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arXiv:1901.06282 · Physical Review Letters

Enhanced Magnetic Sensitivity with Non-Gaussian Quantum Fluctuations

Alexandre Evrard, Vasiliy Makhalov, Thomas Chalopin, Leonid A. Sidorenkov, Jean Dalibard, Raphael Lopes, Sylvain Nascimbène

Published May 1, 2019• 53 citations
arXivHTMLPDF

Abstract

The precision of a quantum sensor can overcome its classical counterpart when its constituents are entangled. In Gaussian squeezed states, quantum correlations lead to a reduction of the quantum projection noise below the shot noise limit. However, the most sensitive states involve complex non-Gaussian quantum fluctuations, making the required measurement protocol challenging. Here we measure the sensitivity of nonclassical states of the electronic spin J=8 of dysprosium atoms, created using light-induced nonlinear spin coupling. Magnetic sublevel resolution enables us to reach the optimal sensitivity of non-Gaussian (oversqueezed) states, well above the capability of squeezed states and about half the Heisenberg limit.

DOI
10.1103/physrevlett.122.173601

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The precision of a quantum sensor can overcome its classical counterpart when its constituents are entangled. In Gaussian squeezed states, quantum correlations lead to a reduction of the quantum projection noise below the shot noise limit. However, the most sensitive states involve complex non-Gaussian quantum fluctuations, making the required measurement protocol challenging. Here we measure the sensitivity of nonclassical states of the electronic spin J=8 of dysprosium atoms, created using light-induced nonlinear spin coupling. Magnetic sublevel resolution enables us to reach the optimal sensitivity of non-Gaussian (oversqueezed) states, well above the capability of squeezed states and about half the Heisenberg limit.
In an ensemble of two-level atoms that can be described in terms of a collective spin, entangled states can be used to enhance the sensitivity of interferometric precision measurements. While non-Gaussian spin states can produce larger quantum enhancements than spin-squeezed Gaussian states, their use requires the measurement of observables that are nonlinear functions of the three components of the collective spin. In this paper we develop strategies that achieve the optimal quantum enhancements using non-Gaussian states produced by a nonlinear one-axis-twisting Hamiltonian, and show that measurement-after-interaction techniques, known to amplify the output signals in quantum parameter estimation protocols, are effective in measuring nonlinear spin observables. Including the presence of the relevant decoherence processes from atomic experiments, we determine analytically the quantum enhancement of non-Gaussian over-squeezed states as a function of the noise parameters for arbitrary atom numbers.
In an ensemble of two-level atoms that can be described in terms of a collective spin, entangled states can be used to enhance the sensitivity of interferometric precision measurements. While non-Gaussian spin states can produce larger quantum enhancements than spin-squeezed Gaussian states, their use requires the measurement of observables that are nonlinear functions of the three components of the collective spin. In this paper we develop strategies that achieve the optimal quantum enhancements using non-Gaussian states produced by a nonlinear one-axis-twisting Hamiltonian, and show that measurement-after-interaction techniques, known to amplify the output signals in quantum parameter estimation protocols, are effective in measuring nonlinear spin observables. Including the presence of the relevant decoherence processes from atomic experiments, we determine analytically the quantum enhancement of non-Gaussian over-squeezed states as a function of the noise parameters for arbitrary atom numbers.
Coherent superposition states of a mesoscopic quantum object play a major role in our understanding of the quantum to classical boundary, as well as in quantum-enhanced metrology and computing. However, their practical realization and manipulation remains challenging, requiring a high degree of control of the system and its coupling to the environment. Here, we use dysprosium atoms-the most magnetic element in its ground state-to realize coherent superpositions between electronic spin states of opposite orientation, with a mesoscopic spin size J = 8. We drive coherent spin states to quantum superpositions using non-linear light-spin interactions, observing a series of collapses and revivals of quantum coherence. These states feature highly non-classical behavior, with a sensitivity to magnetic fields enhanced by a factor 13.9(1.1) compared to coherent spin states-close to the Heisenberg limit 2J = 16-and an intrinsic fragility to environmental noise.
Quantum metrology uses quantum features such as entanglement and squeezing to improve the sensitivity of quantum-limited measurements. Long established as a valuable technique in optical measurements such as gravitational-wave detection, quantum metrology is increasingly being applied to atomic instruments such as matter-wave interferometers, atomic clocks, and atomic magnetometers. Several of these new applications involve dual optical/atomic quantum systems, presenting both new challenges and new opportunities. Here we describe an optical magnetometry system that achieves both shot-noise-limited and projection-noise-limited performance, allowing study of optical magnetometry in a fully-quantum regime [1]. By near-resonant Faraday rotation probing, we demonstrate measurement-based spin squeezing in a magnetically-sensitive atomic ensemble [2-4]. The versatility of this system allows us also to design metrologically-relevant optical nonlinearities, and to perform quantum-noise-limited measurements with interacting photons. As a first interaction-based measurement [5], we implement a non-linear metrology scheme proposed by Boixo et al. with the surprising feature of precision scaling better than the 1/N “Heisenberg limit” [6].
We consider the limitations due to noise (e.g., quantum projection noise and photon shot-noise) on the sensitivity of an idealized atomic magnetometer that utilizes spin squeezing induced by a continuous quantum nondemolition measurement. Such a magnetometer measures spin precession of NNN atomic spins by detecting optical rotation of far-detuned light. We show that for very short measurement times, the optimal sensitivity scales as ${N}^{\ensuremath{-}3/4}$; if strongly squeezed probe light is used, the Heisenberg limit of ${N}^{\ensuremath{-}1}$ scaling can be achieved. However, if the measurement time exceeds ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}/{N}^{1/2}$ in the former case, or ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}/N$ in the latter, where ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}$ is the spin relaxation time, the scaling becomes ${N}^{\ensuremath{-}1/2}$, as for a standard shot-noise-limited magnetometer.
As a cornerstone of quantum science and technology, quantum precision measurement aims to transcend the standard quantum limit (SQL) and achieve sensitivities unattainable by classical approaches by harnessing distinctive quantum resources such as entanglement, squeezing and non-Gaussianity. Within this framework, Gaussian states have historically played a central role, underpinning a series of seminal experimental advances; however, their utility in metrology is fundamentally bounded by theoretical constraints that preclude unlimited gains in measurement precision. In contrast, a growing body of recent research has revealed that non-Gaussian states–endowed with stronger quantum correlations and more pronounced non-classical characteristics — can significantly surpass Gaussian counterparts in key tasks such as phase estimation, quantum imaging and quantum sensing. Under specific conditions, these states even exhibit the potential to approach or saturate the ultimate Heisenberg limit. This review offers a comprehensive overview of the theoretical underpinnings, representative preparation methodologies, experimental progress and emerging applications of non-Gaussian states in quantum metrology. Special attention is devoted to illustrating their transformative potential for the development of next-generation quantum sensors and high-precision measurement instruments, while also addressing prevailing challenges and delineating promising future research trajectories in this rapidly advancing field.