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arXiv:1903.05080

Non-stationary dynamics and dissipative freezing in squeezed superradiance

Carlos Sánchez Muñoz, Berislav Buča, Joseph Tindall, Alejandro González-Tudela, Dieter Jaksch, Diego Porras

Published Mar 11, 2019• 6 citations
arXivHTMLPDF

Abstract

In this work, we study the driven-dissipative dynamics of a coherently-driven spin ensemble with a squeezed, superradiant decay. This decay consists of a sum of both raising and lowering collective spin operators with a tunable weight. The model presents different critical non-equilibrium phases with a gapless Liouvillian that are associated to particular symmetries and that give rise to distinct kinds of non-ergodic dynamics. In Ref. [1] we focus on the case of a strong-symmetry and use this model to introduce and discuss the effect of dissipative freezing, where, regardless of the system size, stochastic quantum trajectories initialized in a superposition of different symmetry sectors always select a single one of them and remain there for the rest of the evolution. Here, we deepen this analysis and study in more detail the other type of non-ergodic physics present in the model, namely, the emergence of non-stationary dynamics in the thermodynamic limit. We complete our description of squeezed superradiance by analysing its metrological properties in terms of spin squeezing and by analysing the features that each of these critical phases imprint on the light emitted by the system.

DOI
10.48550/arxiv.1903.05080

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In this work, we study the driven-dissipative dynamics of a coherently-driven spin ensemble with a squeezed, superradiant decay. This decay consists of a sum of both raising and lowering collective spin operators with a tunable weight. The model presents different critical non-equilibrium phases with a gapless Liouvillian that are associated to particular symmetries and that give rise to distinct kinds of non-ergodic dynamics. In Ref. [1] we focus on the case of a strong-symmetry and use this model to introduce and discuss the effect of dissipative freezing, where, regardless of the system size, stochastic quantum trajectories initialized in a superposition of different symmetry sectors always select a single one of them and remain there for the rest of the evolution. Here, we deepen this analysis and study in more detail the other type of non-ergodic physics present in the model, namely, the emergence of non-stationary dynamics in the thermodynamic limit. We complete our description of squeezed superradiance by analysing its metrological properties in terms of spin squeezing and by analysing the features that each of these critical phases imprint on the light emitted by the system.
In driven-dissipative systems, the presence of a strong symmetry guarantees the existence of several steady states belonging to different symmetry sectors. Here we show that when a system with a strong symmetry is initialized in a quantum superposition involving several of these sectors, each individual stochastic trajectory will randomly select a single one of them and remain there for the rest of the evolution. Since a strong symmetry implies a conservation law for the corresponding symmetry operator on the ensemble level, this selection of a single sector from an initial superposition entails a breakdown of this conservation law at the level of individual realizations. Given that such a superposition is impossible in a classical stochastic trajectory, this is a a purely quantum effect with no classical analog. Our results show that a system with a closed Liouvillian gap may exhibit, when monitored over a single run of an experiment, a behavior completely opposite to the usual notion of dynamical phase coexistence and intermittency, which are typically considered hallmarks of a dissipative phase transition. We discuss our results on a coherently driven spin ensemble with a squeezed superradiant decay, a simple model that presents a wealth of nonergodic dynamics.
Abstract We investigate the non-equilibrium dynamics and quantum metrological potential of an ensemble of four-level atoms interacting with a dissipative optical cavity. By deriving an effective master equation for the atomic degrees of freedom, we identify first-order dissipative phase transitions driven by the competition between coherent driving and collective decay. Focusing on a specific parametric trajectory, we employ Liouvillian spectral projections in the thermodynamic limit to rigorously delineate the basins of attraction corresponding to the multistable phases. Furthermore, the mean-field superradiance potential reveals that the dissipative phase transition manifests as a saddle-node bifurcation where a metastable trapping potential vanishes. In the vicinity of the critical point, the system exhibits critical slowing down, leading to a vanishing Liouvillian spectral gap. Utilizing the matrix product state formalism, we demonstrate that due to this dissipative phase transition, the system possesses the potential to achieve Heisenberg-limited precision in continuous sensing. Our results confirm that the driven four-level superradiant model serves as a robust platform for exploiting critical dynamics to enhance metrological performance.
