Confining particles in hollow-core photonic crystal fibers has opened up new prospects to scale up the distance and time over which particles can be made to interact with light. However, maintaining long-lived quantum spin coherence and/or transporting it over macroscopic distances in a waveguide remain challenging. Here, we demonstrate coherent guiding of ground-state superpositions of ^{85}Rb atoms over a centimeter range and hundreds of milliseconds inside a hollow-core photonic crystal fiber. The decoherence is mainly due to dephasing from the residual differential light shift from the optical trap and the inhomogeneity of an ambient magnetic field. Our experiment establishes an important step towards a versatile platform that can lead to applications in quantum information networks and a matter wave circuit for quantum sensing.
Confining particles in hollow-core photonic crystal fibers has opened up new prospects to scale up the distance and time over which particles can be made to interact with light. However, maintaining long-lived quantum spin coherence and/or transporting it over macroscopic distances in a waveguide remain challenging. Here, we demonstrate coherent guiding of ground-state superpositions of ^{85}Rb atoms over a centimeter range and hundreds of milliseconds inside a hollow-core photonic crystal fiber. The decoherence is mainly due to dephasing from the residual differential light shift from the optical trap and the inhomogeneity of an ambient magnetic field. Our experiment establishes an important step towards a versatile platform that can lead to applications in quantum information networks and a matter wave circuit for quantum sensing.
Cold atoms confined inside a hollow core photonic crystal fiber with core diameter of a few photon wavelengths are a promising medium for studying nonlinear optical interactions at extremely low light levels. The high electric field intensity per photon, large optical depths, and interaction lengths not limited by diffraction are some of the unique features of this system. We describe recent progress in our experiment that uses a combination of magnetic trapping and a red-detuned optical dipole trap to transfer cold rubidium atoms into the hollow-core fiber. We present data on transfer efficiencies as well as preliminary experiments towards nonlinear optics with few photon pulses.
Recent demonstrations of light-matter interactions with atoms and molecules confined to hollow waveguides offer great promise for ultralow-light-level applications. The use of waveguides allows for tight optical confinement over interaction lengths much greater than what could be achieved in bulk geometries. However, the combination of strong atom-photon interactions and nonuniformity of guided light modes gives rise to spectroscopic features that must be understood in order to take full advantage of the properties of such systems. We use light-induced atomic desorption to generate an optically dense Rb vapor at room temperature inside a hollow-core photonic band-gap fiber. Saturable-absorption spectroscopy and passive slow-light experiments reveal large ac Stark shifts, power broadening, and transit-time broadening, that are present in this system even at nanowatt powers.
Our goal is to study quantum optical phenomena in a strong nonlinear optical system. For this purpose, we create a hollow-core photonic-crystal (HCPC) fiber-based platform that confines photons and atomic ensembles together. This enables strong light-matter interactions which are crucial for implementing optical nonlinearities at single-photon levels [1]. We use an optical dipole trap at cesium's magic wavelength to guide laser cooled cesium atoms into and inside the fiber core. This approach will allow us to perform experiments with the dipole trap continuously on as opposed to the previously reported fiber-loading systems [2,3] in which the dipole trap was rapidly amplitude-modulated to avoid the effect from the spatially dependent AC Stark shift. In this system, we perform experiments on electromagnetically induced transparency (EIT) and demonstrate slow light and all optical switch. We also aim to observe large cross-phase modulation (XPM) using a three-level ladder scheme [4,5]. Lastly, the approaches to integrate a cavity into HCPCFs to increase light-matter interactions, thus the optical nonlinearities, will be described.
