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arXiv:1904.00893 · Physical Review Letters

Quantum Bath Control with Nuclear Spin State Selectivity via Pulse-Adjusted Dynamical Decoupling

J. E. Lang, David A. Broadway, Gregory A. L. White, Liam T. Hall, Alastair D. Stacey, Lloyd C. L. Hollenberg, T. S. Monteiro, Jean‐Philippe Tetienne

Published Nov 22, 2019• 11 citations
arXivHTMLPDF

Abstract

Dynamical decoupling (DD) is a powerful method for controlling arbitrary open quantum systems. In quantum spin control, DD generally involves a sequence of timed spin flips (π rotations) arranged to either average out or selectively enhance coupling to the environment. Experimentally, errors in the spin flips are inevitably introduced, motivating efforts to optimize error-robust DD. Here we invert this paradigm: by introducing particular control "errors" in standard DD, namely, a small constant deviation from perfect π rotations (pulse adjustments), we show we obtain protocols that retain the advantages of DD while introducing the capabilities of quantum state readout and polarization transfer. We exploit this nuclear quantum state selectivity on an ensemble of nitrogen-vacancy centers in diamond to efficiently polarize the ^{13}C quantum bath. The underlying physical mechanism is generic and paves the way to systematic engineering of pulse-adjusted protocols with nuclear state selectivity for quantum control applications.

