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arXiv:1811.10571 · Physical Review A

Extended polarized semiclassical model for quantum-dot cavity QED and its application to single-photon sources

Henk Snijders, D. N. L. Kok, M. F. van de Stolpe, J. A. Frey, Justin Norman, Arthur C. Gossard, John Edward Bowers, Martin P. van Exter, Dirk Bouwmeester, W. Löffler

Published May 4, 2020• 5 citations
arXivHTMLPDF

Abstract

We present a simple extension of the semiclassical model for a two-level system in a cavity, in order to incorporate multiple polarized transitions, such as those appearing in neutral and charged quantum dots (QDs), and two nondegenerate linearly polarized cavity modes. We verify the model by exact quantum master equation calculations and experimentally using a neutral QD in a polarization nondegenerate microcavity, and in both cases we observe excellent agreement. Finally, the usefulness of this approach is demonstrated by optimizing a single-photon source based on polarization postselection, where we find an increase in the brightness for optimal polarization conditions as predicted by the model.

DOI
10.1103/physreva.101.053811

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We present a simple extension of the semiclassical model for a two-level system in a cavity, in order to incorporate multiple polarized transitions, such as those appearing in neutral and charged quantum dots (QDs), and two nondegenerate linearly polarized cavity modes. We verify the model by exact quantum master equation calculations and experimentally using a neutral QD in a polarization nondegenerate microcavity, and in both cases we observe excellent agreement. Finally, the usefulness of this approach is demonstrated by optimizing a single-photon source based on polarization postselection, where we find an increase in the brightness for optimal polarization conditions as predicted by the model.
A polarization degenerate microcavity containing charge-controlled quantum dots (QDs) enables equal coupling of all polarization degrees of freedom of light to the cavity QED system, which we explore through resonant laser spectroscopy. We first measure interference of the two fine-split neutral QD transitions and find very good agreement of this V-type three-level system with a coherent polarization dependent cavity QED model. We also study a charged QD that suffers from decoherence, and find also in this case that availability of the full polarization degrees of freedom is crucial to reveal the dynamics of the QD transitions. Our results pave the way for postselection-free quantum devices based on electron spin-photon polarization entanglement.
A polarization degenerate microcavity containing charge-controlled quantum dots (QDs) enables equal coupling of all polarization degrees of freedom of light to the cavity QED system, which we explore through resonant laser spectroscopy. We first measure interference of the two fine-split neutral QD transitions and find very good agreement of this V-type three-level system with a coherent polarization-dependent cavity QED model. We also study a charged QD that suffers from decoherence and find also in this case that availability of the full-polarization degrees of freedom is crucial to reveal the dynamics of the QD transitions. Our results pave the way for postselection-free quantum devices based on electron-spin--photon polarization entanglement.
Semiconductor quantum dots (QDs) coupled with optical microcavities provide an excellent platform for generating high-performance single-photon sources. However, the current microcavity structures are difficult to solve the tradeoff between single-photon purity and indistinguishability without additional filtering, due to challenges in suppressing broad phonon sideband spectrum and two-photon emission in the practical experiments. To address these issues, we have developed a novel asymmetric microcavity that supports two nondegenerate polarized modes, both resonant with a single quantum dot. One cavity mode is broadband and is used for excitation to reduce two-photon emission intensity, while the other is narrowband and is used for collection to enhance the indistinguishability of single-photon sources. This asymmetric microcavity also has the ability to overcome at least half of the photon efficiency loss under polarization filtering. Moreover, our model has employed an excitation pulse that resonates with cavity modes eliminating spectral distortion of intracavity fields, and efficiently achieving deterministic population inversion of QDs compared to an elliptical cavity. Our scheme paves the way to develop the excellent performance single-photon sources with higher brightness, near-unity purity, and indistinguishability without any additional filtering in practical experiments.
Polarization properties of single photons emitted by optical pumping from a single quantum dot (QD) are studied by using a four-level system model. The model is capable of explaining the polarization uncertainty observed in single photon emission experiments. It is found that the dependence of photon emission efficiency and polarization visibility on pump power are opposite in general cases. By employing QDs with small size and strong carrier confinement, the photon polarization visibility under high pump power can be improved. In addition, embedding a QD into a well designed microcavity is also found to be favourable, whereas the trade-off between high polarization visibility and multi-photon emission is noted.
A single atom in a cavity is the model system of cavity quantum electrodynamics (CQED). The strong coupling regime between the atom and cavity-confined photon corresponds to the reversible exchange of energy between the two modes, and underpins a wide range of CQED phenomena with applications in quantum information science, including for example as quantum logic gates and as sources of entangled states. An important advance was achieved recently when strong coupling between excitons and cavity photons was reported for the first time for localized quantum dots (QDs) in micron-size solid state cavities. This has significance in terms of scalability and integration with other optical devices, and could lead to the emergence of "quantum optics on a chip" technology. However the results presented so far for quantum dots are in the linear regime, corresponding to coupling to the vacuum field (vacuum Rabi splitting); they are not a true QED effect and can equally well be described by classical physics as the coupling between two oscillators. In this paper, we present evidence for a purely quantum phenomenon for the QD/cavity photon system, namely the increase in splitting of the levels when the mean number of photons in the cavity is increased. This corresponds to non-linearities on the single-photon scale: the presence of a single excitation in the cavity changes the level structure, affecting the emission energies for a second photon. Such results are a first step in demonstrating the promise of quantum dots for CQED applications.
Multi-photon lasing has been realized in systems with strong nonlinear interactions between emitters and cavity modes, where single-photon processes are suppressed. Coherence between the internal states of a quantum emitter, or among multiple emitters, plays a key role. Such continuous nonclassical sources of light can find applications in quantum computation, quantum sensing, quantum metrology, and quantum communication. This thesis explores the multi-photon lasing phenomena in various quantum dot-photonic crystal cavity quantum electrodynamic (QED) setups. Exciton-phonon interactions are inevitable in such systems and are incorporated using the polaron-transformed master equation. The Born-Markov approximation is employed to obtain the reduced density matrix rate equation. Using quantum laser theory, we derived the Scully-Lamb laser rate equations and evaluated the single- and multi-photon excess emission rates defined as the difference between emission and absorption rates into the cavity mode without mean-field approximations. We investigated cooperative two-photon lasing, correlated emission lasing, hyperradiant lasing, non-degenerate two-mode two-photon lasing, and continuous variable entanglement in open quantum systems with single or multiple semiconductor quantum dots (two-level, three-level, and four-level) driven coherently/incoherently and coupled to single/ bimodal cavities.