Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1902.06657 · Physical Review Letters

Quantum Storage of Frequency-Multiplexed Heralded Single Photons

Alessandro Seri, Dario Lago-Rivera, Andreas Lenhard, Giacomo Corrielli, Roberto Osellame, Margherita Mazzera, Hugues de Riedmatten

Published Aug 22, 2019• 134 citations
arXivHTMLPDF

Abstract

We report on the quantum storage of a heralded frequency-multiplexed single photon in an integrated laser-written rare-earth doped waveguide. The single photon contains 15 discrete frequency modes separated by 261 MHz and spanning across 4 GHz. It is obtained from a nondegenerate photon pair created via cavity-enhanced spontaneous down-conversion, where the heralding photon is at telecom wavelength and the heralded photon is at 606 nm. The frequency-multimode photon is stored in a praseodymium-doped waveguide using the atomic frequency comb (AFC) scheme, by creating multiple combs within the inhomogeneous broadening of the crystal. Thanks to the intrinsic temporal multimodality of the AFC scheme, each spectral bin includes 9 temporal modes, such that the total number of stored modes is about 130. We demonstrate that the storage preserves the nonclassical properties of the single photon, and its normalized frequency spectrum.

DOI
10.1103/physrevlett.123.080502

Related papers

Quantum Storage of Frequency-Multiplexed Heralded Single Photons

Alessandro Seri, Dario Lago-Rivera, Giacomo Corrielli +4 more

Quantum memories for light are important devices in quantum information science, in particular for applications such as quantum networks and quantum repeaters. It has been predicted that multimode quantum memories able to store independently multiple modes would greatly help the scaling of quantum networks by decreasing the entanglement generation time between remote quantum nodes. Current research focuses mostly on time multiplexing in rare-earth doped crystals and in spatial multiplexing in atomic gases. Beyond these demonstrations, rare-earth doped crystals, thanks to their large inhomogeneous broadening, represent a unique quantum system which could also add another degree of freedom for multiplexing, the storage of multiple frequency modes. In this contribution, we report on the first demonstration of quantum storage of a frequency multiplexed single photon into a laser-written waveguide integrated in a Pr3+:Y2SiO5crystal. The great advantage of using a confined waveguide for this task is that the power required to prepare the quantum memory is strongly reduced due to the increased light-matter interaction in the waveguide. This enables simultaneous preparation of several memories at different frequencies, with a moderate laser power.

Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)•Jun 1, 2019•29 citations

Quantum Storage of Frequency-Multiplexed Photons Exhibiting Nonclassical Correlations with Telecom C-Band Photons

Hiroki Tateishi, Daisuke Yoshida, Tomoki Tsuno +6 more

Multiplexing is essential for improving entanglement distribution rates in quantum communication. Frequency multiplexing provides a promising and scalable path toward large-capacity quantum networks. Further progress requires increasing the number of frequency modes and developing broadband photon-pair sources and quantum memories that are spectrally compatible. Here, we report the integration of a cavity-enhanced spontaneous parametric down-conversion source in the telecom C-band with a frequency-multiplexed atomic frequency comb memory. The bow-tie cavity source was simultaneously resonant at 606 nm and 1550 nm, generating non-degenerate photon pairs exhibiting a clustered frequency-comb spectrum. The atomic frequency comb memory, implemented in Praseodymium-doped Yttrium Orthosilicate crystals, provided up to 83 frequency modes with 123 MHz spacing and enabled broadband storage of 606 nm signal photons. By filtering the main cluster, we obtained $32.7 \pm 4.8$ effective modes, as confirmed from coincidence measurements. Importantly, we observed strong nonclassical correlations after storage, with cross-correlation values of $g_{s,i}^{(2)} = 8.1\pm0.7$. Our experimental results demonstrate the feasibility of integrating cavity-enhanced photon-pair sources with rare-earth-ion-doped solid-state memories. The integration reveals a high frequency multiplicity that is essential for scalable quantum networks.

