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arXiv:1904.13393 · Applied Sciences

Investigations on Dynamical Stability in 3D Quadrupole Ion Traps

Bogdan M. Mihalcea, Stephen Lynch

Published Mar 25, 2021• 16 citations
arXivHTMLPDF

Abstract

We firstly discuss classical stability for a dynamical system of two ions levitated in a 3D Radio-Frequency (RF) trap, assimilated with two coupled oscillators. We obtain the solutions of the coupled system of equations that characterizes the associated dynamics. In addition, we supply the modes of oscillation and demonstrate the weak coupling condition is inappropriate in practice, while for collective modes of motion (and strong coupling) only a peak of the mass can be detected. Phase portraits and power spectra are employed to illustrate how the trajectory executes quasiperiodic motion on the surface of torus, namely a Kolmogorov-Arnold-Moser (KAM) torus. In an attempt to better describe dynamical stability of the system, we introduce a model that characterizes dynamical stability and the critical points based on the Hessian matrix approach. The model is then applied to investigate quantum dynamics for many-body systems consisting of identical ions, levitated in 2D and 3D ion traps. Finally, the same model is applied to the case of a combined 3D Quadrupole Ion Trap (QIT) with axial symmetry, for which we obtain the associated Hamilton function. The ion distribution can be described by means of numerical modeling, based on the Hamilton function we assign to the system. The approach we introduce is effective to infer the parameters of distinct types of traps by applying a unitary and coherent method, and especially for identifying equilibrium configurations, of large interest for ion crystals or quantum logic.

DOI
10.3390/app11072938

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Spectral properties of the Hamiltonian function which characterizes a trapped ion are investigated. In order to study semiclassical dynamics of trapped ions, coherent state orbits are introduced as sub-manifolds of the quantum state space, with the Kähler structure induced by the transition probability. The time dependent variational principle (TDVP) is applied on coherent states' orbits. The Hamilton equations of motion on Kähler manifolds of the type of classical phase spaces naturally arise. The associated classical Hamiltonian is obtained from the expected values on symplectic coherent states of the quantum Hamiltonian. Spectral information is thus coded within the phase portrait. We deal with the bosonic realization of the Lie algebra of the SU(1,1) group, which we particularize for the case of an ion confined in a combined, Paul and Penning trap. This formalism can be applied to Hamiltonians which are nonlinear in the infinitesimal generators of a dynamical symmetry group, such as the case of ions confined in electrodynamic traps. Discrete quasienergy spectra are obtained and the corresponding quasienergy states are explicitly realized as coherent states parameterized by the stable solutions of the corresponding classical equations of motion. A correspondence between quantum and classical stability domains is thus established, using the Husimi representation.

