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arXiv:1812.08865 · Nanoscale

Resonance energy transfer and quantum entanglement mediated by epsilon-near-zero and other plasmonic waveguide systems

Ying Li, Andrei Nemilentsau, Christos Argyropoulos

Published Jan 1, 2019• 52 citations
arXivHTMLPDF

Abstract

The resonance energy transfer and entanglement between two-level quantum emitters are typically limited to sub-wavelength distances due to the inherently short-range nature of the dipole-dipole interactions. Moreover, the entanglement of quantum systems is hard to preserve for a long time period due to decoherence and dephasing mainly caused by radiative and nonradiative losses. In this work, we outperform the aforementioned limitations by presenting efficient long-range inter-emitter entanglement and large enhancement of resonance energy transfer between two optical qubits mediated by epsilon-near-zero (ENZ) and other plasmonic waveguide types, such as V-shaped grooves and cylindrical nanorods. More importantly, we explicitly demonstrate that the ENZ waveguide resonant energy transfer and entanglement performance drastically outperforms the other waveguide systems. Only the excited ENZ mode has an infinite phase velocity combined with a strong and homogeneous electric field distribution, which leads to a giant energy transfer and efficient entanglement independent of the emitters' separation distances and nanoscale positions in the ENZ nanowaveguide, an advantageous feature that can potentially accommodate multi-qubit entanglement. Moreover, the transient entanglement can be further improved and become almost independent of the detrimental decoherence effect when an optically active (gain) medium is embedded inside the ENZ waveguide. We also present that efficient steady-state entanglement can be achieved by using a coherent external pumping scheme. Finally, we report a practical way to detect the steady-state entanglement by computing the second-order correlation function. The presented findings stress the importance of plasmonic ENZ waveguides in the design of the envisioned on-chip quantum communication and information processing plasmonic nanodevices.

