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arXiv:1903.02498 · Physical Review Letters

Engineering Quantum States of Matter for Atomic Clocks in Shallow Optical Lattices

Ross B. Hutson, Akihisa Goban, G. Edward Marti, Lindsay Sonderhouse, Christian Sanner, Jun Ye

Published Sep 17, 2019• 52 citations
arXivHTMLPDF

Abstract

We investigate the effects of stimulated scattering of optical lattice photons on atomic coherence times in a state-of-the art ^{87}Sr optical lattice clock. Such scattering processes are found to limit the achievable coherence times to less than 12 s (corresponding to a quality factor of 1×10^{16}), significantly shorter than the predicted 145(40) s lifetime of ^{87}Sr's excited clock state. We suggest that shallow, state-independent optical lattices with increased lattice constants can give rise to sufficiently small lattice photon scattering and motional dephasing rates as to enable coherence times on the order of the clock transition's natural lifetime. Not only should this scheme be compatible with the relatively high atomic density associated with Fermi-degenerate gases in three-dimensional optical lattices, but we anticipate that certain properties of various quantum states of matter-such as the localization of atoms in a Mott insulator-can be used to suppress dephasing due to tunneling.

DOI
10.1103/physrevlett.123.123401

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We investigate the effects of stimulated scattering of optical lattice photons on atomic coherence times in a state-of-the art ^{87}Sr optical lattice clock. Such scattering processes are found to limit the achievable coherence times to less than 12 s (corresponding to a quality factor of 1×10^{16}), significantly shorter than the predicted 145(40) s lifetime of ^{87}Sr's excited clock state. We suggest that shallow, state-independent optical lattices with increased lattice constants can give rise to sufficiently small lattice photon scattering and motional dephasing rates as to enable coherence times on the order of the clock transition's natural lifetime. Not only should this scheme be compatible with the relatively high atomic density associated with Fermi-degenerate gases in three-dimensional optical lattices, but we anticipate that certain properties of various quantum states of matter-such as the localization of atoms in a Mott insulator-can be used to suppress dephasing due to tunneling.
We explore the limits of atomic coherence and measurement precision in a ^{87}Sr optical lattice clock. We perform a detailed characterization of key effects, including lattice Raman scattering and atomic collisions in a shallow lattice configuration, determining a 174(28) s ^{3}P_{0} clock state lifetime. Investigation of atomic coherence across a range of lattice depths and atomic densities reveals decoherence mechanisms related to photon scattering and atomic interaction. At a reduced density, we observe a coherence time of 118(9) s, approaching the fundamental limit set by spontaneous emission. Guided by this coherence understanding, we demonstrate a clock instability for an atomic ensemble of 1.5×10^{-18} at 1 s in fractional frequency units. Our results are important for further advancing the state of the art of an optical lattice clock for fundamental physics applications.
We explore the limits of atomic coherence and measurement precision in a 87Sr optical lattice clock. We perform a detailed characterization of key effects, including lattice Raman scattering and atomic collisions in a shallow lattice configuration, determining a 174(28) s 3P0 clock state lifetime. Investigation of atomic coherence across a range of lattice depths and atomic densities reveals decoherence mechanisms related to photon scattering and atomic interaction. At a reduced density, we observe a coherence time of 118(9) s, approaching the fundamental limit set by spontaneous emission. Guided by this coherence understanding, we demonstrate a clock instability of 1.5E-18 at 1 s in fractional frequency units. Our results are important for further advancing the state-of-the-art of an optical lattice clock for fundamental physics applications.
The quantum metrology with ultra-high precision usually requires the atoms prepared in an ultra-stable environment with well-defined quantum states. Thus, the optical lattice clock system chooses deep lattice potential to trap the ultra-cold atoms. However, building atomic clock in shallow optical lattice can greatly reduce decoherence rate induced by Raman scattering as well as higher order light shift, but tunneling among the lattice sites will cause additional dephasing and strongly broadening of the Rabi spectrum. Here, we periodically drive the shallow 87^{87}87Sr optical lattice clock in the experiment. Counterintuitively, shaking the system can deform the wide broad spectral line into a sharp peak with 5.4Hz line-width. With careful comparison between the theory and experiment, we demonstrate the Rabi frequency and Bloch bands can be simultaneously and independently tuned by adjusting the driving frequency and amplitude. Our work not only provides a different idea for quantum metrology, such as building shallow optical lattice clock in outer space, but also paves the way for quantum simulation of new phase of matter, such as engineering exotic spin orbit coupling Hamiltonian.
Quantum metrology with ultrahigh precision usually requires atoms prepared in an ultrastable environment with well-defined quantum states. Thus, in optical lattice clock systems deep lattice potentials are used to trap ultracold atoms. However, decoherence, induced by Raman scattering and higher order light shifts, can significantly be reduced if atomic clocks are realized in shallow optical lattices. On the other hand, in such lattices, tunneling among different sites can cause additional dephasing and strongly broadening of the Rabi spectrum. Here, in our experiment, we periodically drive a shallow ^{87}Sr optical lattice clock. Counterintuitively, shaking the system can deform the wide broad spectral line into a sharp peak with 5.4 Hz linewidth. With careful comparison between the theory and experiment, we demonstrate that the Rabi frequency and the Bloch bands can be tuned, simultaneously and independently. Our work not only provides a different idea for quantum metrology, such as building shallow optical lattice clock in outer space, but also paves the way for quantum simulation of new phases of matter by engineering exotic spin orbit couplings.
Off-resonant scattering of lattice laser radiation by 87{}^{87}87Sr atoms in the two states 1S0{}^{1}{S}_{0}1S0​ and 3P0{}^{3}{P}_{0}3P0​ and its effect on clock operation are investigated. It is found that Raman scattering eventually limits the achievable frequency instability and thus limits the useful interrogation time in optical lattice clocks at presently used lattice depths.
Optical lattice clocks in space could improve satellite navigation systems and enable new tests of fundamental physics, including gravitational-wave detection and tests of relativity. In microgravity, atoms can tunnel to degenerate neighboring lattice sites, broadening the clock transition and limiting coherence times. We demonstrate Aubry-André localization in a bichromatic optical lattice formed by two magic-wavelength lasers, suppressing tunneling in a horizontal lattice clock emulating free fall. We recover a Fourier-limited clock Rabi spectrum and measure Ramsey coherence times of up to 2 s in shallow lattices, with up to 100-fold improvement over the delocalized regime. These results establish Aubry-André localization as a practical route to controlling tunneling in future space-based clocks, and open a path to operating terrestrial clocks at shallower lattice depths.