quant-pharXiv:2511.16977•Applied Physics Letters•Nov 24, 2025•0 citations

Quantum Storage of Heralded Single Photons in a Praseodymium-Doped Crystal

Daniel Rieländer, Kutlu Kutluer, Patrick M. Ledingham +4 more

We report on experiments demonstrating the reversible mapping of heralded single photons to long-lived collective optical atomic excitations stored in a Pr3+:Y2SiO5 crystal. A cavity-enhanced spontaneous down-conversion source is employed to produce widely nondegenerate narrow-band (≈2 MHz) photon pairs. The idler photons, whose frequency is compatible with telecommunication optical fibers, are used to herald the creation of the signal photons, compatible with the Pr3+ transition. The signal photons are stored and retrieved using the atomic frequency comb protocol. We demonstrate storage times up to 4.5 μs while preserving nonclassical correlations between the heralding and the retrieved photon. This is more than 20 times longer than in previous realizations in solid state devices, and implemented in a system ideally suited for the extension to spin-wave storage.

arXiv:1310.8261•Physical Review Letters•Jan 31, 2014•92 citations

Single-photon storage in laser written waveguides fabricated in rare-earth-doped solids (Conference Presentation)

Giacomo Corrielli, Alessandro Seri, Dario Lago-Rivera +4 more

Efficient and long-lived multimode quantum memories are crucial devices in the development of quantum technolgies. The reversible mapping of quantum states of light in rare earth doped crystals represents one of the most promising routes towards the realization of this goal. Such systems are also compatible with the miniaturization of quantum memories in integrated optics platforms, which offer unique features in terms of experimental scalability and enhanced light-matter interaction. Here, we fabricate single mode channel waveguides for 606 nm light in a praseodymium-doped yttrium orthosilicate crystal (Pr3+:Y2SiO5), that, thanks to its excellent coherence properties, is a widely studied material for light storage experiments. Waveguides are inscribed by femtosecond laser writing, adopting the so-called Type I configuration, where the core is directly obtained at the irradiated area. Remarkably, fabricating this kind of waveguides in crystals is a difficult task, as it requires to operate in a very narrow processing parameters window, if existing. We then use these waveguides for performing the storage and retrieval of single photons, implementing the atomic frequency comb protocol. We achieve a storage time of 5,5 µs, which is almost 2 orders of magnitude longer than previous realizations of quantum light storage in a waveguide. In addition, we investigate the potential information multiplexing capabilities of our system by performing the quantum storage of single photons delocalized over 14 different spectral modes. Our results show that laser written waveguides in rare earth-doped solid state systems are very promising for the development of efficient and long-lived multimode quantum memories.

Advances in Photonics of Quantum Computing, Memory, and Communication•Mar 4, 2019•0 citations

Storage of 1650 modes of single photons at telecom wavelength

Shihai Wei, Bo Jing, Xueying Zhang +10 more

Abstract To advance the full potential of quantum networks one should be able to distribute quantum resources over long distances at appreciable rates. As a consequence, all components in the networks need to have large multimode capacity to manipulate photonic quantum states. Towards this end, a multimode photonic quantum memory, especially one operating at telecom wavelength, remains a key challenge. Here we demonstrate a spectro-temporally multiplexed quantum memory at 1532 nm. Multimode quantum storage of telecom-band heralded single photons is realized by employing the atomic frequency comb protocol in a 10-m-long cryogenically cooled erbium doped silica fibre. The multiplexing encompasses five spectral channels - each 10 GHz wide - and in each of these up to 330 temporal modes, resulting in the simultaneous storage of 1650 modes of single photons. Our demonstrations open doors for high-rate quantum networks, which are essential for future quantum internet.

