Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1909.04294 · Optics Express

Single-photon characterization by two-photon spectral interferometry

Valérian Thiel, Alex O. C. Davis, Ke Sun, Peru d’Ornellas, Xian-Min Jin, Brian J. Smith

Published Jun 5, 2020• 22 citations
arXivHTMLPDF

Abstract

Single-photon sources are a fundamental resource in quantum optics and quantum information science. Photons with differing spectral and temporal shapes do not interfere well and inhibit the performance of quantum applications such as linear optics quantum computing, boson sampling, and quantum networks. Indistinguishability and purity of photons emitted from different sources are crucial properties for many quantum applications. The ability to determine the state of single-photon sources therefore provides a means to assess their quality, compare different sources, and provide feedback for source tuning. Here, we propose and demonstrate a single-configuration experimental method enabling complete characterization of the spectral-temporal state of a pulsed single-photon source having both pure and mixed states. The method involves interference of the unknown single-photon source with a reference at a balanced beam splitter followed by frequency-resolved coincidence detection at the outputs. Fourier analysis of the joint-spectral two-photon interference pattern reveals the density matrix of the single-photon source in the frequency basis. We present an experimental realization of this method for pure and mixed state pulsed single-photon sources.

DOI
10.1364/oe.396960

Related papers

Experimental single-photon pulse characterization by electro-optic shearing interferometry

Alex O. C. Davis, Valérian Thiel, Michał Karpiński +1 more

The ability to characterize the complete quantum state of light is essential for both fundamental and applied science. For single photons the quantum state is provided by the mode that it occupies. The spectral temporal mode structure of light has recently emerged as an essential means for quantum information science. Here we experimentally demonstrate a self-referencing technique to completely determine the pulse-mode structure of single photons by means of spectral shearing interferometry. We detail the calibration and resolution of the measurement and discuss challenges and critical requirements for future advances of this method.

arXiv:1802.07208•Physical Review A•Aug 21, 2018•19 citations

Measuring the Single-Photon Temporal-Spectral Wave Function

Alex O. C. Davis, Valérian Thiel, Michał Karpiński +1 more

Temporal-spectral modes of light provide a fundamental window into the nature of quantum systems and offer a robust means for information encoding. Methods to precisely characterize the temporal-spectral state of light at the single-photon level thus play a central role in understanding single-photon sources and their applications in emerging optical quantum technologies. Here we demonstrate an optical reference-free method, which melds techniques from ultrafast metrology and single-photon spectral detection, to characterize the pulse-mode structure of heralded single photons.

arXiv:1709.05248•Physical Review Letters•Aug 21, 2018•60 citations

Characterizing mixed-state entanglement through single-photon interference

Mayukh Lahiri, Radek Łapkiewicz, Armin Hochrainer +2 more

Entanglement verification and measurement is essential for experimental tests of quantum mechanics and also for quantum communication and information science. Standard methods of verifying entanglement in a bipartite mixed state require detection of both particles and involve coincidence measurement. We present a method that enables us to verify and measure entanglement in a two-photon mixed state without detecting one of the photons, i.e., without performing any coincidence measurement or postselection. We consider two identical sources, each of which can generate the same two-photon mixed state but they never emit simultaneously. We show that one can produce a set of single-photon interference patterns, which contain information about entanglement in the two-photon mixed state. We prove that it is possible to retrieve the information about entanglement from the visibility of the interference patterns. Our method reveals a distinct avenue for verifying and measuring entanglement in mixed states.

arXiv:2009.02829•Physical Review A•Jul 6, 2021•18 citations

Spectral Characterization of Two-Photon Interference between Independent Sources

Lifeng Duan, Aojie Xu, Yun Zhang

We present a spectral characterization of two-photon nonclassical interference on a beam splitter (BS) between a weak coherent state source and another source, which emits a phase-randomized weak coherent state, a single-photon state, or a thermal state. Besides spectral characteristics, the average photon number ratio in a given time interval is also considered in our model. The two-photon coincidence probability of two outputs of the BS is numerically calculated with spectral bandwidth ratio and average photon number ratio. Furthermore, the noise of the detection system is taken into account. This also indicates that two-photon interference is able to significantly improve by subtracting two-photon contributions from the input state. All these parameters have a close relation to a real experiment performance and the results may pave new avenues for quantum information technology when two-photon interference between independent sources is necessary.