DOI
10.1103/physrevlett.123.210401

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Dynamical decoupling (DD) is a powerful method for controlling arbitrary open quantum systems. In quantum spin control, DD generally involves a sequence of timed spin flips (π rotations) arranged to either average out or selectively enhance coupling to the environment. Experimentally, errors in the spin flips are inevitably introduced, motivating efforts to optimize error-robust DD. Here we invert this paradigm: by introducing particular control "errors" in standard DD, namely, a small constant deviation from perfect π rotations (pulse adjustments), we show we obtain protocols that retain the advantages of DD while introducing the capabilities of quantum state readout and polarization transfer. We exploit this nuclear quantum state selectivity on an ensemble of nitrogen-vacancy centers in diamond to efficiently polarize the ^{13}C quantum bath. The underlying physical mechanism is generic and paves the way to systematic engineering of pulse-adjusted protocols with nuclear state selectivity for quantum control applications.
High-fidelity control of quantum systems is crucial for quantum information processing, but is often limited by perturbations from the environment and imperfections in the applied control fields. Here, we investigate the combination of dynamical decoupling (DD) and robust optimal control (ROC) to address this problem. In this combination, ROC is employed to find robust shaped pulses, wherein the directional derivatives of the controlled dynamics with respect to control errors are reduced to a desired order. Then, we incorporate ROC pulses into DD sequences, achieving a remarkable improvement of robustness against multiple error channels. We demonstrate this method in the example of manipulating nuclear spin bath via an electron spin in the nitrogen-vacancy center system. Simulation results indicate that ROC-based DD sequences outperform the state-of-the-art robust DD sequences. Our work has implications for robust quantum control on near-term noisy quantum devices.
We demonstrate a hardware-agnostic protocol for realizing fast, high-fidelity gates through dynamical decoupling (DD) pulse sequences applied to a central qubit coupled to target qubits. The target qubits are controlled by leveraging their intrinsic interaction with the central qubit, eliminating the need for slow, error-prone direct control. We develop and implement the DD-gate protocol within two distinct frameworks: a general model with minimal assumptions, benchmarked on a gate-based digital quantum simulator given by the IBM quantum (IBMQ) platforms; and an experimentally realistic case with a N 15 -vacancy center ( NV 15 ) in diamond. Using IBMQ, we are able to elucidate the underlying quantum dynamics of the DD gates and test them, independently of experimental constraints. For NV 15 , we realize the protocol considering system-specific properties, which could represent a significant reduction in gate duration and improved technological scalability compared with current dynamical-decoupling-based control. We also propose a simple application for high-efficiency polarization of the N 15 nuclear spin that could potentially be less technically demanding than current methods. Altogether, this work provides a robust strategy for quantum control that can be implemented in arbitrary systems fitting the central-target qubit architecture. Beyond these results, our open-source simulations and implementations for both platforms provide a practical framework for simulating time-dependent qubit dynamics on noisy intermediate-scale quantum era gate-based quantum processors.
We demonstrate a hardware-agnostic protocol for realizing fast, high-fidelity gates through dynamical decoupling (DD) pulse sequences applied to a central qubit coupled to target qubits. The target qubits are controlled by leveraging their intrinsic interaction with the central qubit, eliminating the need for slow, error-prone direct control. We develop and implement the DD-gate protocol within two distinct frameworks: a general model with minimal assumptions, benchmarked on a gate-based digital quantum simulator given by the IBM quantum (IBMQ) platforms; and an experimentally realistic case with a 15N-vacancy center (15NV) in diamond. Using IBMQ, we are able to elucidate the underlying quantum dynamics of the DD gates and test them, independently of experimental constraints. For 15NV, we realize the protocol considering system-specific properties, which could represent a significant reduction in gate duration and improved technological scalability compared with current dynamical-decoupling-based control. We also propose a simple application for high-efficiency polarization of the 15N nuclear spin that could potentially be less technically demanding than current methods. Altogether, this work provides a robust strategy for quantum control that can be implemented in arbitrary systems fitting the central-target qubit architecture. Beyond these results, our open-source simulations and implementations for both platforms provide a practical framework for simulating time-dependent qubit dynamics on noisy intermediate-scale quantum era gate-based quantum processors.
Dynamical decoupling (DD) is a popular technique for protecting qubits from the environment. However, unless special care is taken, experimental errors in the control pulses used in this technique can destroy the quantum information instead of preserving it. Here, we investigate techniques for making DD sequences robust against different types of experimental errors while retaining good decoupling efficiency in a fluctuating environment. We present experimental data from solid-state nuclear spin qubits and introduce a new DD sequence that is suitable for quantum computing and quantum memory.
The use of the nuclear spins surrounding electron spin qubits as quantum registers and long-lived memories opens the way to new applications in quantum information and biological sensing. Hence, there is a need for generic and robust forms of control of the nuclear registers. Although adiabatic gates are widely used in quantum information, they can become too slow to outpace decoherence. Here, we introduce a technique whereby adiabatic gates arise from the dynamical decoupling protocols that simultaneously extend coherence. We illustrate this pulse-based adiabatic control for nuclear spins around NV centers in diamond. We obtain a closed-form expression from Landau-Zener theory and show that it reliably describes the dynamics. By identifying robust Floquet states, we show that the technique enables polarization, one-shot flips, and state storage for nuclear spins. These results introduce a control paradigm that combines dynamical decoupling with adiabatic evolution.
Spin ensembles show increasing promise for highly efficient quantum sensing and quantum technologies. However, protecting their coherent properties remains a significant challenge. Dynamical decoupling (DD) typically employs a sequence of fast pulses that aim to reduce the effect of unwanted system-environment interactions. However, the performance of the DD sequences typically suffers in spin ensembles, e.g., due to amplitude and frequency inhomogeneities and control errors. In this work, we compare the performance of an extensive number of DD protocols for coherence protection and quantum sensing in an ensemble of negatively charged NV centers under ambient conditions. We identify the optimal approach that uses rapid adiabatic passage pulses, which are robust to amplitude and frequency inhomogeneity, in combination with the variation of their phases. We experimentally demonstrate an improved signal contrast and an order-of-magnitude increase in memory time with the optimal sequence compared to the widely used XY8 with standard rectangular pulses. We also apply our approach for improved sensing of a weak oscillating field. While our particular demonstration is with NV centers in diamond, the optimized protocol is generally applicable to other spin ensembles and to systems with high amplitude and/or frequency inhomogeneities.