The majority of classical dynamical systems are chaotic and exhibit the butterfly effect: a minute change in initial conditions has exponentially large effects later on. But this phenomenon is difficult to reconcile with quantum mechanics. One of the main goals in the field of quantum chaos is to establish a correspondence between the dynamics of classical chaotic systems and their quantum counterparts. In isolated systems in the absence of decoherence, there is such a correspondence in dynamics, but it usually persists only over a short time window, after which quantum interference washes out classical chaos. We demonstrate that quantum mechanics can also play the opposite role and generate exponential instabilities in classically nonchaotic systems within this early-time window. Our calculations employ the out-of-time-ordered correlator (OTOC)-a diagnostic that reduces to the Lyapunov exponent in the classical limit but is well defined for general quantum systems. We show that certain classically nonchaotic models, such as polygonal billiards, demonstrate a Lyapunov-like exponential growth of the OTOC at early times with Planck's-constant-dependent rates. This behavior is sharply contrasted with the slow early-time growth of the analog of the OTOC in the systems' classical counterparts. These results suggest that classical-to-quantum correspondence in dynamics is violated in the OTOC even before quantum interference develops.
The majority of classical dynamical systems are chaotic and exhibit the butterfly effect: a minute change in initial conditions has exponentially large effects later on. But this phenomenon is difficult to reconcile with quantum mechanics. One of the main goals in the field of quantum chaos is to establish a correspondence between the dynamics of classical chaotic systems and their quantum counterparts. In isolated systems in the absence of decoherence, there is such a correspondence in dynamics, but it usually persists only over a short time window, after which quantum interference washes out classical chaos. We demonstrate that quantum mechanics can also play the opposite role and generate exponential instabilities in classically nonchaotic systems within this early-time window. Our calculations employ the out-of-time-ordered correlator (OTOC)-a diagnostic that reduces to the Lyapunov exponent in the classical limit but is well defined for general quantum systems. We show that certain classically nonchaotic models, such as polygonal billiards, demonstrate a Lyapunov-like exponential growth of the OTOC at early times with Planck's-constant-dependent rates. This behavior is sharply contrasted with the slow early-time growth of the analog of the OTOC in the systems' classical counterparts. These results suggest that classical-to-quantum correspondence in dynamics is violated in the OTOC even before quantum interference develops.
We study two classes of quantum phenomena associated with classical chaos in a variety of quantum models: (i) dynamical localization and its extension and generalization to interacting few- and many-body systems and (ii) quantum exponential divergences in high-order correlators and other diagnostics of quantum chaos. Dynamical localization (DL) is a subtle phenomenon related to Anderson localization. It hinges on quantum interference and is typically destroyed in presence of interactions. DL often manifests as a failure of a driven system to heat up, violating the foundations of statistical physics. Kicked rotor (KR) is a prototypical chaotic classical model that exhibits linear energy growth with time. The quantum kicked rotor (QKR) features DL instead: its energy saturates. Multiple attempts of many-body generalizations faced difficulties in preserving DL. Recently, DL was shown in a special integrable many-body model. We study non-integrable models of few- and many-body QKR-like systems and provide direct evidence that DL can persist there. In addition, we show how a novel related concept of localization landscape can be applied to study transport in rippled channels. Out-of-time-ordered correlator (OTOC) was proposed as an indicator of quantum chaos, since in the semiclassical limit, this correlator's possible exponential growth rate (CGR) resembles the classical Lyapunov exponent (LE). We show that the CGR in QKR is related, but distinct from the LE in KR. We also show a singularity in the OTOC at the Ehrenfest time tᴱ due to a delay in the onset of quantum interference. Next, we study scaling of OTOC beyond tᴱ. We then explore how the OTOC-based approach to quantum chaos relates to the random-matrix-theoretical description by introducing an operator we dub the Lyapunovian. Its level statistics is calculated for quantum stadium billiard, a seminal model of quantum chaos, and aligns perfectly with the Wigner-Dyson surmise. In the semiclassical limit, the Lyapunovian reduces to the matrix of uncorrelated finite-time Lyapunov exponents, connecting the CGR at early times, when the quantum effects are weak, to universal level repulsion that hinges on strong quantum interference. Finally, we consider quantum polygonal billiards: their classical counterparts are non-chaotic. We show exponential growth of the OTOCs in these systems, sharply contrasted with the classical behavior even before quantum interference develops.
The exponential growth of the out-of-time-ordered correlator (OTOC) has been proposed as a quantum signature of classical chaos. The growth rate is expected to coincide with the classical Lyapunov exponent. This quantum-classical correspondence has been corroborated for the kicked rotor and the stadium billiard, which are one-body chaotic systems. The conjecture has not yet been validated for realistic systems with interactions. We make progress in this direction by studying the OTOC in the Dicke model, where two-level atoms cooperatively interact with a quantized radiation field. For parameters where the model is chaotic in the classical limit, the OTOC increases exponentially in time with a rate that closely follows the classical Lyapunov exponent.
