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arXiv:1909.11959 · Physical Review X

Glassy Dynamics in a Disordered Heisenberg Quantum Spin System

Adrien Signoles, T. Franz, R. Ferracini Alves, M. Gärttner, S. Whitlock, G. Zürn, Matthias Weidemüller

Published Jan 19, 2021• 87 citations
arXivHTMLPDF

Abstract

Understanding the dynamics of strongly interacting disordered quantum systems is one of the most challenging problems in modern science, due to features such as the breakdown of thermalization and the emergence of glassy phases of matter.We report on the observation of anomalous relaxation dynamics in an isolated XXZ quantum spin system realized by an ultracold gas of atoms initially prepared in a superposition of two different Rydberg states.The total magnetization is found to exhibit subexponential relaxation analogous to classical glassy dynamics, but in the quantum case this relaxation originates from the buildup of nonclassical correlations.In both experiment and semiclassical simulations, we find the evolution toward a randomized state is independent of the strength of disorder up to a critical value.This hints toward a unifying description of relaxation dynamics in disordered isolated quantum systems, analogous to the generalization of statistical mechanics to out-of-equilibrium scenarios in classical spin glasses.

DOI
10.1103/physrevx.11.011011

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Understanding the dynamics of strongly interacting disordered quantum systems is one of the most challenging problems in modern science, due to features such as the breakdown of thermalization and the emergence of glassy phases of matter.We report on the observation of anomalous relaxation dynamics in an isolated XXZ quantum spin system realized by an ultracold gas of atoms initially prepared in a superposition of two different Rydberg states.The total magnetization is found to exhibit subexponential relaxation analogous to classical glassy dynamics, but in the quantum case this relaxation originates from the buildup of nonclassical correlations.In both experiment and semiclassical simulations, we find the evolution toward a randomized state is independent of the strength of disorder up to a critical value.This hints toward a unifying description of relaxation dynamics in disordered isolated quantum systems, analogous to the generalization of statistical mechanics to out-of-equilibrium scenarios in classical spin glasses.
Understanding how closed quantum systems dynamically approach thermal equilibrium presents a major unresolved problem in statistical physics. Generically, non-integrable quantum systems are expected to thermalize as they comply with the Eigenstate Thermalization Hypothesis. However, in the presence of strong disorder, the dynamics can possibly slow down to a degree that systems fail to thermalize on experimentally accessible timescales, as in spin glasses or many-body localized systems. In general, particularly in long-range interacting quantum systems, the specific nature of the disorder necessary for the emergence of a prethermal, metastable state--distinctly separating the timescales of initial relaxation and subsequent slow thermalization--remains an open question. We study an ensemble of Heisenberg spins with a tunable distribution of random coupling strengths realized by a Rydberg quantum simulator. We observe a drastic change in the late-time magnetization when increasing disorder strength. The data is well described by models based on pairs of strongly interacting spins, which are treated as thermal for weak disorder and isolated for strong disorder. Our results indicate a crossover into a pair-localized prethermal regime in a closed quantum system of thousands of spins in the critical case where the exponent of the power law interaction matches the spatial dimension.
An important step towards a comprehensive understanding of far-from-equilibrium dynamics of quantum many-body systems is the identification of unifying features that are independent of microscopic details of the system. We experimentally observe such robust features in the magnetization relaxation dynamics of disordered Heisenberg XX, XXZ, and Ising Hamiltonians. We realize these Heisenberg spin models with tunable anisotropy parameter and power-law interactions in an ensemble of Rydberg atoms by encoding the spin in suitable Rydberg state combinations. We consistently observe stretched-exponential relaxation of magnetization for all considered spin models, collapsing onto a single curve after appropriate rescaling of time. This robust short-time relaxation behavior is explained by a perturbative treatment that exploits the strong disorder in pairwise couplings, which leads to a description in terms of approximately independent pairs of spins. In numerical simulations of small systems, we show that these pairs of spins constitute approximate local integrals of motion, which remain at least partially conserved on a timescale exceeding the duration of the relaxation dynamics of the magnetization. Published by the American Physical Society 2024
