Highly intense electric field pulses can move the electronic momentum occupation in correlated metals over large portions of the Brillouin zone, leading to phenomena such as dynamic Bloch oscillations. Using the nonequilibrium fluctuation-exchange approximation for the two-dimensional Hubbard model, we study how such nonthermal electron distributions drive collective spin and charge fluctuations. Suitable pulses can induce a highly anisotropic modification of the occupied momenta, and the corresponding spin dynamics results in a transient change from antiferromagnetic to anisotropic ferromagnetic correlations. To good approximation this behavior is understood in terms of an instantaneous response of the spin correlations to the single-particle properties.
Highly intense electric field pulses can move the electronic momentum occupation in correlated metals over large portions of the Brillouin zone, leading to phenomena such as dynamic Bloch oscillations. Using the nonequilibrium fluctuation-exchange approximation for the two-dimensional Hubbard model, we study how such nonthermal electron distributions drive collective spin and charge fluctuations. Suitable pulses can induce a highly anisotropic modification of the occupied momenta, and the corresponding spin dynamics results in a transient change from antiferromagnetic to anisotropic ferromagnetic correlations. To good approximation this behavior is understood in terms of an instantaneous response of the spin correlations to the single-particle properties.
Strong antiferromagnetic correlations can radically change the behavior of an otherwise paramagnetic system, inducing anomalous effects in the single particle properties and driving the behavior of spin-spin response functions. In order to investigate such physics, we have studied the momentum distribution function of the two-dimensional Hubbard model at low doping, low temperatures and high values of the on-site Coulomb repulsion. The interpretation of the results has greatly benefited from the parallel analysis of the filling, temperature and interaction dependences of the spin-spin correlation function, the antiferromagnetic correlation length and the pole of the spin-spin propagator. On reducing doping or temperature and on increasing the interaction strength, the correlations become stronger and stronger and the Fermi surface develops hole and electron pockets and shows a dual nature (small-large).
We study the effect of spatially nonlocal correlations on the nonequilibrium dynamics of interacting fermions by constructing the nonequilibrium dynamical cluster theory, a cluster generalization of the nonequilibrium dynamical mean-field theory (DMFT). The formalism is applied to interaction quenches in the Hubbard model in one and two dimensions, and the results are compared with data from single-site DMFT, the time-dependent density matrix renormalization group, and lattice perturbation theory. Both in one and two dimensions the double occupancy quickly thermalizes, while the momentum distribution relaxes only on much longer time scales. For the two-dimensional square lattice we find a strongly momentum-dependent evolution of the momentum distribution around the Fermi energy, with a much faster relaxation near the momenta $(0,\ensuremath{\pi})$ and $(\ensuremath{\pi},0)$ than near $(\ensuremath{\pi}/2,\ensuremath{\pi}/2)$. This result is interpreted as reflecting the momentum-anisotropic quasiparticle lifetime of the marginal Fermi liquid. The method is further applied to the two-dimensional Hubbard model driven by a dc electric field, where the damping of the Bloch oscillation of the current is found to be less effective than predicted by DMFT and lattice perturbation theory.
We examine electron-electron mediated relaxation following ultrafast electric field pump excitation of the fermionic degrees of freedom in the Falicov-Kimball model for correlated electrons. The results reveal a dichotomy in the temporal evolution of the system as one tunes through the Mott metal-to-insulator transition: in the metallic regime relaxation can be characterized by evolution toward a steady state well described by Fermi-Dirac statistics with an increased effective temperature; however, in the insulating regime this quasithermal paradigm breaks down with relaxation toward a nonthermal state with a complicated electronic distribution as a function of momentum. We characterize the behavior by studying changes in the energy, photoemission response, and electronic distribution as functions of time. This relaxation may be observable qualitatively on short enough time scales that the electrons behave like an isolated system not in contact with additional degrees of freedom which would act as a thermal bath, especially when using strong driving fields and studying materials whose physics may manifest the effects of correlations.