arXiv:1107.0856•Jul 5, 2011•1 citation
We firstly discuss classical stability for a dynamical system of two ions levitated in a 3D Radio-Frequency (RF) trap, assimilated with two coupled oscillators. We obtain the solutions of the coupled system of equations that characterizes the associated dynamics. In addition, we supply the modes of oscillation and demonstrate the weak coupling condition is inappropriate in practice, while for collective modes of motion (and strong coupling) only a peak of the mass can be detected. Phase portraits and power spectra are employed to illustrate how the trajectory executes quasiperiodic motion on the surface of torus, namely a Kolmogorov-Arnold-Moser (KAM) torus. In an attempt to better describe dynamical stability of the system, we introduce a model that characterizes dynamical stability and the critical points based on the Hessian matrix approach. The model is then applied to investigate quantum dynamics for many-body systems consisting of identical ions, levitated in 2D and 3D ion traps. Finally, the same model is applied to the case of a combined 3D Quadrupole Ion Trap (QIT) with axial symmetry, for which we obtain the associated Hamilton function. The ion distribution can be described by means of numerical modeling, based on the Hamilton function we assign to the system. The approach we introduce is effective to infer the parameters of distinct types of traps by applying a unitary and coherent method, and especially for identifying equilibrium configurations, of large interest for ion crystals or quantum logic.
Quasiclassical dynamics of trapped ions is described by applying the time dependent variational principle (TDVP) on coherent state orbits, introduced as sub-manifolds of the quantum state space. The classical Hamilton functions associated to the system are obtained as the expected values of the quantum Hamiltonian on symplectic coherent states. Such formalism can be applied to Hamilton functions which are nonlinear in the infinitesimal generators of a dynamical symmetry group. We give the explicit expression of the quantum Hamilton function in case of nonlinear electromagnetic traps. Discrete quasienergy spectra result, and the corresponding quasienergy states are explicitly realized as coherent states parameterized by the stable solutions of the corresponding classical equations of motion. A dequantization algorithm is also suggested. The method is then applied to combined (Paul and Penning) and ideal Paul traps. We obtain the explicit expressions of the classical Hamilton functions for such particular traps, as well as the classical Hamilton equations of motion in complex coordinates for an octupole trap. In the pseudopotential approximation, the points of minimum of the Hamiton function define equilibrium configurations for trapped ions, of interest for quantum logic.
"We investigate quantum dynamics for an ion confined within an oscillating quadrupole field, starting from two well known and elegant approaches. It is established that the Hamilton equations of motion, in both Schrodinger and Heisenberg representations, are equivalent to the Hill equation. One searches for a linear independent solution associated to a harmonic oscillator (HO). An adiabatic invariant, which is also a constant of motion, is introduced based on the Heisenberg representation. Thus, the state of the non-autonomous system can be determined at any subsequent moment of time. The quantum states for trapped ions are demonstrated to be Fock (number) states, while the exact solutions of the Schrodinger equation for a trapped ion are exactly the quasienergy states. Semiclassical dynamics is also investigated for many-body systems of trapped ions, where the wavefunction associated to the Schrodinger equation is prepared as a Gauss package multiplied by a Hermite polynomial. We also discuss time evolution for the system under investigation and supply the propagator."
A two-ion pair in a linear Paul trap is extensively used in the research of the simplest quantum-logic system; however, there are few quantitative and comprehensive studies on the motional mode coupling of two-ion systems yet. This study proposes a method to investigate the motional mode coupling of sympathetically cooled two-ion crystals by quantifying three-dimensional (3D) secular spectra of trapped ions using molecular dynamics simulations. The 3D resonance peaks of the 40Ca+–27Al+ pair obtained by using this method were in good agreement with the 3D in- and out-of-phase modes predicted by the mode coupling theory for two ions in equilibrium and the frequency matching errors were lower than 2%. The obtained and predicted amplitudes of these modes were also qualitatively similar. It was observed that the strength of the sympathetic interaction of the 40Ca+–27Al+ pair was primarily determined by its axial in-phase coupling. In addition, the frequencies and amplitudes of the ion pair’s resonance modes (in all dimensions) were sensitive to the relative masses of the ion pair, and a decrease in the mass mismatch enhanced the sympathetic cooling rates. The sympathetic interactions of the 40Ca+–27Al+ pair were slightly weaker than those of the 24Mg+–27Al+ pair, but significantly stronger than those of 9Be+–27Al+. However, the Doppler cooling limit temperature of 40Ca+ is comparable to that of 9Be+ but lower than approximately half of that of 24Mg+. Furthermore, laser cooling systems for 40Ca+ are more reliable than those for 24Mg+ and 9Be+. Therefore, 40Ca+ is probably the best laser-cooled ion for sympathetic cooling and quantum-logic operations of 27Al+ and has particularly more notable comprehensive advantages in the development of high reliability, compact, and transportable 27Al+ optical clocks. This methodology may be extended to multi-ion systems, and it will greatly aid efforts to control the dynamic behaviors of sympathetic cooling as well as the development of low-heating-rate quantum logic clocks.
We use the results of a Lagrangian formulation of the dynamics of ions in a Penning trap to calculate the motional frequencies of the ions as a function of the trapping parameters. We then add realistic perturbations to the ideal trapping fields in the formalism and deduce the effects of these perturbations on the ion motion. For an ideal trap there exist values of the applied trapping fields that result in a degeneracy in the ion oscillation frequencies associated with different types of motion. We show that this motional frequency degeneracy is lifted by the inclusion of the effect of a tilt of the trap axis with respect to the axis of the applied magnetic field, leading to an ``avoided crossing'' between the oscillation frequencies. We calculate typical ion orbits for trap parameters that give oscillation frequencies near the avoided crossing between the axial and modified cyclotron frequencies. We generalize the analysis to include the motion of ions in a combined (Penning-Paul) trap and perform an experiment to test the predictions of the theory for a degeneracy between the modified cyclotron frequency and the axial frequency for Mg+{\mathrm{Mg}}^{+}Mg+ ions held in a tilted combined trap. The oscillation frequencies are measured for a range of tilt angles using a photon-photon correlation technique. There is good agreement between the experimental results and the theoretical predictions. The method we describe may prove to be a useful means by which trap imperfections can be identified and subsequently removed.
When ions of slightly different mass and the same charge are stored in a radio-frequency electric quadrupole trap, a collective oscillation is observed rather than the independent motions usually assumed. A high-temperature model of ion clouds, each characterized by ions of one mass, shows that the ions of each cloud move as a unit and exhibit a correlated motion with the other clouds when a strong coupling condition is satisfied. This phenomenon is expected to arise whenever more than one ion is trapped and might be observable in neutral atom traps as well.
Spectral properties of the Hamiltonian function which characterizes a trapped ion are investigated. In order to study semiclassical dynamics of trapped ions, coherent state orbits are introduced as sub-manifolds of the quantum state space, with the Kähler structure induced by the transition probability. The time dependent variational principle (TDVP) is applied on coherent states' orbits. The Hamilton equations of motion on Kähler manifolds of the type of classical phase spaces naturally arise. The associated classical Hamiltonian is obtained from the expected values on symplectic coherent states of the quantum Hamiltonian. Spectral information is thus coded within the phase portrait. We deal with the bosonic realization of the Lie algebra of the SU(1,1) group, which we particularize for the case of an ion confined in a combined, Paul and Penning trap. This formalism can be applied to Hamiltonians which are nonlinear in the infinitesimal generators of a dynamical symmetry group, such as the case of ions confined in electrodynamic traps. Discrete quasienergy spectra are obtained and the corresponding quasienergy states are explicitly realized as coherent states parameterized by the stable solutions of the corresponding classical equations of motion. A correspondence between quantum and classical stability domains is thus established, using the Husimi representation.