DOI
10.1039/c9nr05083c

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The resonance energy transfer and entanglement between two-level quantum emitters are typically limited to sub-wavelength distances due to the inherently short-range nature of the dipole-dipole interactions. Moreover, the entanglement of quantum systems is hard to preserve for a long time period due to decoherence and dephasing mainly caused by radiative and nonradiative losses. In this work, we outperform the aforementioned limitations by presenting efficient long-range inter-emitter entanglement and large enhancement of resonance energy transfer between two optical qubits mediated by epsilon-near-zero (ENZ) and other plasmonic waveguide types, such as V-shaped grooves and cylindrical nanorods. More importantly, we explicitly demonstrate that the ENZ waveguide resonant energy transfer and entanglement performance drastically outperforms the other waveguide systems. Only the excited ENZ mode has an infinite phase velocity combined with a strong and homogeneous electric field distribution, which leads to a giant energy transfer and efficient entanglement independent of the emitters' separation distances and nanoscale positions in the ENZ nanowaveguide, an advantageous feature that can potentially accommodate multi-qubit entanglement. Moreover, the transient entanglement can be further improved and become almost independent of the detrimental decoherence effect when an optically active (gain) medium is embedded inside the ENZ waveguide. We also present that efficient steady-state entanglement can be achieved by using a coherent external pumping scheme. Finally, we report a practical way to detect the steady-state entanglement by computing the second-order correlation function. The presented findings stress the importance of plasmonic ENZ waveguides in the design of the envisioned on-chip quantum communication and information processing plasmonic nanodevices.
Multi-qubit entanglement is of paramount importance to perform truly secure quantum optical communication operations. In this work, we present efficient long-range entanglement mediated by plasmonic waveguides operating at their cut-off frequency, where they exhibit an effective epsilon-near-zero (ENZ) response. Only the excited ENZ mode at plasmonic waveguides has a strong and homogeneous electric field distribution compared to different modes excited at groove and rod waveguides, resulting in an efficient two- and multi-qubit entanglement that can persist over extended time periods and long distances. Efficient multipartite entanglement from three equidistantly arranged two-level quantum emitters (qubits) inside the ENZ waveguide is also demonstrated by using three different multi-qubit entanglement criterions, i.e., pairwise concurrence, negativity, and genuine multipartite entanglement. The findings of this work stress the importance of ENZ plasmonic waveguides as an ideal nanophotonic platform to support efficient quantum optical effects.
Multiqubit entanglement is extremely important to perform truly secure quantum optical communication and computing operations. However, the efficient generation of long-range entanglement over extended time periods between multiple qubits randomly distributed in a photonic system remains an outstanding challenge. This constraint is mainly due to the detrimental effects of decoherence and dephasing. To alleviate this issue, we present engineered epsilon-near-zero (ENZ) nanostructures that can maximize the coherence of light–matter interactions at room temperature. We investigate a practical ENZ plasmonic waveguide system, which simultaneously achieves multiqubit entanglement in elongated distances, extended time periods, and, even more importantly, independent of the emitters' positions. More specifically, we present efficient transient entanglement between three and four optical qubits mediated by ENZ with results that can be easily generalized to an arbitrary number of emitters. The entanglement between multiple qubits is characterized by computing the negativity metric applied to the proposed nanophotonic ENZ configuration. The ENZ response is found to be substantially advantageous to boost the coherence between multiple emitters compared to alternative plasmonic waveguide schemes. Finally, the super-radiance collective emission response at the ENZ resonance is utilized to design a high fidelity two-qubit quantum phase gate that can be used in various emerging quantum computing applications.
Abstract Entanglement is paramount in quantum information processing. Many quantum systems suffer from spatial decoherence in distances over a wavelength and cannot be sustained over short time periods due to dissipation. However, long range solutions are required for the development of quantum information processing on chip. Photonic reservoirs mediating the interactions between qubits and their environment are suggested. Recent research takes advantage of extended wavelength inside near-zero refractive index media to solve the long-range problem along with less sensitivity on the position of quantum emitters. However, those recent proposals use plasmonic epsilon near-zero waveguides that are intrinsically lossy. Here, we propose a fully dielectric platform, compatible with the Nitrogen Vacancy (NV) diamond centers on-chip technology, to drastically improve the range of entanglement over 17 free-space wavelengths, or approximatively 12.5 µm, using mu near-zero metamaterials. We evaluate transient and steady state concurrence demonstrating an order of magnitude enhancement compared to previous works. This is, to the best of our knowledge, the first time that such a long distance is reported using this strategy. Moreover, value of the zero time delay second order correlation function g12(2)(0){g}_{12}^{(2)}(0)g12(2)​(0) g 12 ( 2 ) ( 0 ) are provided, showing antibunching signature correlated with a high degree of concurrence.
We demonstrate a plasmonic route to control the collective spontaneous emission of two-level quantum emitters. Superradiance and subradiance effects are observed over distances comparable to the operating wavelength inside plasmonic nanochannels. These plasmonic waveguides can provide an effective epsilon-near-zero operation in their cut-off frequency and Fabry-Pérot resonances at higher frequencies. The related plasmonic resonant modes are found to efficiently enhance the constructive (superradiance) or destructive (subradiance) interference between different quantum emitters located inside the waveguides. By increasing the number of emitters located in the elongated plasmonic channel, the superradiance effect is enhanced at the epsilon-near-zero operation, leading to a strong coherent increase in the collective spontaneous emission rate. In addition, the separation distance between neighboring emitters and their emission wavelengths can be changed to dynamically control the collective emission properties of the plasmonic system. It is envisioned that the dynamic modification between quantum superradiant and subradiant modes will find applications in quantum entanglement of qubits, low-threshold nanolasers and efficient sensors.
We present a a plasmonic route to superradiant and subradiant effects excited by a pair of two-level emitters embedded inside plasmonic nanochannels. These channels can provide an effective epsilon-near-zero (ENZ) response in their cut-off frequency and Fabry-Perot (FP) resonances in higher frequencies. The plasmonic resonant modes are found to enhance the constructive (superradiance) or destructive (subradiance) interference between two different quantum emitters located inside the channels. The separation distance between neighboring emitters and their emission wavelength can be changed to dynamically control the collective emission properties of the plasmonic system. It is envisioned that the dynamic modification between superradiant and subradiant modes will find applications to future quantum communication and computing systems.
We theoretically investigate the entanglement between two well-separated quantum emitters (QEs) mediated by dark-gap-plasmon waveguides. Both the plasmon-QE coupling strength and the energy transfer efficiency between QEs are crucial for entanglement based on analytical results. To overcome the low energy transfer efficiency brought by common plasmonic waveguides, we construct a simple dark-gap-plasmon waveguide. Such a structure consists of two parallel silver nanowires, where dark plasmon modes are formed in the gap between the two nanowires. The leaky (or radiative) feature of propagating plasmons is highly suppressed, which results in the quality factors of the dark plasmon modes reaching the material limit. Thus, the energy transfer efficiency can reach more than 94% with a distance even over ten working wavelengths ($>10\phantom{\rule{4pt}{0ex}}\textmu{}\mathrm{m}$). Meanwhile, by introducing a tip dimer structure in the nanowire gap, the plasmon-QE coupling can reach a strong coupling regime with realistic parameters. The influences from the geometric parameters of the system are also considered. The energy transfer efficiency is robust to the geometric variations due to the dark feature of the plasmon responses.