•Sep 2, 2022•10 citations

Long-lived telecom-heralded single-photon storage in an absorptive spin-rephased quantum memory

Alberto E. Rodríguez-Moldes, Félicien Appas, Jonathan Hänni +3 more

Long-lived storage of single photons under the form of atomic excitations is at the foundation of long-distance entanglement distribution in quantum networks. To mitigate decoherence effects induced by the environment, rephasing of the hyperfine coherences using microwave pulses have been implemented in a variety of single-emitter and ensemble-based solid-state systems. However, the demonstration of storage of single photons in an absorptive quantum memory including such spin rephasing mechanism remains elusive. In this work, we show non-classical storage of telecom-heralded single photons in a Pr$^{3+}$:Y$_2$SiO$_5$ rare-earth ion doped crystal quantum memory using the atomic frequency comb (AFC) spin-wave protocol combined with a XY4 spin rephasing sequence. Long-lived AFC photon echoes are first observed in the classical regime for storage times of up to approximately 3 ms. We then demonstrate non-classical correlations between heralding photons and stored signal photons generated by a cavity-enhanced parametric photon-pair source for storage times of up to 180 $μ$s and with measured cross-correlation values as high as 4.6(4). Together with the capacity of Pr$^{3+}$:Y$_2$SiO$_5$ QMs to support highly efficient and multiplexed storage, this result represents a significant step towards scalable long-distance quantum repeater links.

