Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1906.08123 · Journal of Physics B Atomic Molecular and Optical Physics

Resonant single-photon double ionization driven by combined intra- and interatomic electron correlations

A Eckey, A B Voitkiv, C Müller

Published Nov 29, 2019• 9 citations
arXivHTMLPDF

Abstract

Abstract The double ionization of an atom by single-photon absorption in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom, leading to its double ionization. The process relies on the combined effect of interatomic and intra-atomic electron correlations. It can dominate over the direct double photoionization by several orders of magnitude at interatomic distances up to a few nanometers. The relative position of the neighbouring atom is shown to exert a characteristic influence on the angular distribution of emitted electrons.

DOI
10.1088/1361-6455/ab5d91

Related papers

Two-center resonant photoionization-excitation driven by combined intra- and interatomic electron correlations

S Kim, S Steinhäuser, Alexander B Voitkiv +1 more

Abstract Ionization-excitation of an atom induced by the absorption of a single photon in the presence of a neighboring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom, leading to its ionization with simultaneous excitation. The process relies on the combined effects of interatomic and intraatomic electron correlations. Under suitable conditions, it can dominate by several orders of magnitude over direct photoionization-excitation and even over direct photoionization. In addition, we briefly discuss another kind of two-center resonant photoionization with excitation where the ionization and residual excitation in the final state are located at different atomic sites.

arXiv:2309.01143•Journal of Physics B Atomic Molecular and Optical Physics•Jan 30, 2024•0 citations

Resonantly enhanced photoionization in correlated three-atomic systems

Bennaceur Najjari, Müller, C., Voitkiv, A.

Modifications of photoionization arising from resonant electron-electron correlations between neighbouring atoms in an atomic sample are studied. The sample contains atomic species A and B, with the ionization potential of A being smaller than the energy of a dipole-allowed transition in B. The atoms are subject to an external radiation field which is near-resonant with the dipole transition in B. Photoionization of an atom A may thus proceed via a two-step mechanism: photoexcitation in the subsystem of species B, followed by interatomic Coulombic decay. As a basic atomic configuration, we investigate resonant photoionization in a three-atomic system A-B-B, consisting of an atom A and two neighbouring atoms B. It is found that, under suitable conditions, the influence of the neighbouring atoms can strongly affect the photoionization process, including its total probabilty, time development and photoelectron spectra. In particular, by comparing our results with those for photoionization of an isolated atom A and a two-atomic system A-B, respectively, we reveal the characteristic impact exerted by the third atom.

•Oct 29, 2012•7 citations

Strong-field photoionization in two-center atomic systems

Jacqueline Fedyk, Alexander B Voitkiv, Carsten Müller

Photoionization of an atom $A$ by a strong laser field in the presence of a spatially well-separated neighboring atom $B$ is considered. The laser field frequency is assumed to lie below the ionization potential of atom $A$ and be resonant with a dipole-allowed transition in atom $B$. In this situation, the ionization may occur either directly by multiphoton absorption from the laser field at the first atomic center or via an indirect pathway involving two-center electron-electron correlations, where the neighbor atom $B$ is first photoexcited and, afterwards, transfers its energy upon deexcitation radiationlessly to atom $A$. Considering monochromatic as well as bichromatic laser fields, we study various coupling regimes of the photoionization process and identify experimentally accessible parameter domains where the two-center channel is dominant.

arXiv:1807.09650•Physical Review A•Sep 27, 2018•2 citations

Resonantly enhanced photoionization in correlated three-atomic systems

Bennaceur Najjari, C Müller, A B Voitkiv

Modifications of photoionization arising from resonant electron–electron correlations between neighbouring atoms in an atomic sample are studied. The sample contains atomic species A and B , with the ionization potential of A being smaller than the energy of a dipole-allowed transition in B . The atoms are subject to an external radiation field which is near resonant with the dipole transition in B . Photoionization of an atom A may thus proceed via a two-step mechanism: photoexcitation in the subsystem of species B , followed by interatomic Coulombic decay. As a basic atomic configuration, we investigate resonant photoionization in a three-atomic system A – B – B consisting of an atom A and two neighbouring atoms B . It is found that, under suitable conditions, the presence of neighbouring atoms can strongly affect the photoionization process, including its total probability, time development and photoelectron spectra. In particular, comparing our results with those for photoionization of an isolated atom A and a two-atomic system A – B , respectively, we reveal the characteristic impact made by the third atom.

arXiv:1203.2038•New Journal of Physics•Oct 29, 2012•8 citations

Resonant Two-Photon Single Ionization of Two Identical Atoms

Carsten Müller, Alexander B Voitkiv

Resonant two-photon single ionization in a system consisting of two spatially well-separated identical atoms is studied. Because of two-center electron-electron correlations, the ionization may also proceed through photoexcitation of both atoms with subsequent interatomic Coulombic decay. We show that this channel may qualitatively change the dependence of the photoionization on the field intensity as well as the spectra of emitted electrons.

