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arXiv:1906.03933 · Physical Review A

Dissipative quantum state preparation and metastability in two-photon micromasers

Andreas Kouzelis, Katarzyna Macieszczak, Jiří Minář, Igor Lesanovsky

Published Apr 29, 2020• 11 citations
arXivHTMLPDF

Abstract

We study the preparation of coherent quantum states in a two-photon micromaser for applications in quantum metrology. While this setting can be in principle realized in a host of physical systems, we consider atoms interacting with the field of a cavity. We focus on the case of the interaction described by the Jaynes-Cummings Hamiltonian, which cannot be achieved by the conventional approach with three-level atoms coupled to the cavity field at two-photon resonance. We find that additional levels are required in order to cancel Stark shifts emerging in the leading order. Once this is accomplished, the dynamics of the cavity features a degenerate stationary state manifold of pure states. We derive the analytic form of these states and show that they include Schr\"odinger cat states with a tunable mean photon number. We also confirm these states can be useful in phase estimation protocols with their quantum Fisher information exceeding the standard limit. To account for realistic imperfections, we consider single-photon losses from the cavity, finite lifetime of atom levels, and higher order corrections in the far-detuned limit, which result in metastability of formerly stationary cavity states and long-time dynamics with a unique mixed stationary state. Despite being mixed, this stationary state can still feature quantum Fisher information above the standard limit. Our work delivers a comprehensive overview of the two-photon micromaser dynamics with particular focus on application in phase estimation and, while we consider the setup with atoms coupled to a cavity, the results can be directly translated to optomechanical systems.

DOI
10.1103/physreva.101.043847

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Non-classical states in light-matter interactions.

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In this thesis we investigate the possibilities to create non-classical states by using light-matter interactions. Our basic approach to describe these interactions is the Jaynes-Cummings model. It describes interactions between a two-level atom and a quantized field in a lossless cavity (ultra high Q quality factor). The model can be easily generalized to describe multi-level atoms, Stark shifts, Kerr interactions, micromasers, etc. We use some of these generalizations in our study. Our main interest is in the production of Schrodinger cat states, that is, the coherent superposition of two or more classical macroscopic states; and the production of sub-Poissonian photostatistics. First of all, we use the simple Jaynes-Cummings model to investigate the interaction of coherent states with two-level atoms, and compare it to the case of interaction with a statistical mixture to show that we can discern between the two. We investigate as well the interaction of two level atoms and squeezed light, where we show that these states have a strong coherent character. However, the model itself is very simple, and as we have said before, some generalizations are necessary if we are to describe more realistically the atom field interactions. In particular, we use a phenomenological Hamiltonian, which incorporates Stark shifts in the atomic levels due to the electric field in the cavity, and show that some experimental results concerning the lineshapes in micromasers may be explained by such effects. Another step is to allow the atoms to enter and leave the cavity, which leads us to investigate a micromaser system. Within this structure, we allow for one- and two-photon transitions. In the latter case, it is shown that sub-Poissonian fields (by using special atom-field interaction times) and multi Schrodinger cat states (by measuring the state of the atoms as they leave the cavity) can be generated.

