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arXiv:1811.02371 · Physical Review Letters

Certifying Nonclassical Behavior for Negative Keldysh Quasiprobabilities

Patrick P. Potts

Published Mar 18, 2019• 11 citations
arXivHTMLPDF

Abstract

We introduce an experimental test for ruling out classical explanations for the statistics obtained when measuring arbitrary observables at arbitrary times using individual detectors. This test requires some trust in the measurements, represented by a few natural assumptions on the detectors. In quantum theory, the considered scenarios are well captured by von Neumann measurements. These can be described naturally in terms of the Keldysh quasiprobability distribution (KQPD), and the imprecision and backaction exerted by the measurement apparatus. We find that classical descriptions can be ruled out from measured data if and only if the KQPD exhibits negative values. We provide examples based on simulated data, considering the influence of a finite amount of statistics. In addition to providing an experimental tool for certifying nonclassicality, our results bestow an operational meaning upon the nonclassical nature of negative quasiprobability distributions such as the Wigner function and the full counting statistics.

DOI
10.1103/physrevlett.122.110401

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We introduce an experimental test for ruling out classical explanations for the statistics obtained when measuring arbitrary observables at arbitrary times using individual detectors. This test requires some trust in the measurements, represented by a few natural assumptions on the detectors. In quantum theory, the considered scenarios are well captured by von Neumann measurements. These can be described naturally in terms of the Keldysh quasiprobability distribution (KQPD), and the imprecision and backaction exerted by the measurement apparatus. We find that classical descriptions can be ruled out from measured data if and only if the KQPD exhibits negative values. We provide examples based on simulated data, considering the influence of a finite amount of statistics. In addition to providing an experimental tool for certifying nonclassicality, our results bestow an operational meaning upon the nonclassical nature of negative quasiprobability distributions such as the Wigner function and the full counting statistics.
We develop a general framework to investigate fluctuations of non-commuting observables. To this end, we consider the Keldysh quasi-probability distribution (KQPD). This distribution provides a measurement-independent description of the observables of interest and their time-evolution. Nevertheless, positive probability distributions for measurement outcomes can be obtained from the KQPD by taking into account the effect of measurement back-action and imprecision. Negativity in the KQPD can be linked to an interference effect and acts as an indicator for non-classical behavior. Notable examples of the KQPD are the Wigner function and the full counting statistics, both of which have been used extensively to describe systems in the absence as well as in the presence of a measurement apparatus. Here we discuss the KQPD and its moments in detail and connect it to various time-dependent problems including weak values, fluctuating work, and Leggett-Garg inequalities. Our results are illustrated using the simple example of two subsequent, non-commuting spin measurements.
Negative probability values have been widely employed as an indicator of the nonclassicality of quantum systems. Known as a quasiprobability distribution, they are regarded as a useful tool that provides significant insight into the underlying fundamentals of quantum theory when compared to the classical statistics. However, in this approach, an operational interpretation of these negative values with respect to the definition of probability---the relative frequency of occurred event---is missing. An alternative approach is therefore considered where the quasiprobability operationally reveals the negativity of measured quantities. We here present an experimental realization of the operational quasiprobability, which consists of sequential measurements in time. To this end, we implement two sets of polarization measurements of single photons. We find that the measured negativity can be interpreted in the context of selecting measurements, and it reflects the nonclassical nature of photons. Our results suggest a new operational way to unravel the nonclassicality of photons in the context of measurement selection.
Quasiprobability distributions offer a useful way of describing nonclassical features of quantum systems through their departure from classical probability theory. In this work, we investigate the quantification of nonclassicality associated with the Margenau--Hill quasiprobability (MHQ) distribution using its moments, without requiring reconstruction of the full distribution. First we introduce the logarithmic MHQ negativity as a quantifier of nonclassicality, and then derive a hierarchy of rigorous lower bounds in terms of low-order moments. Within the resulting hierarchy, the fourth-moment bound is the strongest among the bounds based on even moments. For qubits, we further derive a tight upper bound on the exact MHQ negativity and identify the corresponding extremal state. We also obtain an optimal positivity threshold based on the fourth moment for arbitrary pairs of qubit observables. Finally, we show that the relevant moments admit exact multicopy representations, providing a route to their estimation using interferometry or classical shadow techniques. Our results establish a moment-based framework for extracting quantitative information about MHQ negativity from a finite set of low-order observables.
Negative probability values have been widely employed as an indicator of the nonclassicality of quantum systems. Known as a quasiprobability distribution, they are regarded as a useful tool that provides significant insight into the underlying fundamentals of quantum theory when compared to the classical statistics. However, in this approach, an operational interpretation of these negative values with respect to the definition of probability-the relative frequency of occurred event-is missing. An alternative approach is therefore considered where the quasiprobability operationally reveals the negativity of measured quantities. We here present an experimental realization of the operational quasiprobability, which consists of sequential measurements in time. To this end, we implement two sets of polarization measurements of single photons. We find that the measured negativity can be interpreted in the context of selecting measurements, and it reflects the nonclassical nature of photons. Our results suggest a new operational way to unravel the nonclassicality of photons in the context of measurement selection.
The Keldysh-ordered full counting statistics is a quasiprobability distribution describing the fluctuations of a time-integrated quantum observable. While it is well known that this distribution can fail to be positive, the interpretation and origin of this negativity has been somewhat unclear. Here, we show how the full counting statistics can be tied to trajectories through Hilbert space, and how this directly connects negative quasiprobabilities to an unusual interference effect. Our findings are illustrated with the example of energy fluctuations in a driven bosonic resonator; we discuss how negative quasiprobability here could be detected experimentally using superconducting microwave circuits.
We show that a Kirkwood-Dirac type quasiprobability distribution is sufficient to reveal any arbitrary quantum resource. This is achieved by demonstrating that it is always possible to identify a set of incompatible measurements that distinguishes between resourceful states and nonresourceful states. The quasiprobability reveals a resourceful quantum state by having at least one quasiprobabilty outcome with a strictly negative numerical value. We also show that there always exists a quasiprobabilty distribution where the total negativity can be interpreted as the geometric distance between a resourceful quantum state to the closest nonresourceful state. It can also be shown that Kirkwood-Dirac type quasiprobability distributions, like the Wigner distribution, can be made informationally complete, in the sense that it can provide complete information about the quantum state while simultaneously revealing nonclassicality whenever a quasiprobability outcome is negative. Moreover, we demonstrate the existence of sufficiently strong anomalous weak values whenever the quasiprobability distribution is negative, which suggests a means to experimentally test such quasiprobability distributions. Since incompatible measurements are necessary in order for the quasiprobability to be negative, this result suggests that measurement incompatibility may underlie any quantum advantage gained from utilizing a nonclassical quantum resource