The influence of spin and charge fluctuations on spectra of the two-dimensional fermionic Hubbard model is considered using the strong coupling diagram technique. Infinite sequences of diagrams containing ladder inserts, which describe the interaction of electrons with these fluctuations, are summed, and obtained equations are self-consistently solved for the ranges of Hubbard repulsions [Formula: see text], temperatures [Formula: see text] and electron concentrations [Formula: see text] with t the intersite hopping constant. For all considered U the system exhibits a transition to the long-range antiferromagnetic order at [Formula: see text]. At the same time no indication of charge ordering is observed. Obtained solutions agree satisfactorily with results of other approaches and obey moments sum rules. In the considered region of the U-T plane, the curve separating metallic solutions passes from [Formula: see text] at the highest temperatures to U = 2t at [Formula: see text] for half-filling. If only short-range fluctuations are allowed for the remaining part of this region is occupied by insulating solutions. Taking into account long-range fluctuations leads to strengthening of maxima tails, which transform a part of insulating solutions into bad-metal states. For low T, obtained results allow us to trace the gradual transition from the regime of strong correlations with the pronounced four-band structure and well-defined Mott gap for [Formula: see text] to the Slater regime of weak correlations with the spectral intensity having a dip along the boundary of the magnetic Brillouin zone due to an antiferromagnetic ordering for [Formula: see text]. For [Formula: see text] and [Formula: see text] doping leads to the occurrence of a pseudogap near the Fermi level, which is a consequence of the splitting out of a narrow band from a Hubbard subband. Obtained spectra feature waterfalls and Fermi arcs, which are similar to those observed in hole-doped cuprates.
Recent advances in time-resolved spectroscopies have enabled direct access to the momentum-selective nonequilibrium dynamics of correlated quantum materials, revealing a strongly momentum-dependent response of electrons and collective excitations. Interpreting these observations requires a real-time theoretical framework that consistently captures the interplay between strong local electronic correlations and nonlocal collective fluctuations, a capability that remains beyond state-of-the-art nonequilibrium approaches. Using a recently developed real-time many-body framework, we resolve the momentum-selective ultrafast dynamics of a photoexcited correlated electron system. We predict a transient nodal-antinodal anisotropy in electronic heating, providing a microscopic explanation for the momentum-dependent response debated in time-resolved photoemission and Raman experiments, and identify the nonthermal spectral-weight transfer responsible for the transient antinodal in-gap states observed in ultrafast photoemission. We further uncover a momentum-selective magnetic response, in which antiferromagnetic fluctuations undergo a strongly nonthermal, quench-like excitation far above the electronic temperature while preserving their correlation length, before relaxing through a momentum-space magnon cascade toward lower-momentum modes. Finally, by tracking the real-time local spin susceptibility, we identify a dynamical, experimentally accessible signature of local-moment formation and its photoinduced melting. Our results establish a unified microscopic picture of ultrafast electronic and magnetic dynamics, providing a framework for interpreting momentum-resolved pump-probe experiments.
Intense time-periodic laser fields can transform the electronic structure of a solid into strongly modified Floquet-Bloch bands. While this suggests multiple pathways to induce electronic orders such as superconductivity or charge density waves, the possibility of preparing low-energy phases of Floquet Hamiltonians remains unclear because of the energy absorption at typical experimentally accessible driving frequencies. Here we investigate a realistic pathway towards laser control of electronic orders, which is the transient enhancement of fluctuating orders. Using a conserving Keldysh Green's function formalism, we simulate the buildup of short range Cooper-pair correlations out of a normal metal in the driven attractive Hubbard model. Even for frequencies only slightly above or within the bandwidth, a substantial enhancement of correlations can be achieved before the system reaches a high electronic temperature. This behavior relies on the nonthermal nature of the driven state. The effective temperature of the electrons at the Fermi surface, which more closely determines the superconducting correlations, remains lower than an estimate from the global energy density. Even though short ranged, the fluctuations can have marked signatures in the electronic spectra.