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arXiv:1908.04368 · Physical Review A

Dark-state optical potential barriers with nanoscale spacing

Wenchao Ge, Muhammad Suhail Zubairy

Published Feb 5, 2020• 12 citations
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Abstract

Optical potentials have been a versatile tool for the study of atomic motions and many-body interactions in cold atoms. Recently, optical subwavelength single barriers were proposed to enhance the atomic interaction energy scale, which is based on nonadiabatic corrections to Born-Oppenheimer potentials. Here we present a study for creating an alternative landscape of nonadiabatic potentials---multiple barriers with subwavelength spacing at tens of nanometers. To realize these potentials, spatially rapid-varying dark states of atomic $\mathrm{\ensuremath{\Lambda}}$ configurations are formed by controlling the spatial intensities of the driving lasers. As an application, we show that bound states of very long lifetimes on the order of seconds can be realized. Imperfections and experimental realizations of the multiple barriers are also discussed.

DOI
10.1103/physreva.101.023403

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Optical potentials have been a versatile tool for the study of atomic motions and many-body interactions in cold atoms. Recently, optical subwavelength single barriers were proposed to enhance the atomic interaction energy scale, which is based on nonadiabatic corrections to Born-Oppenheimer potentials. Here we present a study for creating an alternative landscape of nonadiabatic potentials---multiple barriers with subwavelength spacing at tens of nanometers. To realize these potentials, spatially rapid-varying dark states of atomic \ensuremathΛ\mathrm{\ensuremath{\Lambda}}\ensuremathΛ configurations are formed by controlling the spatial intensities of the driving lasers. As an application, we show that bound states of very long lifetimes on the order of seconds can be realized. Imperfections and experimental realizations of the multiple barriers are also discussed.
We discuss the generation of subwavelength optical barriers on the scale of tens of nanometers, as conservative optical potentials for cold atoms. These arise from nonadiabatic corrections to Born-Oppenheimer potentials from dressed "dark states" in atomic Λ configurations. We illustrate the concepts with a double layer potential for atoms obtained from inserting an optical subwavelength barrier into a well generated by an off-resonant optical lattice, and discuss bound states of pairs of atoms interacting via magnetic dipolar interactions. The subwavelength optical barriers represent an optical "Kronig-Penney" potential. We present a detailed study of the band structure in optical Kronig-Penney potentials, including decoherence from spontaneous emission and atom loss to open "bright" channels.
We propose a method for creating far-field optical barrier potentials for ultracold atoms with widths that are narrower than the diffraction limit and can approach tens of nanometers. The reduced widths stem from the nonlinear atomic response to control fields that create spatially varying dark resonances. The subwavelength barrier is the result of the geometric scalar potential experienced by an atom prepared in such a spatially varying dark state. The performance of this technique, as well as its applications to the study of many-body physics and to the implementation of quantum-information protocols with ultracold atoms, are discussed, with a focus on the implementation of tunnel junctions.
We report on the experimental realization of a conservative optical lattice for cold atoms with a subwavelength spatial structure. The potential is based on the nonlinear optical response of three-level atoms in laser-dressed dark states, which is not constrained by the diffraction limit of the light generating the potential. The lattice consists of a one-dimensional array of ultranarrow barriers with widths less than 10 nm, well below the wavelength of the lattice light, physically realizing a Kronig-Penney potential. We study the band structure and dissipation of this lattice and find good agreement with theoretical predictions. Even on resonance, the observed lifetimes of atoms trapped in the lattice are as long as 44 ms, nearly 10^{5} times the excited state lifetime, and could be further improved with more laser intensity. The potential is readily generalizable to higher dimensions and different geometries, allowing, for example, nearly perfect box traps, narrow tunnel junctions for atomtronics applications, and dynamically generated lattices with subwavelength spacings.
We report on the experimental realization of a conservative optical lattice for cold atoms with a subwavelength spatial structure.The potential is based on the nonlinear optical response of three-level atoms in laser-dressed dark states, which is not constrained by the diffraction limit of the light generating the potential.The lattice consists of a one-dimensional array of ultranarrow barriers with widths less than 10 nm, well below the wavelength of the lattice light, physically realizing a Kronig-Penney potential.We study the band structure and dissipation of this lattice and find good agreement with theoretical predictions.Even on resonance, the observed lifetimes of atoms trapped in the lattice are as long as 44 ms, nearly 10 5 times the excited state lifetime, and could be further improved with more laser intensity.The potential is readily generalizable to higher dimensions and different geometries, allowing, for example, nearly perfect box traps, narrow tunnel junctions for atomtronics applications, and dynamically generated lattices with subwavelength spacings.
Optical lattices are typically created via the ac Stark shift and are limited by diffraction to periodicities $\ensuremath{\ge}\ensuremath{\lambda}/2$, where $\ensuremath{\lambda}$ is the wavelength of light used to create them. Lattices with smaller periodicities may be useful for many-body physics with cold atoms and can be generated by stroboscopic application of a phase-shifted lattice with subwavelength features. Here we demonstrate a $\ensuremath{\lambda}/4$-spaced lattice by stroboscopically applying optical Kronig-Penney-like potentials which are generated using spatially dependent dark states. We directly probe the periodicity of the $\ensuremath{\lambda}/4$-spaced lattice by measuring the average probability density of the atoms loaded into the ground band of the lattice. We measure lifetimes of atoms in this lattice and discuss the mechanisms that limit the applicability of this stroboscopic approach.
There has been a recent surge of interest and progress in creating subwavelength free-space optical potentials for ultracold atoms. A key open question is whether geometric potentials, which are repulsive and ubiquitous in the creation of subwavelength free-space potentials, forbid the creation of narrow traps with long lifetimes. Here, we show that it is possible to create such traps. We propose two schemes for realizing subwavelength traps and demonstrate their superiority over existing proposals. We analyze the lifetime of atoms in such traps and show that long-lived bound states are possible. This work allows for subwavelength control and manipulation of ultracold matter, with applications in quantum chemistry and quantum simulation.