The dissipative quantum Rabi model exhibits rich non-equilibrium physics, including a dissipative phase transition from the normal phase to the superradiant phase. In this work, we investigate the stability of the superradiant phase in the presence of a weak spin relaxation. We find that even a weak spin relaxation can render the superradiant phase a superradiant metastable phase, in which symmetry-breaking states are stable only for a finite time. This arises because each spin jump induced by relaxation applies as a strong perturbation to the system, potentially driving the system from a symmetry-breaking state to the symmetry-preserving saddle point with finite probability, before it eventually relaxes back to a symmetry-breaking state. Such dynamical processes lead to a finite lifetime of the symmetry-breaking states and restore the symmetry in the steady state. To substantiate these results, we combine mean-field and cumulant expansion analyses with exact numerical simulations. The lifetimes of the symmetry-breaking states are analyzed in finite-size systems and the conclusions are extrapolated to the thermodynamic limit via finite-size scaling. Our findings establish the metastable nature of the symmetry-breaking states in the dissipative quantum Rabi model and reveal the complexity of the dissipative phase transition beyond their equilibrium counterpart. The mechanisms uncovered here can be generalized to a broad class of open quantum systems, highlighting fundamental distinctions between equilibrium phase transitions and steady-state phase transitions.
We analyze the properties across steady-state phase transitions of two all-to-all driven-dissipative spin models that describe possible dynamics of NNN two-level systems inside an optical cavity: squeezed superradiance and driven superradiance. We show that the finite size behavior around the critical points can be captured correctly by carefully identifying the relevant nonlinearities in the Holstein-Primakoff representation of spin operators in terms of bosonic variables. With these tools, we calculate analytically various observables across the phase transitions and obtain their finite size scalings, including numerical prefactors. In particular, we look at the amount of spin squeezing carried by the steady states, of relevance for quantum metrology applications, and describe in analytical detail the mechanism by which the optimal spin squeezing acquires logarithmic corrections that depend on the system size. We also demonstrate that the logarithmic nature of these corrections is difficult to characterize through numerical procedures for any experimentally realistic and/or simulable values of particle number. We complement all of our analytical arguments with numerical benchmarks.
Cavity quantum electrodynamics (QED) with quantum emitters coupled to resonators provides a powerful platform for engineering light-matter interactions and exploring collective phenomena. In particular, superradiance, arising from collective quantum interference among emitters, has been explored as a route to ultrastable continuous radiation. However, engineering superradiance in the time domain to realize periodic pulsed sources or frequency combs remains largely unexplored. Here, we investigate the non-equilibrium many-body dynamics of a driven spin ensemble coupled to an on-chip superconducting resonator and uncover a dynamical phase transition from continuous-wave to periodic pulsed superradiant emission. To quantitatively capture the observed dynamical phases, we introduce a driven-dissipative cavity-QED model that elucidates how the periodic pulsed superradiant phase emerges from collective, periodically repeating spin dynamics stabilized by the interplay of coherence growth, disorder, and dissipation. We also find that rare-earth ion spin systems exhibiting both optical and microwave transitions enable phase-synchronized, dual-rail superradiant frequency combs in both the microwave and optical domains. Our results not only open new avenues for dual-rail frequency-comb applications in quantum metrology and information processing, but also establish a fundamental connection between periodic pulsed superradiance and the emergence of a continuous time crystal as a novel nonequilibrium phase in driven open systems.
Superradiance is an extensive cooperative spontaneous emission phenomenon, exhibited by some atomic collective-spin states. However, distinct initial states differ in their decay dynamics. Dicke states ∣j,m⟩|j,m\rangle∣j,m⟩ with distinct numbers of excitations n=m+jn=m+jn=m+j, driven by vacuum fluctuations, have their peak emission intensity shifted in time. Rotating Dicke states relative to the decay axis introduces an interesting parity structure that affects the pulse profile and photon correlations. Squeezed-bath prepared states undergo a squeezing-controlled crossover to the rotated Dicke states, making the emission character dependent on the amount of squeezing transferred from light to the atomic state. For semiclassical states with a macroscopic dipole moment, like the atomic coherent state, the emission intensity depends on their polarization. We present detailed results on the superradiant dynamics of a representative selection of states expanded in Dicke states to highlight the initial state as an independent dynamical control parameter. For large-NNN, we are able to predict fairly accurately the pulse profile in each case using the mean-field approximation, an approach based on the Fokker--Planck equation. We also present comparative results on the intensity correlation function, quantify the coherent and incoherent contributions of the emission, and contrast between small and large ensembles.