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arXiv:1907.04387 · Physical Review Letters

Quantum Interference between Photons from an Atomic Ensemble and a Remote Atomic Ion

Alexander N. Craddock, John Hannegan, Dalia Ornelas-Huerta, James Siverns, Andrew J. Hachtel, Elizabeth A. Goldschmidt, J. V. Porto, Qudsia Sara Quraishi, S. L. Rolston

Published Nov 18, 2019• 37 citations
arXivHTMLPDF

Abstract

Many remote-entanglement protocols rely on the generation and interference of photons produced by nodes within a quantum network. Quantum networks based on heterogeneous nodes provide a versatile platform by utilizing the complementary strengths of the differing systems. Implementation of such networks is challenging, due to the disparate spectral and temporal characteristics of the photons generated by the different quantum systems. Here, we report on the observation of quantum interference between photons generated from a single ion and an atomic ensemble. The photons are produced on demand by each source located in separate buildings, in a manner suitable for quantum networking. Given these results, we analyze the feasibility of hybrid ion-ensemble remote entanglement generation.

DOI
10.1103/physrevlett.123.213601

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Many remote-entanglement protocols rely on the generation and interference of photons produced by nodes within a quantum network. Quantum networks based on heterogeneous nodes provide a versatile platform by utilizing the complementary strengths of the differing systems. Implementation of such networks is challenging, due to the disparate spectral and temporal characteristics of the photons generated by the different quantum systems. Here, we report on the observation of quantum interference between photons generated from a single ion and an atomic ensemble. The photons are produced on demand by each source located in separate buildings, in a manner suitable for quantum networking. Given these results, we analyze the feasibility of hybrid ion-ensemble remote entanglement generation.
Abstract Hybrid quantum systems play a crucial role in advancing scalable and versatile quantum networks as they combine the strengths of different quantum platforms. An important challenge for the development of hybrid quantum networks lies in interfacing heterogeneous quantum nodes and distributing entanglement among them. Single photons emitted from these dissimilar quantum nodes typically show distinct spectral and temporal properties. Therefore, they necessitate spectral filtering and temporal synchronization, which introduce significant photon losses and require additional resources. In this work, we successfully generate indistinguishable photons from two distinct quantum systems of a warm atomic ensemble and a solid-state quantum dot. Remarkably, quantum interference between dissimilar sources is achieved without additional spectral filtering and time synchronization, which enables autonomous quantum nodes for a hybrid quantum network. 133Cs atomic ensemble can efficiently generate heralded single photons at the wavelength of 917 nm of the 6P_(3/2)-6D_(5/2) transition, while the single photons emitted from an InAs/GaAs quantum dot can be tuned to match the 133Cs transition wavelength. Our dense warm atomic ensemble and cavity-coupled quantum dot can efficiently generate bright and resonant single photons at detection rates approaching MHz, respectively. More importantly, these single photons exhibit inherent spectral similarities not only in the wavelength but also in the spectral linewidth, achieving a high spectral overlap of 0.92. Such intrinsic compatibility between dissimilar quantum sources is essential to leverage the advantages of different quantum platforms, paving the way toward a large-scale and functional hybrid quantum network.
Different quantum systems possess different favorable qualities. On the one hand, ensemble-based quantum memories are suited for fast multiplexed long-range entanglement generation. On the other hand, single-atomic systems provide access to gates for processing of information. Both of those can provide advantages for high-rate entanglement generation within quantum networks. We develop a hybrid architecture that takes advantage of these properties by combining trapped-ion nodes and nodes comprised of spontaneous parametric down conversion photon pair sources and absorptive memories based on rare-earth ion ensembles. To this end, we solve the central challenge of matching the different bandwidths of photons emitted by those systems in an initial entanglement-generation step. This enables the parallel execution of multiple probabilistic tasks in the initial stage. As a particular example, we show that our approach can lead to a significant speed-up for the fundamental task of creating ion-ion entanglement over hundreds of kilometers in a quantum network.
Long-range quantum information processing will require the integration of different technologies to form hybrid architectures combining the strengths of multiple quantum systems. In this work, we propose a hybrid networking architecture designed to improve entanglement rates in quantum networks based on trapped ions. Trapped ions are excellent candidates as network nodes, but photon losses make long-distance networking difficult. To overcome some losses and extend the range of trapped-ion-based networks, we propose including neutral-atom-based nondestructive single-photon detection and single-photon storage in between networking nodes, forming a hybrid network. This work builds on recently demonstrated optical frequency conversion of single photons emitted by trapped ions. We derive the average two-node entanglement rate for this proposed network architecture as a function of distance. Using reasonable experimental parameters, we show that this proposed quantum network can generate remote entanglement rates up to a factor of 100 larger than that of an equivalent homogeneous network at both near-IR and C-band wavelengths for distances up to 50 km.
