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arXiv:1810.08230 · Physical Review Applied

Improved Indirect Control of Nuclear Spins in Diamond N- V Centers

Jingfu Zhang, Swathi S. Hegde, Dieter Suter

Published Dec 20, 2019• 16 citations
arXivHTMLPDF

Abstract

Hybrid spin systems such as the N-$V$ center in diamond are promising candidates for building quantum devices,as they combine useful properties like fast operation based on electron spins, and long storage times based on nuclear spins. Their properties also pose challenges, including the slow response of nuclear spins to external control fields. Here the authors experimentally implement a scheme that allows them to control the nuclear spins of an N-$V$ center system indirectly, via control operations applied to the electron spin. This versatile approach can be implemented over a wide range of magnetic field strengths, and at any temperature.

DOI
10.1103/physrevapplied.12.064047

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Hybrid spin systems such as the N-VVV center in diamond are promising candidates for building quantum devices,as they combine useful properties like fast operation based on electron spins, and long storage times based on nuclear spins. Their properties also pose challenges, including the slow response of nuclear spins to external control fields. Here the authors experimentally implement a scheme that allows them to control the nuclear spins of an N-VVV center system indirectly, via control operations applied to the electron spin. This versatile approach can be implemented over a wide range of magnetic field strengths, and at any temperature.
Hybrid quantum registers consisting of different types of qubits offer a range of advantages as well as challenges. The main challenge is that some types of qubits react only slowly to external control fields, thus considerably slowing down the information processing operations. Here, we propose and demonstrate an indirect control scheme that allows us to control the nuclear spins of an NV center indirectly, by control operations applied to the electron spin, combined with free precession under the anisotropic hyperfine interaction. The scheme provides universal control and we present two typical applications : polarizing the nuclear spin and measuring nuclear spin free induction decay signal, both without applying radio-frequency pulses. This scheme is versatile as it can be implemented over a wide range of magnetic field strengths and at any temperature.
Coherent control and optical readout of the electron spin of the ${}^{29}{\mathrm{SiV}}^{\ensuremath{-}}$ center in diamond have been demonstrated in the literature, with exciting prospects for implementations as memory nodes and spin qubits. Nuclear spins may be even better suited for many applications in quantum information processing due to their long coherence times. Control of the ${}^{29}{\mathrm{SiV}}^{\ensuremath{-}}$ nuclear spin using conventional NMR techniques is feasible, albeit at slow kilohertz rates due to the nuclear spin's low gyromagnetic ratio. In this work we theoretically demonstrate how indirect control using the electron spin-orbit effect can be employed for high-speed, megahertz control of the 29Si^{29}\mathrm{Si}29Si nuclear spin. We discuss the impact of the nuclear spin precession frequency on gate times and the exciting possibility of all-optical nuclear spin control.
Hybrid quantum registers, such as electron-nuclear spin systems, have emerged as promising hardware for implementing quantum information and computing protocols in scalable systems. Nevertheless, the coherent control of such systems still faces challenges. Particularly, the lower gyromagnetic ratios of the nuclear spins cause them to respond slowly to control fields, resulting in gate times that are generally longer than the coherence time of the electron. Here, we demonstrate a scheme for circumventing this problem by indirect control: we apply a small number of short pulses only to the electron and let the full system undergo free evolution under the hyperfine coupling between the pulses. Using this scheme, we realize robust quantum gates in an electron-nuclear spin system, including a Hadamard gate on the nuclear spin and a controlled-NOT gate with the nuclear spin as the target qubit. The durations of these gates are shorter than the electron coherence time, and thus additional operations to extend the system coherence time are not needed. Our demonstration serves as a proof of concept for achieving efficient coherent control of electron-nuclear spin systems, such as nitrogen vacancy centers in diamond. Our scheme is still applicable when the nuclear spins are only weakly coupled to the electron.
Abstract A nitrogen-vacancy (NV) center in a diamond enables the access to an electron spin, which is expected to present highly sensitive quantum sensors. Although exploiting a nitrogen nuclear spin improves the sensitivity, manipulating it using a resonant pulse requires a long gate time owing to its small gyromagnetic ratio. Another technique to control nuclear spins is a conditional rotation gate based on dynamical decoupling, which is faster but unavailable for nitrogen spins owing to the lack of transverse hyperfine coupling with the electron spin. In this study, we generated effective transverse coupling by applying a weak off-axis magnetic field. An effective coupling depends on the off-axis field; the conditional rotation gate on the nitrogen-14 spins of an NV center was demonstrated within 4.2 μs under an 1.8% off-axis field and a longitudinal field of approximately 280 mT. We estimated that a population transfer from the electron to nitrogen spins can be implemented with 8.7 μs. Our method is applicable to an ensemble of NV centers, in addition to a single NV center.