Photonics•Oct 7, 2023•2 citations

Temporal Purity and Quantum Interference of Single Photons from Two Independent Cold Atomic Ensembles

Peng Qian, Zhenjie Gu, Rong Cao +4 more

The temporal purity of single photons is crucial to the indistinguishability of independent photon sources for the fundamental study of the quantum nature of light and the development of photonic technologies. Currently, the technique for single photons heralded from time-frequency entangled biphotons created in nonlinear crystals does not guarantee the temporal-quantum purity, except using spectral filtering. Nevertheless, an entirely different situation is anticipated for narrow-band biphotons with a coherence time far longer than the time resolution of a single-photon detector. Here we demonstrate temporally pure single photons with a coherence time of 100 ns, directly heralded from the time-frequency entangled biphotons generated by spontaneous four-wave mixing in cold atomic ensembles, without any supplemented filters or cavities. A near-perfect purity and indistinguishability are both verified through Hong-Ou-Mandel quantum interference using single photons from two independent cold atomic ensembles. The time-frequency entanglement provides a route to manipulate the pure temporal state of the single-photon source.

Physical Review Letters•Jul 1, 2016•41 citations

Time–frequency mode structure study of ultrafast two-photon quantum state with two-color dual-comb-based optical sampling

Prasad Koviri, Takahisa Kuwana, Hajime Komori +6 more

Quantum correlations of ultrafast quantum optical states in the time–frequency domain manifest prominently on femtosecond time scales, an elusive challenging regime. We develop a new method to probe the time–frequency mode structure of ultrafast two-photon states utilizing dual-comb-based asynchronously overlapping pulses with single-photon frequency upconversion through femtosecond optical sampling. This method enables quick, highly precise joint temporal intensity measurements over a broad temporal dynamic range with only a single linear scanning stage. We demonstrate full characterization of time–frequency entangled two-photon states in both time and frequency domains. We quantified the time–frequency mode structure in both time and frequency domains through Schmidt decomposition, resulting in temporal and spectral purities of 87.7% and 76.9%, respectively, for heralded single-photons without any spectral filtering. Furthermore, through the simple control of pump spectral bandwidth, we demonstrate the ability to tailor time–frequency entanglement, verifying the two-dimensional Fourier duality. This method paves the way for a substantial upgrade to ultrafast quantum optical techniques, enabling a rapid, detailed, and multi-dimensional characterization of entangled states with potential applications in quantum metrology and photon-deficient fluorescence imaging.