Irhe field of quantum information processing (QIP) has evolved rapidly in the last decade. Strings of single rapped ions have proven to be one of the most promising candidates for the implementation of quantum information processing tasks such as universal gate operations or eleportation. Besides the challenge of scaling up these quantum processors to a larger number of ions, another important problem is to interconnect different processors on a macroscopic scale and integrate them into a quantum network. Irhis thesis describes the construction of a new experiment dedicated to the study of quantum communication and quantum networking with laser cooled single ions and first experiments carried out with it. Two linear Paul traps for 4DCa+ have been set up at a distance of one meter. Two-photon interference of the fluorescence light of two remotely trapped single ions could be observed with a contrast of 80%. This proves the suitability of the setup for the creation of remote entanglement, an important building block for quantum networking. Irhe first part of the thesis describes the experimental setup that ~as constructed from scratch. It consists of a newly designed trap apparatus and the laser setup. The apparatus was designed to ulfill the requirement of interferometric stability, which is a pre requisite for one remote entanglement protocol. Another important feature are two high numerical aperture in-vacuum lenses hat optimize the collection efficiency of photons scattered by he ions. In order to frequency-stabilize the laser systems, a ransfer stabilization scheme referenced to a transition in atomic ~s has been developed. The stabilization chain comprises low-cost open transfer cavities and offers very good long term stability. Irhe second part of the thesis presents the experimental results starting with the calibration of the two traps through excitation spectra. After that, the realization of two-photon interference rom single ions under continuous excitation is presented. The model analysis of the data usinq eiqht level Bloch equations reveals the individual coherence properties of the interfering ~ingle photons. The coherence time of the fluorescence light does not exceed 20- ns, indicating that incoherent scattering is ~ominant. fA,n analysis of the efficiency of methods for remote entanglement relying on two-photon and single-photon interference, focussing on he role of the detection efficiency is discussed. It is revealed hat Single-photon schemes are more efficient if the detection ~fficiency is low (like in present experiments). The created setup is suitable for the realization of both types of protocols, based pn single- and two-photon interference. Jhe conditioned dynamics of photon emission of a single ion are studied using correlation functions. The engineering of second ~rder correlation functions used as a tool which relies on conditional dynamics, might have interesting applications in probabilistic quantum information processing. pingle-atom single-photon interfaces are an important application in quantum networks. As opposed to the emission of single photons by single atoms, the absorption of Single photons by single atoms cannot be controlled in a similar way. With the future goal of realizing a heralded absorption of a single photon by a single atom, one of the ion traps was linked to a Spontaneous Parametric Down Conversion source. Quantum jump spectroscopy on a single ion using single photons from this source is shown. Finally the reported two-photon interference could be extended also to pulsed excitation. This marks an important technological step towards remote entanglement.
Establishing quantum entanglement between individual nodes is crucial for building large-scale quantum networks, enabling secure quantum communications, distributed quantum computing, enhanced quantum metrology, and fundamental tests of quantum mechanics. However, the shared entanglements have been merely observed in either extremely low-temperature or well-isolated systems, which limits quantum networks for real-life applications. Here, we report the realization of heralding quantum entanglement between two atomic ensembles at room temperature, which are contained in two spatially separated, centimeter-sized vapor cells. By mapping the atomic state onto a photonic state after the readout process, we measure the quantum interference of the Raman-scattered photons and reconstruct the entangled state, then we strongly verify the existence of a single excitation delocalized in two atomic ensembles. The demonstrated building block paves the way to construct quantum networks and distributing entanglement across multiple remote nodes at ambient conditions.
Increasing the number of qubits that can be controlled in a quantum system represents an essential challenge to the field of quantum computing. Quantum networks consisting of nodes for local information processing and photonic channels to distribute entanglement between different nodes represent a promising modular approach to achieve this scaling. Trapped atomic ions are an ideal candidate for quantum network nodes, with long-lived identical qubit memories that can be locally entangled through their Coulomb interaction and remotely entangled through photonic channels. In this work I will first discuss our established toolkit for using 171Yb+ and 138Ba+ ions individually or together within a quantum node. Next I will show how the 138Ba+ toolkit has been extended to allow for quantum operations in the 52D3/2 manifold. I will then demonstrate how we can generate ion-photon entanglement as a resource to connect separate nodes with a focus on some important improvements which will allow us to implement it as part of a larger network. These improvements include first the use of separate memory (171Yb+ ) and photon generating (138Ba+ ) ions. Additionally, the use of separate atomic lines within 138Ba+ for excitation and collection allows us to preserve integrity of this photonic interface by ensuring the purity of the single photons that are produced. To this end I demonstrate a single-photon source for quantum networking based on a trapped 138Ba+ ion with a single photon purity of g2(0) = (8.1 ± 2.3) × 10−5 without background subtraction. Trade-offs between the photonic generation rate and the memory-photon entanglement fidelity for the case of polarization photonic qubits are also examined and optimized by tailoring the spatial mode of the collected light. These techniques should be useful in constructing larger ion-photon networks.