Indirect control of qubits by a quantum actuator has been proposed as an appealing strategy to manipulate qubits that couple only weakly to external fields. While universal quantum control can be easily achieved when the actuator-qubit coupling is anisotropic, the efficiency of this approach is less clear. Here we analyze the time-efficiency of the quantum actuator control. We describe a strategy to find time-optimal control sequence by the quantum actuator and compare their gate times with direct driving, identifying regimes where the actuator control performs faster. As an example, we focus on a specific implementation based on the Nitrogen-Vacancy center electronic spin in diamond (the actuator) and nearby carbon-13 nuclear spins (the qubits).
This thesis describes a series of experiments on the control of the optical properties of the nitrogen-vacancy (NV) center in diamond, and on control of the electron and nuclear spin states associated with the NV center. The NV center is a fluorescing atomic defect center in diamond, consisting of a substitutional nitrogen atom adjacent to a vacancy in the diamond carbon lattice. The electron spin of the NV center can be initialized and read out optically, and coherently manipulated with high fidelity even at room temperature. This unique combination of properties has attracted much attention to the NV center in recent years for application in quantum information technologies. The experiments in this work focus on exploiting the intrinsic hybrid nature of the NV center. The NV center forms a hybrid spin register, as its electron spin is always coupled to the nuclear spin of its own nitrogen nucleus, and can furthermore be coupled to additional nuclear carbon-13 spins in the diamond. In addition, the electronic spin state can be mapped onto the state of a photon, in principle allowing long range transmission of quantum information and measurement-based entanglement of distant NV center registers. The long-term goal is to achieve a large scale quantum network where the different constituents each perform the task they are most well suited for: the stable nuclear spins store the quantum information, photons transfer quantum information over long distances, and the fast electron spin interfaces between spin and photon states. For measurement-based entanglement of distant NV centers it is of primary importance to maximize the emission and detection of coherent photons emitted by the NV center. Spontaneous emission can be controlled and enhanced by coupling an emitter to a photonic cavity. Chapters 3, 4, and 5 of this thesis describe experiments aimed at maximizing the coherent photon emission rate of an NV center by coupling the NV center to a photonic crystal cavity. One of the main challenges is to position a single NV center into the nanometer-sized cavity mode. Chapter 3 describes the development of a nanopositioning technique, which allows diamond nanocrystals ~50 nm in size containing single NV centers to be placed at arbitrary locations on a chip, with nanometer precision. By using a sharp etched tungsten tip, individual nanocrystals can be picked up, moved and placed under real-time imaging with an electron microscope. We explicitly demonstrate that the unique optical and spin properties of the NV center are conserved by the nanopositioning process. In chapter 4, we apply the nanopositioning technique to couple single NV centers contained in a diamond nanocrystals to gallium phosphide photonic crystal cavities. These cavities resonate in the visible with high quality factors, and are designed to have the lowest energy mode coincide with the zero-phonon line of the NV center. Efficient coupling is evidenced by a strong enhancement of NV center emission at the cavity wavelength. The high quality factor of a photonic crystal cavity is a result of careful design and fabrication. The introduction of a nanocrystal may therefore be expected to have a detrimental effect on the optical properties of a cavity. In chapter 5 we investigate the effect of a nanocrystal on the optical properties of photonic crystal cavities. Our simulations and measurements show that the effect of a nanocrystal is in fact only minor, a promising result for future work on cavity-QED systems in the solid state and with diamond defect centers in particular. Understanding and mitigating decoherence is a key challenge for quantum science and technology. The main source of decoherence for solid-state spin systems is the uncontrolled spin bath environment. Chapter 6 describes experiments that exploit quantum control of the NV center and recently developed dynamical decoupling techniques to study the properties of the surrounding bath of spins belonging to single substitutional nitrogen atoms. The coherence properties of a single NV center are affected by changes in the state of the bath spins, allowing a single NV center to be used as a probe to detect bath spin resonances and study the quantum dynamics of the spin bath. We use quantum control of the spin bath to extend the dephasing time of the NV center, important for the application of the NV center in DC magnetometry. In chapter 7 we describe the development and implementation of decoherence protected quantum gates for the hybrid spin register formed by the NV center electron spin that is coupled to the nuclear spin of its own nitrogen atom. Electron and nuclear spins evolve and decohere at vastly different rates, making it challenging to use such a hybrid system as a fully functional quantum register. We create a universal set of two-qubit quantum gates by integrating dynamical decoupling techniques into the gate operation. We demonstrate the power of our gate design by implementing for the first time Grover's quantum search algorithm on a solid-state spin register.