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arXiv:1909.12856 · Physical Review Letters

Dynamical Variational Approach to Bose Polarons at Finite Temperatures

David Dzsotjan, Richard Schmidt, Michael Fleischhauer

Published Jun 2, 2020• 40 citations
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Abstract

We discuss the interaction of a mobile quantum impurity with a Bose-Einstein condensate of atoms at finite temperature. To describe the resulting Bose polaron formation we develop a dynamical variational approach applicable to an initial thermal gas of Bogoliubov phonons. We study the polaron formation after switching on the interaction, e.g., by a radio-frequency (rf) pulse from a noninteracting to an interacting state. To treat also the strongly interacting regime, interaction terms beyond the Fröhlich model are taken into account. We calculate the real-time impurity Green's function and discuss its temperature dependence. Furthermore we determine the rf absorption spectrum and find good agreement with recent experimental observations. We predict temperature-induced shifts and a substantial broadening of spectral lines. The analysis of the real-time Green's function reveals a crossover to a linear temperature dependence of the thermal decay rate of Bose polarons as unitary interactions are approached.

DOI
10.1103/physrevlett.124.223401

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We discuss the interaction of a mobile quantum impurity with a Bose-Einstein condensate of atoms at finite temperature. To describe the resulting Bose polaron formation we develop a dynamical variational approach applicable to an initial thermal gas of Bogoliubov phonons. We study the polaron formation after switching on the interaction, e.g., by a radio-frequency (rf) pulse from a noninteracting to an interacting state. To treat also the strongly interacting regime, interaction terms beyond the Fröhlich model are taken into account. We calculate the real-time impurity Green's function and discuss its temperature dependence. Furthermore we determine the rf absorption spectrum and find good agreement with recent experimental observations. We predict temperature-induced shifts and a substantial broadening of spectral lines. The analysis of the real-time Green's function reveals a crossover to a linear temperature dependence of the thermal decay rate of Bose polarons as unitary interactions are approached.
Recent experimental advances enabled the realization of mobile impurities immersed in a Bose-Einstein condensate (BEC) of ultracold atoms. Here, we consider impurities with two or more internal hyperfine states, and study their radio-frequency (rf) absorption spectra, which correspond to transitions between two different hyperfine states. We calculate rf spectra for the case when one of the hyperfine states involved interacts with the BEC, while the other state is noninteracting, by performing a nonperturbative resummation of the probabilities of exciting different numbers of phonon modes. In the presence of interactions, the impurity gets dressed by Bogoliubov excitations of the BEC, and forms a polaron. The rf signal contains a $\ensuremath{\delta}$-function peak centered at the energy of the polaron measured relative to the bare impurity transition frequency with a weight equal to the amount of bare impurity character in the polaron state. The rf spectrum also has a broad incoherent part arising from the background excitations of the BEC, with a characteristic power-law tail that appears as a consequence of the universal physics of contact interactions. We discuss both the direct rf measurement, in which the impurity is initially in an interacting state, and the inverse rf measurement, in which the impurity is initially in a noninteracting state. In the latter case, in order to calculate the rf spectrum, we solve the problem of polaron formation: a mobile impurity is suddenly introduced in a BEC, and dynamically gets dressed by Bogoliubov phonons. Our solution is based on a time-dependent variational ansatz of coherent states of Bogoliubov phonons, which becomes exact when the impurity is localized. Moreover, we show that such an ansatz compares well with a semiclassical estimate of the propagation amplitude of a mobile impurity in the BEC. Our technique can be extended to cases when both initial and final impurity states are interacting with the BEC.
Mobile impurity atoms immersed in Bose–Einstein condensates provide a new platform for exploring Bose polarons. Recent experimental advances in the field of ultracold atoms make it possible to realize such systems with highly tunable microscopic parameters and to explore equilibrium and dynamical properties of polarons using a rich toolbox of atomic physics. In this paper we present a detailed theoretical analysis of Bose polarons in one-dimensional systems of ultracold atoms. By combining a non-perturbative renormalization group approach with numerically exact diffusion Monte Carlo calculations we obtain not only detailed numerical results over a broad range of parameters but also qualitative understanding of different regimes of the system. We find that an accurate description of Bose polarons requires the inclusion of two-phonon scattering terms which go beyond the commonly used Fröhlich model. Furthermore we show that when the Bose gas is in the strongly interacting regime, one needs to include interactions between the phonon modes. We use several theoretical approaches to calculate the polaron energy and its effective mass. The former can be measured using radio-frequency spectroscopy and the latter can be studied experimentally using impurity oscillations in a harmonic trapping potential. We compare our theoretical results for the effective mass to the experiments by Catani et al (2012 Phys. Rev. A 85 023623). In the weak-to-intermediate coupling regimes we obtain excellent quantitative agreement between theory and experiment, without any free fitting parameter. We supplement our analysis by full dynamical simulations of polaron oscillations in a shallow trapping potential. We also use our renormalization group approach to analyze the full phase diagram and identify regions that support repulsive and attractive polarons, as well as multi-particle bound states.