•Jan 1, 1993•0 citations
We study the preparation of coherent quantum states in a two-photon micromaser for applications in quantum metrology. While this setting can be in principle realized in a host of physical systems, we consider atoms interacting with the field of a cavity. We focus on the case of the interaction described by the Jaynes-Cummings Hamiltonian, which cannot be achieved by the conventional approach with three-level atoms coupled to the cavity field at two-photon resonance. We find that additional levels are required in order to cancel Stark shifts emerging in the leading order. Once this is accomplished, the dynamics of the cavity features a degenerate stationary state manifold of pure states. We derive the analytic form of these states and show that they include Schr"odinger cat states with a tunable mean photon number. We also confirm these states can be useful in phase estimation protocols with their quantum Fisher information exceeding the standard limit. To account for realistic imperfections, we consider single-photon losses from the cavity, finite lifetime of atom levels, and higher order corrections in the far-detuned limit, which result in metastability of formerly stationary cavity states and long-time dynamics with a unique mixed stationary state. Despite being mixed, this stationary state can still feature quantum Fisher information above the standard limit. Our work delivers a comprehensive overview of the two-photon micromaser dynamics with particular focus on application in phase estimation and, while we consider the setup with atoms coupled to a cavity, the results can be directly translated to optomechanical systems.
We study the dynamics of a two-photon micromaser driven by a sequence of polarized Rydberg atoms. If cavity losses are neglected, the density matrix of the cavity mode consists of four dynamically decoupled components. Under appropriate trapping conditions, similar to those for the one-photon micromaser, it evolves to a stationary state. When the bare two-photon frequency cancels the ac Stark shift we cannot satisfy the trapping conditions for odd and even photon number states simultaneously. For specific initial conditions, where either only odd or only even number states are initially populated, we may find, however, stationary states that are pure and that can lead to macroscopic superpositions. These pure states are analogous to the cotangent and tangent states of the one-photon micromaser. When the two atomic levels are in resonance with the bare two-photon transition, trapping conditions for odd and even photon number states can be fulfilled simultaneously. Although the ac Stark shift does not allow for pure stationary states, the stationary state resembles an incoherent superposition of only two pure states, to within a relative deviation of 10-3 off purity.
A single beam of excited two-level atoms couples two micromasers in a series. It is shown that in the absence of dissipation the possible steady states of their fields are superpositions, of two-field trapping number states. Which one is realized depends upon the initial state of the fields and the interaction parameters, g'\ensuremath{\tau}' and g''\ensuremath{\tau}'', of the two cavities. A large number of these trapping states are pure quantum states, some of them showing entanglement of the two nonlocal micromaser fields of the form \ensuremath{\Vert}N,N+M〉\ifmmode\pm\else\textpm\fi{}\ensuremath{\Vert}N+M,N〉. Here, N and N+M are arbitrary trapping numbers that belong to disconnected blocks of the photon number space and M specifies the order of correlation between the fields. The time evolution of the system toward steady states is investigated numerically, mainly concentrating on the production of pure entangled trapping states of the form discussed earlier. We describe a special procedure to amplify a number state, \ensuremath{\Vert}N,N〉, into such states that is based on conditions regarding the interaction parameters. In principle, N and M can be made arbitrarily large resulting in a steady-state nonlocal quantum superposition of distinct macroscopical fields (nonlocal ``Schr\"odinger cat''). We also present a solution of the standard master equation of a damped harmonic oscillator at finite temperature and apply it to study the effect of dissipation on the production of entangled trapping states at regular and Poissonian pump statistics.It is found that although the entanglement does not survive at a steady state it can build up in the short-time transient regime when cavity losses and the number of thermal photons are not too large. In this small-loss (large Nex{\mathit{N}}_{\mathrm{ex}}Nex​) regime the quantum correlation between the micromaser fields decays into a steady-state classical superposition at a rate that depends on the cavity lifetime and the difference (or order of correlation), M, between the superposed photon numbers. In the large-loss (small Nex{\mathit{N}}_{\mathrm{ex}}Nex​) regime, however, no transient correlation can be produced and the photon statistics spreads out towards a vacuum for increasing losses. The system undergoes a transition from an uncorrelated to a correlated behavior when the pumping parametrized by Nex{\mathit{N}}_{\mathrm{ex}}Nex​ exceeds the threshold between the large- and small-loss regimes. Thermal photons enhance the decay of the correlation and by coupling the disconnected blocks of the photon number space they populate the trapping number states of adjacent blocks. However, it is shown that the production of transient entanglement is not significantly affected by either thermal radiation or pumping fluctuations. The experimental realization of the entanglement of nonlocal micromaser fields employing these two-field trapping states of small photon numbers is shown to be feasible in the short-time transient regime using the presently available high-Q cavities and low temperatures, and could be possible on the macroscopic scale in the near future.