It was proposed recently that the out-of-time-ordered four-point correlator (OTOC) may serve as a useful characteristic of quantum-chaotic behavior, because, in the semiclassical limit ℏ→0, its rate of exponential growth resembles the classical Lyapunov exponent. Here, we calculate the four-point correlator C(t) for the classical and quantum kicked rotor-a textbook driven chaotic system-and compare its growth rate at initial times with the standard definition of the classical Lyapunov exponent. Using both quantum and classical arguments, we show that the OTOC's growth rate and the Lyapunov exponent are, in general, distinct quantities, corresponding to the logarithm of the phase-space averaged divergence rate of classical trajectories and to the phase-space average of the logarithm, respectively. The difference appears to be more pronounced in the regime of low kicking strength K, where no classical chaos exists globally. In this case, the Lyapunov exponent quickly decreases as K→0, while the OTOC's growth rate may decrease much slower, showing a higher sensitivity to small chaotic islands in the phase space. We also show that the quantum correlator as a function of time exhibits a clear singularity at the Ehrenfest time t_{E}: transitioning from a time-independent value of t^{-1}lnC(t) at t<t_{E} to its monotonic decrease with time at t>t_{E}. We note that the underlying physics here is the same as in the theory of weak (dynamical) localization [Aleiner and Larkin, Phys. Rev. B 54, 14423 (1996)PRBMDO0163-182910.1103/PhysRevB.54.14423; Tian, Kamenev, and Larkin, Phys. Rev. Lett. 93, 124101 (2004)PRLTAO0031-900710.1103/PhysRevLett.93.124101] and is due to a delay in the onset of quantum interference effects, which occur sharply at a time of the order of the Ehrenfest time.
It was proposed recently that the out-of-time-ordered four-point correlator (OTOC) may serve as a useful characteristic of quantum-chaotic behavior, because in the semi-classical limit, ℏ→0, its rate of exponential growth resembles the classical Lyapunov exponent. Here, we calculate the four-point correlator, C(t), for the classical and quantum kicked rotor -- a textbook driven chaotic system -- and compare its growth rate at initial times with the standard definition of the classical Lyapunov exponent. Using both quantum and classical arguments, we show that the OTOC's growth rate and the Lyapunov exponent are in general distinct quantities, corresponding to the logarithm of phase-space averaged divergence rate of classical trajectories and to the phase-space average of the logarithm, respectively. The difference appears to be more pronounced in the regime of low kicking strength, where no classical chaos exists globally. In this case, the Lyapunov exponent vanishes, while the OTOC's growth rate may remain finite corresponding to disconnected local chaotic islands in the phase space. We also show that the quantum correlator as a function of time exhibits a clear singularity at the Ehrenfest time tE: transitioning from a time-independent value of t−1lnC(t) at ttE. We note that the underlying physics here is the same as in the theory of weak (dynamical) localization [Aleiner and Larkin, Phys. Rev. B 54, 14423 (1996); Tian, Kamenev, and Larkin, Phys. Rev. Lett. 93, 124101 (2004)] and is due to a delay in the onset of quantum interference effects, which occur sharply at a time of the order of the Ehrenfest time.
The correspondence principle is a cornerstone in the entire construction of quantum mechanics. This principle has been recently challenged by the observation of an early-time exponential increase of the out-of-time-ordered correlator (OTOC) in classically nonchaotic systems [E. B. Rozenbaum et al., Phys. Rev. Lett. 125, 014101 (2020)PRLTAO0031-900710.1103/PhysRevLett.125.014101]. Here, we show that the correspondence principle is restored after a proper treatment of the singular points. Furthermore, our results show that the OTOC maintains its role as a diagnostic of chaotic dynamics.
We examine three billiard systems -- the cardioid, diamond (Superman), and Sinai billiards -- all of which are known to be classically chaotic. We compute their classical Lyapunov exponents, and using out-of-time-order correlators (OTOCs) in the semi-classical regime, we also derive their quantum Lyapunov exponents. We observe that the classical and quantum Lyapunov exponents are in agreement, strengthening the role of OTOCs as a diagnostic for quantum chaos in billiard systems. At very low temperatures, the OTOC of the Sinai billiard shows sharp growth, a phenomenon absent in the other two billiards. We identify the source of this anomalous behaviour in the geometry of the ground state wave function of the Sinai billiard, which is more sensitive to the curvature of the billiard compared to the other billiards. We also remark on the late-time behaviour of the OTOCs and how the scrambling/Ehrenfest time is related to the temperature of quantum billiards.