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arXiv:1909.01393

Effects of spatial dispersion on Self--induced transparency in two--level media

Zoran M. Ivić, Dalibor Čevizović, Željko Pržulj, Nikos Lazaridess, George P. Tsironis

Published Sep 3, 2019• 0 citations
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Abstract

We study the effects of dispersion in carrier waves on the properties of soliton self--induced transparency (SIT) in two level media. We found substantial impact of dispersion effects on typical SIT soliton features. For example, the degree of SIT pulse velocity slowing down (acceleration) is determined by the ratio of the incoming pulse frequency over atomic transition frequency - $x=ω/ω_0$. Specifically, an immediate pulse stopping is predicted for absorbing media when pulse duration time exceeds some critical value. In the sharp line limit stopping may emerge only for frequency ratio above unity, while for the inhomogeneously broadened systems it appears irrespective of the value of $x$. Analysis performed on the basis of Mcall\& Hahn \textit{Area theorem} implies that pulse stopping is achieved when Ber's absorption coefficient approaches infinity, that is, pulse energy is fully absorbed in the medium. In the case of amplifying media super-luminal motion is predicted as in the case of resonance. However, there is a lowest value in the frequency ratio below which the pulse velocity tends to the sub-luminal region. These new features of the SIT phenomenon open novel ways on how it may be exploited for the control of electromagnetic wave radiation in two-level media. This may be achieved by varying frequency ratio.