APL Photonics•May 1, 2025•2 citations
Single-photon sources are a fundamental resource in quantum optics and quantum information science. Photons with differing spectral and temporal shapes do not interfere well and inhibit the performance of quantum applications such as linear optics quantum computing, boson sampling, and quantum networks. Indistinguishability and purity of photons emitted from different sources are crucial properties for many quantum applications. The ability to determine the state of single-photon sources therefore provides a means to assess their quality, compare different sources, and provide feedback for source tuning. Here, we propose and demonstrate a single-configuration experimental method enabling complete characterization of the spectral-temporal state of a pulsed single-photon source having both pure and mixed states. The method involves interference of the unknown single-photon source with a reference at a balanced beam splitter followed by frequency-resolved coincidence detection at the outputs. Fourier analysis of the joint-spectral two-photon interference pattern reveals the density matrix of the single-photon source in the frequency basis. We present an experimental realization of this method for pure and mixed state pulsed single-photon sources.
The ability to characterize the complete quantum state of light is essential for both fundamental and applied science. For single photons the quantum state is provided by the mode that it occupies. The spectral temporal mode structure of light has recently emerged as an essential means for quantum information science. Here we experimentally demonstrate a self-referencing technique to completely determine the pulse-mode structure of single photons by means of spectral shearing interferometry. We detail the calibration and resolution of the measurement and discuss challenges and critical requirements for future advances of this method.
Temporal-spectral modes of light provide a fundamental window into the nature of quantum systems and offer a robust means for information encoding. Methods to precisely characterize the temporal-spectral state of light at the single-photon level thus play a central role in understanding single-photon sources and their applications in emerging optical quantum technologies. Here we demonstrate an optical reference-free method, which melds techniques from ultrafast metrology and single-photon spectral detection, to characterize the pulse-mode structure of heralded single photons.
Entanglement verification and measurement is essential for experimental tests of quantum mechanics and also for quantum communication and information science. Standard methods of verifying entanglement in a bipartite mixed state require detection of both particles and involve coincidence measurement. We present a method that enables us to verify and measure entanglement in a two-photon mixed state without detecting one of the photons, i.e., without performing any coincidence measurement or postselection. We consider two identical sources, each of which can generate the same two-photon mixed state but they never emit simultaneously. We show that one can produce a set of single-photon interference patterns, which contain information about entanglement in the two-photon mixed state. We prove that it is possible to retrieve the information about entanglement from the visibility of the interference patterns. Our method reveals a distinct avenue for verifying and measuring entanglement in mixed states.
We present a spectral characterization of two-photon nonclassical interference on a beam splitter (BS) between a weak coherent state source and another source, which emits a phase-randomized weak coherent state, a single-photon state, or a thermal state. Besides spectral characteristics, the average photon number ratio in a given time interval is also considered in our model. The two-photon coincidence probability of two outputs of the BS is numerically calculated with spectral bandwidth ratio and average photon number ratio. Furthermore, the noise of the detection system is taken into account. This also indicates that two-photon interference is able to significantly improve by subtracting two-photon contributions from the input state. All these parameters have a close relation to a real experiment performance and the results may pave new avenues for quantum information technology when two-photon interference between independent sources is necessary.
The temporal purity of single photons is crucial to the indistinguishability of independent photon sources for the fundamental study of the quantum nature of light and the development of photonic technologies. Currently, the technique for single photons heralded from time-frequency entangled biphotons created in nonlinear crystals does not guarantee the temporal-quantum purity, except using spectral filtering. Nevertheless, an entirely different situation is anticipated for narrow-band biphotons with a coherence time far longer than the time resolution of a single-photon detector. Here we demonstrate temporally pure single photons with a coherence time of 100 ns, directly heralded from the time-frequency entangled biphotons generated by spontaneous four-wave mixing in cold atomic ensembles, without any supplemented filters or cavities. A near-perfect purity and indistinguishability are both verified through Hong-Ou-Mandel quantum interference using single photons from two independent cold atomic ensembles. The time-frequency entanglement provides a route to manipulate the pure temporal state of the single-photon source.
Quantum correlations of ultrafast quantum optical states in the time–frequency domain manifest prominently on femtosecond time scales, an elusive challenging regime. We develop a new method to probe the time–frequency mode structure of ultrafast two-photon states utilizing dual-comb-based asynchronously overlapping pulses with single-photon frequency upconversion through femtosecond optical sampling. This method enables quick, highly precise joint temporal intensity measurements over a broad temporal dynamic range with only a single linear scanning stage. We demonstrate full characterization of time–frequency entangled two-photon states in both time and frequency domains. We quantified the time–frequency mode structure in both time and frequency domains through Schmidt decomposition, resulting in temporal and spectral purities of 87.7% and 76.9%, respectively, for heralded single-photons without any spectral filtering. Furthermore, through the simple control of pump spectral bandwidth, we demonstrate the ability to tailor time–frequency entanglement, verifying the two-dimensional Fourier duality. This method paves the way for a substantial upgrade to ultrafast quantum optical techniques, enabling a rapid, detailed, and multi-dimensional characterization of entangled states with potential applications in quantum metrology and photon-deficient fluorescence imaging.