arXiv:1102.5677•Physical Review Letters•Jun 27, 2011•14 citations

Dynamic two-center resonant photoionization in slow atomic collisions

Alexander B Voitkiv, C Müller, S F Zhang +1 more

Abstract An additional channel for photoionization of an atom A by an electromagnetic field opens if it interacts with an atom B resonantly coupled to this field. In this channel, which is known to be very efficient when A and B constitute a bound system, A is ionized via resonant photoexcitation of B with subsequent energy transfer to A through two-center electron correlations. We show that it can strongly dominate the ionization of A also in collisions with B, even though the average distance between A and B exceeds the typical size of a bound system by orders of magnitude.

arXiv:1809.06526•New Journal of Physics•Sep 19, 2019•8 citations
Abstract The double ionization of an atom by single-photon absorption in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom, leading to its double ionization. The process relies on the combined effect of interatomic and intra-atomic electron correlations. It can dominate over the direct double photoionization by several orders of magnitude at interatomic distances up to a few nanometers. The relative position of the neighbouring atom is shown to exert a characteristic influence on the angular distribution of emitted electrons.
Abstract Ionization-excitation of an atom induced by the absorption of a single photon in the presence of a neighboring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom, leading to its ionization with simultaneous excitation. The process relies on the combined effects of interatomic and intraatomic electron correlations. Under suitable conditions, it can dominate by several orders of magnitude over direct photoionization-excitation and even over direct photoionization. In addition, we briefly discuss another kind of two-center resonant photoionization with excitation where the ionization and residual excitation in the final state are located at different atomic sites.
Modifications of photoionization arising from resonant electron-electron correlations between neighbouring atoms in an atomic sample are studied. The sample contains atomic species A and B, with the ionization potential of A being smaller than the energy of a dipole-allowed transition in B. The atoms are subject to an external radiation field which is near-resonant with the dipole transition in B. Photoionization of an atom A may thus proceed via a two-step mechanism: photoexcitation in the subsystem of species B, followed by interatomic Coulombic decay. As a basic atomic configuration, we investigate resonant photoionization in a three-atomic system A-B-B, consisting of an atom A and two neighbouring atoms B. It is found that, under suitable conditions, the influence of the neighbouring atoms can strongly affect the photoionization process, including its total probabilty, time development and photoelectron spectra. In particular, by comparing our results with those for photoionization of an isolated atom A and a two-atomic system A-B, respectively, we reveal the characteristic impact exerted by the third atom.
Photoionization of an atom AAA by a strong laser field in the presence of a spatially well-separated neighboring atom BBB is considered. The laser field frequency is assumed to lie below the ionization potential of atom AAA and be resonant with a dipole-allowed transition in atom BBB. In this situation, the ionization may occur either directly by multiphoton absorption from the laser field at the first atomic center or via an indirect pathway involving two-center electron-electron correlations, where the neighbor atom BBB is first photoexcited and, afterwards, transfers its energy upon deexcitation radiationlessly to atom AAA. Considering monochromatic as well as bichromatic laser fields, we study various coupling regimes of the photoionization process and identify experimentally accessible parameter domains where the two-center channel is dominant.
Modifications of photoionization arising from resonant electron–electron correlations between neighbouring atoms in an atomic sample are studied. The sample contains atomic species A and B , with the ionization potential of A being smaller than the energy of a dipole-allowed transition in B . The atoms are subject to an external radiation field which is near resonant with the dipole transition in B . Photoionization of an atom A may thus proceed via a two-step mechanism: photoexcitation in the subsystem of species B , followed by interatomic Coulombic decay. As a basic atomic configuration, we investigate resonant photoionization in a three-atomic system A – B – B consisting of an atom A and two neighbouring atoms B . It is found that, under suitable conditions, the presence of neighbouring atoms can strongly affect the photoionization process, including its total probability, time development and photoelectron spectra. In particular, comparing our results with those for photoionization of an isolated atom A and a two-atomic system A – B , respectively, we reveal the characteristic impact made by the third atom.
Abstract An additional channel for photoionization of an atom A by an electromagnetic field opens if it interacts with an atom B resonantly coupled to this field. In this channel, which is known to be very efficient when A and B constitute a bound system, A is ionized via resonant photoexcitation of B with subsequent energy transfer to A through two-center electron correlations. We show that it can strongly dominate the ionization of A also in collisions with B, even though the average distance between A and B exceeds the typical size of a bound system by orders of magnitude.