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arXiv:1811.00481 · Physical Review Letters

Boiling a Unitary Fermi Liquid

Zhenjie Yan, Parth Patel, Biswaroop Mukherjee, Richard J. Fletcher, Julian Struck, Martin W. Zwierlein

Published Mar 6, 2019• 135 citations
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Abstract

We study the thermal evolution of a highly spin-imbalanced, homogeneous Fermi gas with unitarity limited interactions, from a Fermi liquid of polarons at low temperatures to a classical Boltzmann gas at high temperatures. Radio-frequency spectroscopy gives access to the energy, lifetime, and short-range correlations of Fermi polarons at low temperatures T. In this regime, we observe a characteristic T^{2} dependence of the spectral width, corresponding to the quasiparticle decay rate expected for a Fermi liquid. At high T, the spectral width decreases again towards the scattering rate of the classical, unitary Boltzmann gas, ∝T^{-1/2}. In the transition region between the quantum degenerate and classical regime, the spectral width attains its maximum, on the scale of the Fermi energy, indicating the breakdown of a quasiparticle description. Density measurements in a harmonic trap directly reveal the majority dressing cloud surrounding the minority spins and yield the compressibility along with the effective mass of Fermi polarons.

DOI
10.1103/physrevlett.122.093401

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•Feb 1, 2013•0 citations
We study the thermal evolution of a highly spin-imbalanced, homogeneous Fermi gas with unitarity limited interactions, from a Fermi liquid of polarons at low temperatures to a classical Boltzmann gas at high temperatures. Radio-frequency spectroscopy gives access to the energy, lifetime, and short-range correlations of Fermi polarons at low temperatures T. In this regime, we observe a characteristic T^{2} dependence of the spectral width, corresponding to the quasiparticle decay rate expected for a Fermi liquid. At high T, the spectral width decreases again towards the scattering rate of the classical, unitary Boltzmann gas, ∝T^{-1/2}. In the transition region between the quantum degenerate and classical regime, the spectral width attains its maximum, on the scale of the Fermi energy, indicating the breakdown of a quasiparticle description. Density measurements in a harmonic trap directly reveal the majority dressing cloud surrounding the minority spins and yield the compressibility along with the effective mass of Fermi polarons.
We measure radio frequency (rf) spectra of the homogeneous unitary Fermi gas at temperatures ranging from the Boltzmann regime through quantum degeneracy and across the superfluid transition. For all temperatures, a single spectral peak is observed. Its position smoothly evolves from the bare atomic resonance in the Boltzmann regime to a frequency corresponding to nearly one Fermi energy at the lowest temperatures. At high temperatures, the peak width reflects the scattering rate of the atoms, while at low temperatures, the width is set by the size of fermion pairs. Above the superfluid transition, and approaching the quantum critical regime, the width increases linearly with temperature, indicating non-Fermi-liquid behavior. From the wings of the rf spectra, we obtain the contact, quantifying the strength of short-range pair correlations. We find that the contact rapidly increases as the gas is cooled below the superfluid transition.
We investigate the thermal evolution of radio-frequency (RF) spectra of a spin-imbalanced Fermi gas near a Feshbach resonance in which degenerate Fermi-polaron and classical Boltzmann-gas regimes emerge in the low-temperature and high-temperature limits, respectively. By using self-consistent frameworks of strong-coupling diagrammatic approaches, both the ejection and the reserve RF spectra available in cold-atom experiments are analyzed. We find a variety of transfers from Fermi polarons to the Boltzmann gas such that a thermal crossover expected in the weak-coupling regime is shifted to a sharp transition near unitarity and to double-peak coexistence of attractive and repulsive branches in the strong-coupling regime. Our theory provides semiquantitative descriptions for a recent experiment on the ejection RF spectroscopy at unitarity [Z. Yan, P. B. Patel, B. Mukherjee, R. J. Fletcher, J. Struck, and M. W. Zwierlein, Phys. Rev. Lett. 122, 093401 (2019)] and suggests the importance of beyond-two-body correlations in the high-temperature regime due to the absence of Pauli-blocking effects.
Understanding the behavior of an impurity strongly interacting with a Fermi sea is a long-standing challenge in many-body physics. When the interactions are short-ranged, two vastly different ground states exist: a polaron quasiparticle and a molecule dressed by the majority atoms. In the single-impurity limit, it is predicted that at a critical interaction strength, a first-order transition occurs between these two states. Experiments, however, are always conducted in the finite temperature and impurity density regime. The fate of the polaron-to-molecule transition under these conditions, where the statistics of quantum impurities and thermal effects become relevant, is still unknown. Here, we address this question experimentally and theoretically. Our experiments are performed with a spin-imbalanced ultracold Fermi gas with tunable interactions. Utilizing a novel Raman spectroscopy combined with a high-sensitivity fluorescence detection technique, we isolate the quasiparticle contribution and extract the polaron energy, spectral weight, and the contact parameter. As the interaction strength is increased, we observe a continuous variation of all observables, in particular a smooth reduction of the quasiparticle weight as it goes to zero beyond the transition point. Our observation is in good agreement with a theoretical model where polaron and molecule quasiparticle states are thermally occupied according to their quantum statistics. At the experimental conditions, polaron states are hence populated even at interactions where the molecule is the ground state and vice versa. The emerging physical picture is thus that of a smooth transition between polarons and molecules and a coexistence of both in the region around the expected transition.
We show that atomic Fermi mixtures with density and mass imbalance exhibit a rich diversity of scaling laws for the quasiparticle decay rate beyond the quadratic energy and temperature dependence of conventional Fermi liquids. For certain densities and mass ratios, the decay rate is linear, whereas in other cases, it exhibits a plateau. Remarkably, this plateau extends from the deeply degenerate to the high temperature classical regime of the light species. Many of these scaling laws are analogous to what is found in very different systems, including dirty metals, liquid metals, and high temperature plasmas. The Fermi mixtures can in this sense span a whole range of seemingly diverse and separate physical systems. Our results are derived in the weakly interacting limit, making them quantitatively reliable. The different regimes can be detected with radio-frequency spectroscopy.
We show that the measurement of the quasiparticle lifetime can reveal new Fermi liquid regimes in atom mixtures with density and/or mass imbalance. In these recently created mixtures, the existence of two Fermi energies leads to novel and unusual Fermi liquids where the quasiparticle decay rate is no longer quadratic in energy and temperature. For certain densities and mass ratios, the decay rate exhibits a linear scaling similar to that of marginal Femi liquids, whereas in other regimes it exhibits a plateau. It is demonstrated that this novel Fermi liquid behaviour can extend to rather high temperatures which are within current experimental reach. The novel Fermi liquid regimes can be detected with radio-frequency spectroscopy.