In this work, we investigate the dissipative generation of metrologically useful steady states in a generalized atom-cavity system that incorporates two-photon exchange, diamagnetic interactions, and auxiliary nonlinearities inherent to superconducting circuits. By quantifying the normalized Quantum Fisher Information (QFI), we demonstrate that the interplay between coherent driving and Kerr–Stark anharmonicity allows for the autonomous preparation of states that surpass the Standard Quantum Limit (SQL). Our results reveal that unlike simple Gaussian squeezing, the introduction of realistic nonlinearities induces non-Gaussian phase-space distortions, accompanied by small but finite Wigner negativity, that maximise the information content for photon-number encoding while maintaining a mean photon number below unity throughout. The Mandel Q M parameter is found to exceed the thermal-state reference 〈 n ^ 〉 across all dynamical regimes and coupling strengths, providing a stringent quantitative demonstration that the observed super-Poissonian statistics originate from non-classical correlations rather than thermal fluctuations. Crucially, a rigorous spectral decomposition of the Liouvillian superoperator confirms that these high-sensitivity regimes are protected by a finite spectral gap, precluding critical slowing down and ensuring that state preparation occurs on timescales significantly shorter than typical qubit decoherence times. These findings establish a viable blueprint for engineering always-on quantum sensors that are both metrologically superior and dynamically robust.
An approximate solution is given for the Jaynes-Cummings model with cavity losses, i.e., the problem of a two-level atom interacting with a single mode of the quantized radiation field, in the rotating-wave approximation, when the field is damped by a reservoir at zero temperature. The approximate solution is derived for initial coherent field states with moderately large numbers of photons. It is simpler in form than earlier results derived by other authors and, over the appropriate parameter range, substantially more accurate than some of them, as shown by direct numerical integration of the master equation. In particular, it is found that an earlier treatment of this problem based on a secular approximation is seriously flawed, in that the conditions for its validity are much more restrictive than was previously believed. Among the results derived it is shown that, just as for the lossless case, when the atom is initially prepared in one of the semiclassical eigenstates the evolution is very simple, with the field and the atomic dipole drifting together in phase. For moderate losses this leads, as in the lossless case, to a ``state preparation''; i.e., to a good approximation, the state of the atom at a specific time can be made independent of its initial state. The effect of losses on the recently discovered ``Schr\"odinger cat'' state of the field is also analyzed. It is found that, although the dissipation destroys the coherence of the macroscopic superposition very rapidly, preparation and observation of the ``cat'' should be possible with the cavity quality factors reported in recent micromaser experiments.
In this thesis we investigate the possibilities to create non-classical states by using light-matter interactions. Our basic approach to describe these interactions is the Jaynes-Cummings model. It describes interactions between a two-level atom and a quantized field in a lossless cavity (ultra high Q quality factor). The model can be easily generalized to describe multi-level atoms, Stark shifts, Kerr interactions, micromasers, etc. We use some of these generalizations in our study. Our main interest is in the production of Schrodinger cat states, that is, the coherent superposition of two or more classical macroscopic states; and the production of sub-Poissonian photostatistics. First of all, we use the simple Jaynes-Cummings model to investigate the interaction of coherent states with two-level atoms, and compare it to the case of interaction with a statistical mixture to show that we can discern between the two. We investigate as well the interaction of two level atoms and squeezed light, where we show that these states have a strong coherent character. However, the model itself is very simple, and as we have said before, some generalizations are necessary if we are to describe more realistically the atom field interactions. In particular, we use a phenomenological Hamiltonian, which incorporates Stark shifts in the atomic levels due to the electric field in the cavity, and show that some experimental results concerning the lineshapes in micromasers may be explained by such effects. Another step is to allow the atoms to enter and leave the cavity, which leads us to investigate a micromaser system. Within this structure, we allow for one- and two-photon transitions. In the latter case, it is shown that sub-Poissonian fields (by using special atom-field interaction times) and multi Schrodinger cat states (by measuring the state of the atoms as they leave the cavity) can be generated.