quant-pharXiv:2609.02579•Physical Review Letters•Sep 3, 2026•1 citation
We report on the quantum storage of a heralded frequency-multiplexed single photon in an integrated laser-written rare-earth doped waveguide. The single photon contains 15 discrete frequency modes separated by 261 MHz and spanning across 4 GHz. It is obtained from a nondegenerate photon pair created via cavity-enhanced spontaneous down-conversion, where the heralding photon is at telecom wavelength and the heralded photon is at 606 nm. The frequency-multimode photon is stored in a praseodymium-doped waveguide using the atomic frequency comb (AFC) scheme, by creating multiple combs within the inhomogeneous broadening of the crystal. Thanks to the intrinsic temporal multimodality of the AFC scheme, each spectral bin includes 9 temporal modes, such that the total number of stored modes is about 130. We demonstrate that the storage preserves the nonclassical properties of the single photon, and its normalized frequency spectrum.
Quantum memories for light are important devices in quantum information science, in particular for applications such as quantum networks and quantum repeaters. It has been predicted that multimode quantum memories able to store independently multiple modes would greatly help the scaling of quantum networks by decreasing the entanglement generation time between remote quantum nodes. Current research focuses mostly on time multiplexing in rare-earth doped crystals and in spatial multiplexing in atomic gases. Beyond these demonstrations, rare-earth doped crystals, thanks to their large inhomogeneous broadening, represent a unique quantum system which could also add another degree of freedom for multiplexing, the storage of multiple frequency modes. In this contribution, we report on the first demonstration of quantum storage of a frequency multiplexed single photon into a laser-written waveguide integrated in a Pr3+:Y2SiO5crystal. The great advantage of using a confined waveguide for this task is that the power required to prepare the quantum memory is strongly reduced due to the increased light-matter interaction in the waveguide. This enables simultaneous preparation of several memories at different frequencies, with a moderate laser power.
Multiplexing is essential for improving entanglement distribution rates in quantum communication. Frequency multiplexing provides a promising and scalable path toward large-capacity quantum networks. Further progress requires increasing the number of frequency modes and developing broadband photon-pair sources and quantum memories that are spectrally compatible. Here, we report the integration of a cavity-enhanced spontaneous parametric down-conversion source in the telecom C-band with a frequency-multiplexed atomic frequency comb memory. The bow-tie cavity source was simultaneously resonant at 606 nm and 1550 nm, generating non-degenerate photon pairs exhibiting a clustered frequency-comb spectrum. The atomic frequency comb memory, implemented in Praseodymium-doped Yttrium Orthosilicate crystals, provided up to 83 frequency modes with 123 MHz spacing and enabled broadband storage of 606 nm signal photons. By filtering the main cluster, we obtained 32.7±4.832.7 \pm 4.832.7±4.8 effective modes, as confirmed from coincidence measurements. Importantly, we observed strong nonclassical correlations after storage, with cross-correlation values of gs,i(2)=8.1±0.7g_{s,i}^{(2)} = 8.1\pm0.7gs,i(2)​=8.1±0.7. Our experimental results demonstrate the feasibility of integrating cavity-enhanced photon-pair sources with rare-earth-ion-doped solid-state memories. The integration reveals a high frequency multiplicity that is essential for scalable quantum networks.
We report on experiments demonstrating the reversible mapping of heralded single photons to long-lived collective optical atomic excitations stored in a Pr3+:Y2SiO5 crystal. A cavity-enhanced spontaneous down-conversion source is employed to produce widely nondegenerate narrow-band (≈2 MHz) photon pairs. The idler photons, whose frequency is compatible with telecommunication optical fibers, are used to herald the creation of the signal photons, compatible with the Pr3+ transition. The signal photons are stored and retrieved using the atomic frequency comb protocol. We demonstrate storage times up to 4.5 μs while preserving nonclassical correlations between the heralding and the retrieved photon. This is more than 20 times longer than in previous realizations in solid state devices, and implemented in a system ideally suited for the extension to spin-wave storage.
Efficient and long-lived multimode quantum memories are crucial devices in the development of quantum technolgies. The reversible mapping of quantum states of light in rare earth doped crystals represents one of the most promising routes towards the realization of this goal. Such systems are also compatible with the miniaturization of quantum memories in integrated optics platforms, which offer unique features in terms of experimental scalability and enhanced light-matter interaction. Here, we fabricate single mode channel waveguides for 606 nm light in a praseodymium-doped yttrium orthosilicate crystal (Pr3+:Y2SiO5), that, thanks to its excellent coherence properties, is a widely studied material for light storage experiments. Waveguides are inscribed by femtosecond laser writing, adopting the so-called Type I configuration, where the core is directly obtained at the irradiated area. Remarkably, fabricating this kind of waveguides in crystals is a difficult task, as it requires to operate in a very narrow processing parameters window, if existing. We then use these waveguides for performing the storage and retrieval of single photons, implementing the atomic frequency comb protocol. We achieve a storage time of 5,5 µs, which is almost 2 orders of magnitude longer than previous realizations of quantum light storage in a waveguide. In addition, we investigate the potential information multiplexing capabilities of our system by performing the quantum storage of single photons delocalized over 14 different spectral modes. Our results show that laser written waveguides in rare earth-doped solid state systems are very promising for the development of efficient and long-lived multimode quantum memories.
Abstract To advance the full potential of quantum networks one should be able to distribute quantum resources over long distances at appreciable rates. As a consequence, all components in the networks need to have large multimode capacity to manipulate photonic quantum states. Towards this end, a multimode photonic quantum memory, especially one operating at telecom wavelength, remains a key challenge. Here we demonstrate a spectro-temporally multiplexed quantum memory at 1532 nm. Multimode quantum storage of telecom-band heralded single photons is realized by employing the atomic frequency comb protocol in a 10-m-long cryogenically cooled erbium doped silica fibre. The multiplexing encompasses five spectral channels - each 10 GHz wide - and in each of these up to 330 temporal modes, resulting in the simultaneous storage of 1650 modes of single photons. Our demonstrations open doors for high-rate quantum networks, which are essential for future quantum internet.
Long-lived storage of single photons under the form of atomic excitations is at the foundation of long-distance entanglement distribution in quantum networks. To mitigate decoherence effects induced by the environment, rephasing of the hyperfine coherences using microwave pulses have been implemented in a variety of single-emitter and ensemble-based solid-state systems. However, the demonstration of storage of single photons in an absorptive quantum memory including such spin rephasing mechanism remains elusive. In this work, we show non-classical storage of telecom-heralded single photons in a Pr3+^{3+}3+:Y2_22​SiO5_55​ rare-earth ion doped crystal quantum memory using the atomic frequency comb (AFC) spin-wave protocol combined with a XY4 spin rephasing sequence. Long-lived AFC photon echoes are first observed in the classical regime for storage times of up to approximately 3 ms. We then demonstrate non-classical correlations between heralding photons and stored signal photons generated by a cavity-enhanced parametric photon-pair source for storage times of up to 180 μμμs and with measured cross-correlation values as high as 4.6(4). Together with the capacity of Pr3+^{3+}3+:Y2_22​SiO5_55​ QMs to support highly efficient and multiplexed storage, this result represents a significant step towards scalable long-distance quantum repeater links.