectral phase, whose difficult manipulation and characterisation made it less appealing for experimental applications. The production of states encoded in pulse modes has been demonstrated through sum frequency generation in waveguides [1] and parametric down conversion in bulk crystals [2], as well as the demonstration of schemes for creating hyper-entanglement among energy-time DoF and other high-dimensional DoFs [3], [4]. However, their implementation is still an area of continuous development and evolution, given the complexity of manipulating and characterising them.
The time-frequency degree of freedom is a powerful resource for implementing high-dimensional quantum information processing. In particular, field-orthogonal pulsed temporal modes offer a flexible framework compatible with both long-distance fibre networks and integrated waveguide devices. In order for this architecture to be fully utilised, techniques to reliably generate diverse quantum states of light and accurately measure complex temporal waveforms must be developed. To this end, nonlinear processes mediated by spectrally shaped pump pulses in group-velocity engineered waveguides and crystals provide a capable toolbox. In this review, we examine how tailoring the phasematching conditions of parametric downconversion and sum-frequency generation allows for highly pure single-photon generation, flexible temporal-mode entanglement, and accurate measurement of time-frequency photon states. We provide an overview of experimental progress towards these goals, and summarise challenges that remain in the field.
Hyper-entanglement between two or more photonic degrees of freedom (DOF) can enhance and enable new quantum protocols by allowing each DOF to perform the task it is optimally suited for. Here we demonstrate the generation of photon pairs hyper-entangled between pulse modes and frequency bins. The pulse modes are generated via parametric downconversion in a domain-engineered crystal and subsequently entangled to two frequency bins via a spectral mapping technique. The resulting hyper-entangled state is characterized and verified via measurement of its joint spectral intensity and non-classical two-photon interference patterns from which we infer its spectral phase. The protocol combines the robustness to loss, intrinsic high dimensionality and compatibility with standard fiber-optic networks of the energy-time DOF with the ability of hyper-entanglement to increase the capacity and efficiency of the quantum channel, already exploited in recent experimental applications in both quantum information and quantum computation.
Entanglement is a unique property of quantum systems and an essential resource for many quantum technologies. The ability to transfer or swap entanglement between systems is an important protocol in quantum information science. Entanglement swapping between photons forms the basis of distributed quantum networks. Here an experiment demonstrating entanglement swapping from two independent multimode time-frequency entangled sources is presented, resulting in multiple heralded frequency-mode Bell states. Entanglement in the heralded states is verified by measuring conditional anticorrelated joint spectra and quantum beating in two-photon interference. Our experiment heralds up to five orthogonal Bell pairs within the same setup, and this number is ultimately limited only by the entanglement of the initial sources.
Frequency encoding is quickly becoming an attractive prospect for quantum information protocols owing to larger Hilbert spaces and increased resilience to noise compared to other photonic degrees of freedom. To fully make use of frequency encoding as a practical paradigm for quantum information processing, an efficient and simple source of frequency entanglement is required. Here, we present a single-pass source of discrete frequency-bin entanglement that does not use filtering or a resonant cavity. We use a domain-engineered nonlinear crystal to generate an eight-mode frequency-bin entangled source at telecommunication wavelengths. Our approach leverages the high heralding efficiency and simplicity associated with bulk crystal sources.
Creating and controlling well-defined single-photon states is important for many quantum enhanced technologies. Information can be encoded in any degree of freedom associated with a single-photon field excitation, for example in the polarization or transverse spatial mode structure. The ability to encode multiple qubits in these states is desirable for high data transmission rates and increased information processing capacity. The spectral-temporal domain offers a large Hilbert space for encoding information, well suited to integrated optical architectures owing to the low cross-talk between channels. Indeed, time-frequency encoding is an integral component of existing information technologies infrastructure. Thus, complete, coherent control of the spectral-temporal mode structure of light is essential to advancing optical quantum technologies. Arbitrary control of single-photon states has been demonstrated in the polarization and spatial-momentum degrees of freedom however, is yet to be established in the spectral-temporal domain. Recently it was shown that spectral-temporal pulse shaping is experimentally feasible using nonlinear optical methods. However, such techniques can introduce noise photons, are challenging to implement deterministically and require specially prepared auxiliary pump pulses. Furthermore, they are typically only possible at relatively low repetition rates to avoid damage of nonlinear optical materials. Here, we demonstrate deterministic pulse shaping of single-photon wave packets by introducing a time-varying phase. Applying linear or quadratic phase to the wave packet introduces a spectral shift or spectral broadening, respectively. Achieving significant spectral manipulation requires temporal-phase modulation on the order of π. The phase must also vary on the same time scale as the optical pulses, approximately 1 ps in duration here. This relatively rapid phase variation is achieved using a fast electro-optic phase modulator. The modulator is driven by a time-varying voltage that is synchronized with a pulse train of single-photon wave packets for accurate temporal phase control. In this thesis, we experimentally demonstrate control of the spectral-temporal state of single-photon wave packets using this method. Heralded single-photon wave packets are generated by spontaneous parametric down conversion pumped by a frequency-doubled Titanium-Sapphire laser oscillator with 80 MHz repetition rate. To achieve significant modulation of single-photon pulses a 10 V peak-to-peak radio-frequency signal of 40 GHz drives the phase modulator, which requires approximately 3.6 V to achieve a π phase shift. The signal is synchronized with the oscillator pulse train using custom designed electronics. Details of these electronics are presented, resulting in a robust phase and amplitude controllable 40 GHz voltage source, phase locked to the single-photon pulse train. To demonstrate the utility of this pulse-shaping method we experimentally show spectral shearing of almost 1 nm for single-photon wave packets with 830 nm central wavelength and 1 nm bandwidth. Measurement of the second-order intensity correlation before and after the wave-packet manipulation remains constant within uncertainty of the measurement, showing that the quantum nature of the single-photon source is not deteriorated by the modulator. Preservation of the wave-packet coherence is verified by two-photon interference between spectrally sheared and non-modulated single-photons.