We numerically study out-of-equilibrium dynamics in a family of Heisenberg models with 1/r61/{r}^{6}1/r6 power-law interactions and positional disorder. Using the semiclassical discrete truncated Wigner approximation (dTWA) method, we investigate the time evolution of the magnetization and ensemble-averaged single-spin purity for a strongly disordered system after initializing the system in an out-of-equilibrium state. We find that both quantities display robust glassy behavior for almost any value of the anisotropy parameter of the Heisenberg Hamiltonian. Furthermore, a systematic analysis allows us to quantitatively show that, for all the scenarios considered, the stretch power lies close to the one analytically obtained in the Ising limit. This indicates that glassy relaxation behavior occurs widely in disordered quantum spin systems, independent of the particular symmetries and integrability of the Hamiltonian.
We study the out-of-equilibrium dynamics of the quantum Ising model with power-law interactions and positional disorder. For arbitrary dimension ddd and interaction range $\ensuremath{\alpha}\ensuremath{\ge}d$ we analytically find a stretched-exponential decay of the global magnetization and ensemble-averaged single-spin purity with a stretch power $\ensuremath{\beta}=d/\ensuremath{\alpha}$ in the thermodynamic limit. Numerically, we confirm that glassy behavior persists for finite system sizes and sufficiently strong disorder. We identify dephasing between disordered coherent pairs as the main mechanism leading to a relaxation of global magnetization, whereas genuine many-body interactions lead to a loss of single-spin purity which signifies the buildup of entanglement. The emergence of glassy dynamics in the quantum Ising model extends prior findings in classical and open quantum systems, where the stretched-exponential law is explained by a scale-invariant distribution of timescales, to both integrable and nonintegrable quantum systems.
How do isolated quantum systems approach an equilibrium state? We experimentally and theoretically address this question for a prototypical spin system formed by ultracold atoms prepared in two Rydberg states with different orbital angular momenta. By coupling these states with a resonant microwave driving, we realize a dipolar XY spin-1/2 model in an external field. Starting from a spin-polarized state, we suddenly switch on the external field and monitor the subsequent many-body dynamics. Our key observation is density dependent relaxation of the total magnetization much faster than typical decoherence rates. To determine the processes governing this relaxation, we employ different theoretical approaches that treat quantum effects on initial conditions and dynamical laws separately. This allows us to identify an intrinsically quantum component to the relaxation attributed to primordial quantum fluctuations.
Recent advances in theoretical physics have increasingly focused on the dynamics of quantum systems with many interacting degrees of freedom, while ultracold atom platforms now enable the realization of diverse theoretical models with precise control over system parameters and advanced monitoring techniques. A prominent example is cavity quantum electrodynamics (CQED), where large atomic or molecular ensembles are coupled to high-finesse optical cavities, enabling strong interaction with confined electromagnetic modes and leading to phenomena such as the superradiant phase transition, in which atoms and photons form a coherent state. Most theoretical studies of CQED have concentrated on regimes of spatially uniform atom–cavity coupling, where collective behavior allows a description in terms of the classical dynamics of a few macroscopic variables. However, experimental capabilities now permit exploration beyond this limit, though theoretical progress is hindered by the exponential computational complexity of simulating large quantum systems, particularly when environmental coupling is included. This thesis addresses such challenges by developing efficient approaches, within the Keldysh formalism of non-equilibrium quantum field theory, to study systems with strongly disordered interactions coupled to external reservoirs. Two representative models are considered: a disordered spin–boson model describing light–matter interactions with quenched disorder, relevant to recent CQED experiments in confocal cavities, and a fermion–phonon system governed by the Yukawa–Sachdev–Ye–Kitaev (Yukawa-SYK) model. Both systems are quantum critical, exhibiting a continuum of low-energy modes above their stationary states, yet disorder produces qualitatively distinct dynamical behaviors: in the spin–boson system it induces slow, glassy relaxation, whereas in the Yukawa-SYK model it leads to rapid thermalization. These contrasting outcomes reveal the non-trivial role of disorder in quantum many-body systems and motivate further investigation into its effects on non-equilibrium quantum dynamics.