DOI
10.48550/arxiv.1909.01393

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We study the effects of dispersion in carrier waves on the properties of soliton self--induced transparency (SIT) in two level media. We found substantial impact of dispersion effects on typical SIT soliton features. For example, the degree of SIT pulse velocity slowing down (acceleration) is determined by the ratio of the incoming pulse frequency over atomic transition frequency - x=ω/ω0x=ω/ω_0x=ω/ω0​. Specifically, an immediate pulse stopping is predicted for absorbing media when pulse duration time exceeds some critical value. In the sharp line limit stopping may emerge only for frequency ratio above unity, while for the inhomogeneously broadened systems it appears irrespective of the value of xxx. Analysis performed on the basis of Mcall& Hahn \textit{Area theorem} implies that pulse stopping is achieved when Ber's absorption coefficient approaches infinity, that is, pulse energy is fully absorbed in the medium. In the case of amplifying media super-luminal motion is predicted as in the case of resonance. However, there is a lowest value in the frequency ratio below which the pulse velocity tends to the sub-luminal region. These new features of the SIT phenomenon open novel ways on how it may be exploited for the control of electromagnetic wave radiation in two-level media. This may be achieved by varying frequency ratio.
The standard self-induced transparency (SIT) phenomenon represents the lossless propagation of a long multicycle stable soliton in an absorbing two-level resonant medium, if the soliton's envelope area equals $2\ensuremath{\pi}$ ($2\ensuremath{\pi}$ pulse). In this case, the leading half of the $2\ensuremath{\pi}$ pulse excites the medium, while the trailing half completely brings the medium back to the ground state. In this work, we theoretically demonstrate an analogous phenomenon for subcycle pulses propagating in an arbitrary multilevel resonant medium. The duration of the obtained solitary pulses must be smaller than the periods of resonant transitions in the medium. The obtained subcycle solitary solutions first turn an initially unexcited multi-level resonant medium to excited levels and then fully return it back to the ground state.
We theoretically show that a self-induced transparency (SIT) soliton and a Bragg soliton can coexist in a nonlinear photonic band gap (PBG) medium doped uniformly with inhomogeneous-broadening two-level atoms. The Maxwell-Bloch equations for the pulse propagating through such a uniformly doped PBG structure are derived first and further reduced to an effective nonlinear Schrödinger equation. This model describes an equivalent physical mechanism for a Bragg-soliton propagation resulting from the effective quadratic dispersion balancing with the effective third-order nonlinearity. Because the resonant atoms are taken into account, the original band gap can be shifted both by the dopants and the instantaneous nonlinearity response originating from an intense optical pulse. As a result, even if a SIT soliton with its central frequency deep inside the original forbidden band, it still can propagate through the resonant PBG medium as long as this SIT soliton satisfies the effective Bragg-soliton propagation. An approximate soliton solution describing such coexistence is found. We also show that the pulse width and group velocity of this soliton solution can be uniquely determined for given material parameters, atomic transition frequency, and input central frequency of the soliton. The numerical examples of the SIT soliton in a one-dimensional As2S3-based PBG structure doped uniformly with Lorentzian line-shape resonant atoms are shown. It is found that a SIT soliton with approximately 100-ps width in such a resonant PBG structure can travel with the velocity being two orders of magnitude slower than the light speed in an unprocessed host medium.
Above a critical power threshold for a given pulse width, a short pulse of coherent traveling-wave optical radiation is observed to propagate with anomalously low energy loss while at resonance with a two-quantum-level system of absorbers. The line shape of the resonant system is determined by inhomogeneous broadening, and the pulse width is short compared to dissipative relaxation times. A new mechanism of self-induced transparency, which accounts for the low energy loss, is analyzed in the ideal limit of a plane wave which excites a resonant medium with no damping present. The stable condition of transparency results after the traversal of the pulse through a few classical absorption lengths into the medium. This condition exists when the initial pulse has evolved into a symmetric hyperbolic-secant pulse function of time and distance, and has the area characteristic of a "$2\ensuremath{\pi}$ pulse." Ideal transparency then persists when coherent induced absorption of pulse energy during the first half of the pulse is followed by coherent induced emission of the same amount of energy back into the beam direction during the second half of the pulse. The effects of dissipative relaxation times upon pulse energy, pulse area, and pulse delay time are analyzed to first order in the ratio of short pulse width to long damping time. The analysis shows that the $2\ensuremath{\pi}$ pulse condition can be maintained if losses caused by damping are compensated by beam focusing. In an amplifying inhomogeneously broadened medium an analytic "$\ensuremath{\pi}$ pulse area" solution is presented in the limit of a sharp leading edge of the pulse. The dynamics of self-induced transparency are studied for the particular effects of Doppler velocities upon a resonant gas. The analysis of transparency for random orientations of dipole moments associated with degenerate rotational states yields modified forms of self-induced transparency behavior, which indicates a finite pulse energy loss as a function of distance in some cases. The effect of self-induced transparency on the photon echo is considered. Experimental observations of self-induced transparency have been made in a ruby sample at resonance with a pulsed ruby-laser beam. Single and multiple $2\ensuremath{\pi}$ pulse outputs have been observed, and pulse areas measured in the range of $2\ensuremath{\pi}$. The experimental results are compared with the predictions of the ideal-plane-wave theory. Deviations from the ideal-plane-wave theory are discussed. An analysis is made of the effect of a transverse mode of the propagating beam upon the transparency properties of the pulse.
Self-induced transparency (SIT) is a kind of coherent transient phenomena in two-level atomic system. The optical pulse with an area that is an integer multiple of 2π, which causes SIT in an absorber, is stable and a kind of soliton. Thus SIT is expected to be useful in pulse compression and pulse shaping. In this paper, we discuss some problems in experiments of SIT and surveys the experimental results of SIT. It is also described the recent experimental results of coherent nonlinear pulse propagation in BiI3 crystal using tunable sub-picosecond pulses.
We derive the properties of self-induced transparency (SIT) solitary waves in a one-dimensional periodic structure doped uniformly with resonance two-level atoms. In our model, the electromagnetic field is treated classically and the dopant atoms are described quantum mechanically. The resulting solitary waves take the form of ultrashort (picosecond) laser pulses which propagate near the band edge of the nonlinear photonic band gap (PBG) material doped with rare-earth atoms such as erbium. Solitary wave formation involves the combined effects of group velocity dispersion (GVD), nonresonant Kerr nonlinearity, and resonant interaction with dopant atoms. We derive the general Maxwell-Bloch equations for a nonlinear PBG system and then demonstrate the existence of elementary solitary wave solutions for frequencies far outside the gap where GVD effects are negligible and for frequencies near the photonic band edge where GVD effects are crucial. We find two distinct new types of propagating SIT solitary wave pulses. Far from Bragg resonance, we recapture the usual McCall-Hahn soliton with hyperbolic secant profile when the nonlinear Kerr coefficient ${\ensuremath{\chi}}^{(3)}=0.$ However, when the host nonresonant Kerr coefficient is nonzero, we obtain the first new type of soliton. In this case, the optical soliton envelope function deviates from the hyperbolic secant profile and pulse propagation requires nontrivial phase modulation (chirping). We derive the dependence of the solitary wave structure on the Kerr coefficient ${\ensuremath{\chi}}^{(3)},$ the resonance impurity atom density, and the detuning of the average laser frequency from the atomic transition. When the laser frequency and the atomic transition frequencies are near the photonic band edge we obtain the second type of soliton. To illustrate the second type of soliton we consider two special cases. In the first case, GVD facilitates the propagation of an unchirped SIT-gap soliton moving at a velocity fixed by the material's parameters. The soliton structure changes dramatically as the laser frequency is tuned through the atomic resonance. In the second illustrative case we set the Kerr coefficient ${\ensuremath{\chi}}^{(3)}=0.$ In this case, the solution is a chirped pulse which arises from the balance between GVD and the resonance interaction with the dopant atoms. Finally, we show that under certain circumstances, these solitary wave solutions may persist even in the presence of (subpicosecond) dipolar dephasing of the dopant atoms and absorption losses of the host PBG material, provided that the system is incoherently pumped. These results may be relevant to the application of PBG materials as optical devices in fiber-optic networks.