Coherent manipulation and interaction between atoms and light are the core ingredients in modern quantum science and technology. Various applications such as quantum computation, quantum memories and quantum sensors which are promising in future technologies, are currently under exploration. However, due to the diffraction nature of light, miniaturizing quantum systems involving atom-light interactions has been highly limited. To avoid diffraction, I load cold atoms into a hollow-core fiber (HCF) and demonstrate four major experiments inside the fiber: inertia-sensitive Mach-Zehnder atom interferometer, long-lived quantum spin coherence, light storage and creation of an array of Schr\"odinger cat states. In this thesis, I show the theoretical framework of each experiment and demonstrate experimentally a cold atoms quantum laboratory realized a HCF. Cold 85Rb atoms of temperature ∼\SI{6}{\micro\kelvin} are loaded into a Kagome type photonic crystal hollow-core fiber (HCF) through an optical trapping beam coupled into the HCF. I first demonstrate an inertia-sensitive Mach-Zehnder atom interferometer using two counter-propagating Raman beams. However, the short quantum spin coherence time of ∼\SI{100}{\micro\second} due to the differential AC stark shift from the trapping beam is a major obstacle to reaching high sensitivity of the optically trapped atom interferometer inside the HCF. By introducing a vector light shift from the dipole trap to cancel the differential scalar light shift, the quantum spin coherence time is increased to hundreds of milliseconds. The long quantum spin coherence time opens up possibilities for various quantum experiments in HCF. Here, I demonstrate light storage using atoms as the storage medium in the HCF. A maximum storage efficiency of \SI{3}{\percent} and storage time of over \SI{20}{\milli\second} is shown in this thesis. With the implementation of dynamical decoupling, the storage time is improved to ∼\SI{100}{\milli\second}. Moreover, I create a 1D array of Schr\"odinger cats states in facilitated by an optical lattice in the HCF and study its potential for applications in quantum sensing and quantum simulation in HCF. Both odd and even cat states are validated and their coherence properties are studied. This thesis realized the state-of-the-art quantum experiments that are miniaturized into a HCF. The results signify a promise in future quantum sciences and technologies with compact fiber-based devices.
We demonstrate a fiber-guided atom interferometer in a far-off-resonant trap (FORT) of 100 μK. The differential light shift (DLS) introduced by the FORT leads to the inhomogeneous dephasing of the tightly trapped atoms inside a hollow-core fiber. The DLS-induced dephasing is greatly suppressed in π/2-π-π/2 Doppler-insensitive interferometry. The spin coherence time is extended to 13.4 ms by optimizing the coupling of the trapping laser beam into a quasi-single-mode hollow-core anti-resonant fiber. The Doppler-sensitive interferometry shows a much shorter coherence time, indicating that the main limits to our fiber-guided atom interferometer are the wide axial velocity distribution and the irregular modes of the Raman laser beams inside the fiber. This work paves the way for portable and miniaturized quantum devices, which have advantages for inertial sensing at arbitrary orientations and in dynamic environments.
The realization of a large-scale quantum network of interconnected quantum nodes is one of the most promising directions in quantum technology. Such a network distributes entanglement between remote matter qubits via single photons in optical fibers, enabling quantum repeaters and long-distance secure communication and supporting emerging applications such as distributed quantum computing and network-enhanced metrology. To realize this vision, proposed architectures require quantum nodes that provide an efficient quantum light-matter interface for entanglement generation, serve as a quantum memory allowing long-lived storage of quantum states, and have the possibility to connect to telecommunication fiber-based photonic channels. This thesis presents the development and experimental realization of a quantum network node based on a single Rb-87 atom. A single atom is confined in a tightly focused optical dipole trap, and entanglement is generated between the polarization of an emitted photon and the Zeeman state of the atom. To enable long-lived quantum storage, we coherently map the atomic qubit to a basis less sensitive to magnetic fields using Zeeman-state-selective Raman transfer, reducing magnetic field sensitivity by a factor of 500. Such hyperfine qubit control is implemented via a two-photon Raman process driven by a laser field that is amplitude modulated at the qubit splitting using a fiber-based Mach-Zehnder interferometer. With this approach, we achieve a 1/e storage lifetime of 10 ms, extending coherence by a factor of 30 compared with the initial qubit encoding. Residual dephasing arises primarily from position-dependent effective magnetic fields caused by the tightly focused optical dipole trap beam together with atomic motion, and the differential AC-Stark shifts come from the trap detuning. While the first can be fully canceled via a standing-wave dipole trap, which needs to change the trap setup. We mitigate the second effects with a spin-echo pulse, extending coherence by a factor of two. Nonetheless, the significantly longer coherence time already allows high-fidelity entanglement distribution over fiber links with a length of a few hundred kilometers. To reduce fiber attenuation for long-distance distribution, we convert the emitted 780 nm single photons to the low-loss telecom S band using difference-frequency generation in a periodically poled lithium niobate waveguide, pumped at 1607 nm to produce 1517 nm photons. By combining long-lived quantum memory with a telecom interface, we demonstrated long-distance atom-photon entanglement distribution through 50 km and 101 km of spooled fiber with fidelities of 85% and 71%, respectively, establishing a key component for scalable quantum communication. These results establish neutral atom nodes as promising building blocks for metropolitan-scale quantum networking and outline a scalable path toward repeater protocols based on multiplexing memories and Rydberg-mediated interactions.