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arXiv:1811.12232 · Physical Review A

Optical detection and storage of entanglement in plasmonically coupled quantum-dot qubits

Matthew Otten, Stephen K. Gray, G. V. Kolmakov

Published Mar 25, 2019• 12 citations
arXivHTMLPDF

Abstract

Recent proposals and advances in quantum simulations, quantum cryptography, and quantum communications substantially rely on quantum entanglement formation. Contrary to the conventional wisdom that dissipation destroys quantum coherence, coupling with a dissipative environment can also generate entanglement. We consider a system composed of two quantum-dot qubits coupled with a common, damped surface plasmon mode; each quantum dot is also coupled to a separate photonic cavity mode. Cavity quantum electrodynamics calculations show that upon optical excitation by a femtosecond laser pulse, entanglement of the quantum-dot excitons occurs, and the time evolution of the ${g}^{(2)}$ pair correlation function of the cavity photons is an indicator of the entanglement. We also show that the degree of entanglement is conserved during the time evolution of the system. Furthermore, if coupling of the photonic cavity and quantum-dot modes is large enough, the quantum-dot entanglement can be transferred to the cavity modes to increase the overall entanglement lifetime. This latter phenomenon can be viewed as a signature of entangled, long-lived quantum-dot exciton-polariton formation. The preservation of total entanglement in the strong-coupling limit of the cavity--quantum-dot interactions suggests a novel means of entanglement storage and manipulation in high-quality optical cavities.

DOI
10.1103/physreva.99.032339

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Recent proposals and advances in quantum simulations, quantum cryptography, and quantum communications substantially rely on quantum entanglement formation. Contrary to the conventional wisdom that dissipation destroys quantum coherence, coupling with a dissipative environment can also generate entanglement. We consider a system composed of two quantum-dot qubits coupled with a common, damped surface plasmon mode; each quantum dot is also coupled to a separate photonic cavity mode. Cavity quantum electrodynamics calculations show that upon optical excitation by a femtosecond laser pulse, entanglement of the quantum-dot excitons occurs, and the time evolution of the g(2){g}^{(2)}g(2) pair correlation function of the cavity photons is an indicator of the entanglement. We also show that the degree of entanglement is conserved during the time evolution of the system. Furthermore, if coupling of the photonic cavity and quantum-dot modes is large enough, the quantum-dot entanglement can be transferred to the cavity modes to increase the overall entanglement lifetime. This latter phenomenon can be viewed as a signature of entangled, long-lived quantum-dot exciton-polariton formation. The preservation of total entanglement in the strong-coupling limit of the cavity--quantum-dot interactions suggests a novel means of entanglement storage and manipulation in high-quality optical cavities.
Can quantum light reliably generate entanglement in systems with dissipation? Our cavity quantum electrodynamics calculations demonstrate that a single-mode squeezed light source can robustly generate steady-state entanglement between a plasmonically coupled pair of quantum dots. The strong coupling of plasmons to the light source and the pairwise nature of squeezed photon generation enable entanglement between quantum dots. This entanglement, measured as concurrence, can be improved by replacing an entangled photon-pair pulsed source of light with continuous pumping of squeezed photons. Unlike previously introduced schemes, the concurrence is robust against variations in the system parameters. Specifically, the generation of entanglement does not rely on fine-tuning of the plasmon-quantum dot coupling. These results provide a new perspective for robust entangled-state preparation in open quantum systems.
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A quantum dot strongly coupled to a photonic crystal has been recently proposed as a source of entangled photon pairs [R. Johne et al., Phys. Rev. Lett. 100, 240404 (2008)]. The biexction decay via intermediate polariton states can be used to overcome the natural splitting between the exciton states coupled to the horizontally and vertically polarized light modes so that high degrees of entanglement can be expected. We investigate theoretically the features of realistic dot-cavity systems, including the effect of the different oscillator strength of excitons resonances coupled to the different polarizations of light. We show that in this case, an independent adjustment of the cavity resonances is needed in order to keep a high entanglement degree. We also consider the case when the biexciton-exciton transition is also strongly coupled to a cavity mode. We show that a very fast emission rate can be achieved allowing the repetition rates close to the terahertz range. Such fast emission should however be paid for by a very complex tuning of the many strongly coupled resonances involved and by a loss of quantum efficiency. Altogether a strongly coupled dot-cavity system seems to be very promising as a source of entangled photon pairs.
The generation of entanglement between two identical, interacting quantum dots---initially in ground states---by a coherent field and the subsequent time evolution of the entanglement are studied by calculating the concurrence between the two dots. The results predict that while it is possible to generate entanglement (or entanglement of formation, as defined for a mixed state) between the two dots, at no time do the dots become fully entangled to each other or is a maximally entangled Bell state ever achieved. We also observe that the degree of entanglement increases with an increase in the photon number inside the cavity and a decrease in the dot-photon coupling. The behavior of the two-dot system, initially prepared in an entangled state and interacting with thermal light, is also studied.
A system of two or more quantum dots interacting with a dissipative plasmonic nanostructure is investigated in detail by using a cavity quantum electrodynamics approach with a model Hamiltonian. We focus on determining and understanding system configurations that generate multiple bipartite quantum entanglements between the occupation states of the quantum dots. These configurations include allowing for the quantum dots to be asymmetrically coupled to the plasmonic system. Analytical solution of a simplified limit for an arbitrary number of quantum dots and numerical simulations and optimization for the two- and three-dot cases are used to develop guidelines for maximizing the bipartite entanglements. For any number of quantum dots, we show that through simple starting states and parameter guidelines, one quantum dot can be made to share a strong amount of bipartite entanglement with all other quantum dots in the system, while entangling all other pairs to a lesser degree.
Semiconductor quantum dots are among the best sources of on-demand entangled photon pairs. The degree of entanglement, however, is generally limited by the fine structure splitting of exciton states. In this paper, we theoretically investigate the generation of polarization-entangled photon pairs under two-photon excitation and cavity-assisted two-photon emission, both in the weak and strong cavity coupling regimes. We demonstrate and clarify that cavity coupling together with an excitation pulse reduces the degree of entanglement in three different ways. First, in a strong coupling regime, the cavity introduces the unequal ac-Stark shift of horizontally and vertically polarized exciton states, which results in the effective splitting of exciton states. Second, it induces the cross-coupling between the exciton states even in the weak coupling regime, causing the creation of unfavorable two-photon states. Finally, higher excited states of the cavity modes also contribute to the reduction of entanglement. Therefore, in the setting considered here, cavity coupling, which is generally required for the efficient collection of emitted photons, degrades the entanglement both in weak and strong coupling regimes.