Mobile impurity atoms immersed in Bose–Einstein condensates provide a new platform for exploring Bose polarons. Recent experimental advances in the field of ultracold atoms make it possible to realize such systems with highly tunable microscopic parameters and to explore equilibrium and dynamical properties of polarons using a rich toolbox of atomic physics. In this paper we present a detailed theoretical analysis of Bose polarons in one-dimensional systems of ultracold atoms. By combining a non-perturbative renormalization group approach with numerically exact diffusion Monte Carlo calculations we obtain not only detailed numerical results over a broad range of parameters but also qualitative understanding of different regimes of the system. We find that an accurate description of Bose polarons requires the inclusion of two-phonon scattering terms which go beyond the commonly used Fröhlich model. Furthermore we show that when the Bose gas is in the strongly interacting regime, one needs to include interactions between the phonon modes. We use several theoretical approaches to calculate the polaron energy and its effective mass. The former can be measured using radio-frequency spectroscopy and the latter can be studied experimentally using impurity oscillations in a harmonic trapping potential. We compare our theoretical results for the effective mass to the experiments by Catani et al (2012 Phys. Rev. A 85 023623). In the weak-to-intermediate coupling regimes we obtain excellent quantitative agreement between theory and experiment, without any free fitting parameter. We supplement our analysis by full dynamical simulations of polaron oscillations in a shallow trapping potential. We also use our renormalization group approach to analyze the full phase diagram and identify regions that support repulsive and attractive polarons, as well as multi-particle bound states.
We analyze the dynamics of Bose polarons in the vicinity of a Feshbach resonance between the impurity and host atoms. We compute the radio-frequency absorption spectra for the case when the initial state of the impurity is noninteracting and the final state is strongly interacting with the host atoms. We compare results of different theoretical approaches including a single excitation expansion, a self-consistent T-matrix method, and a time-dependent coherent state approach. Our analysis reveals sharp spectral features arising from metastable states with several Bogoliubov excitations bound to the impurity atom. This surprising result of the interplay of many-body and few-body Efimov type bound state physics can only be obtained by going beyond the commonly used Fröhlich model and including quasiparticle scattering processes. Close to the resonance we find that strong fluctuations lead to a broad, incoherent absorption spectrum where no quasiparticle peak can be assigned.
When a mobile impurity interacts with a surrounding bath of bosons, it forms a polaron. Numerous methods have been developed to calculate how the energy and the effective mass of the polaron are renormalized by the medium for equilibrium situations. Here, we address the much less studied nonequilibrium regime and investigate how polarons form dynamically in time. To this end, we develop a time-dependent renormalization-group approach which allows calculations of all dynamical properties of the system and takes into account the effects of quantum fluctuations in the polaron cloud. We apply this method to calculate trajectories of polarons following a sudden quench of the impurity-boson interaction strength, revealing how the polaronic cloud around the impurity forms in time. Such trajectories provide additional information about the polaron's properties which are challenging to extract directly from the spectral function measured experimentally using ultracold atoms. At strong couplings, our calculations predict the appearance of trajectories where the impurity wavers back at intermediate times as a result of quantum fluctuations. Our method is applicable to a broader class of nonequilibrium problems. As a check, we also apply it to calculate the spectral function and find good agreement with experimental results. At very strong couplings, we predict that quantum fluctuations lead to the appearance of a dark continuum with strongly suppressed spectral weight at low energies. While our calculations start from an effective Fr\"ohlich Hamiltonian describing impurities in a three-dimensional Bose-Einstein condensate, we also calculate the effects of additional terms in the Hamiltonian beyond the Fr\"ohlich paradigm. We demonstrate that the main effect of these additional terms on the attractive side of a Feshbach resonance is to renormalize the coupling strength of the effective Fr\"ohlich model.
We consider an impurity immersed in a Bose-Einstein condensate with tunable boson-impurity interactions. Such a Bose polaron has recently been predicted to exhibit an intriguing energy spectrum at finite temperature, where the ground-state quasiparticle evenly splits into two branches as the temperature is increased from zero [Guenther et al., Phys. Rev. Lett. 120, 050405 (2018)]. To investigate this theoretical prediction, we employ a recently developed variational approach that systematically includes multibody correlations between the impurity and the finite-temperature medium, thus allowing us to go beyond previous finite-temperature methods. Crucially, we find that the number of quasiparticle branches is simply set by the number of hole excitations of the thermal cloud, such that including up to one hole yields one splitting, two holes yields two splittings, and so on. Moreover, this effect is independent of the impurity mass. We thus expect that the exact ground-state quasiparticle will evolve into a single broad peak for temperatures T>0T>0T>0, with a broadening that scales as T3/4{T}^{3/4}T3/4 at low temperatures and sufficiently weak boson-boson interactions. In the zero-temperature limit, we show that our calculated ground-state polaron energy is in excellent agreement with recent quantum Monte Carlo results and with experiments.