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arXiv:1810.07157 · Physical Review A

Sisyphus optical lattice decelerator

Chun-Chia Chen, Shayne Bennetts, Rodrigo González Escudero, Florian Schreck, Benjamin Pasquiou

Published Aug 1, 2019• 13 citations
arXivHTMLPDF

Abstract

Leading tests of the Standard Model, like measurements of the electron electric dipole moment or of matter-antimatter asymmetry, are built upon our ability to laser-cool atoms and molecules to ultracold temperatures. Unfortunately, laser-cooling remains limited to a minute collection of species with very specific electronic structures. To include more species, such as polyatomic molecules or exotic atoms like antihydrogen, new cooling methods are needed. Here we demonstrate a method based on Sisyphus cooling that was proposed for laser-cooling antihydrogen. In our implementation, atoms are selectively excited to an electronic state whose energy is spatially modulated by an optical lattice, and the ensuing spontaneous decay completes one Sisyphus cycle. We show that this method eliminates many constraints of traditional radiation-pressure-based approaches, while providing similar atom numbers with lower temperatures. This laser-cooling method can be instrumental in bringing new exotic species and molecules to the ultracold regime.

DOI
10.1103/physreva.100.023401

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Leading tests of the Standard Model, like measurements of the electron electric dipole moment or of matter-antimatter asymmetry, are built upon our ability to laser-cool atoms and molecules to ultracold temperatures. Unfortunately, laser-cooling remains limited to a minute collection of species with very specific electronic structures. To include more species, such as polyatomic molecules or exotic atoms like antihydrogen, new cooling methods are needed. Here we demonstrate a method based on Sisyphus cooling that was proposed for laser-cooling antihydrogen. In our implementation, atoms are selectively excited to an electronic state whose energy is spatially modulated by an optical lattice, and the ensuing spontaneous decay completes one Sisyphus cycle. We show that this method eliminates many constraints of traditional radiation-pressure-based approaches, while providing similar atom numbers with lower temperatures. This laser-cooling method can be instrumental in bringing new exotic species and molecules to the ultracold regime.
High-precision hydrogen spectroscopy is an active field which helps to determine the Rydberg constant and proton charge radius, tests bound-state QED, and can search for Beyond Standard Model (BSM) Physics. Additionally, with recent demonstrations of anti-hydrogen trapping and spectroscopy, a new line of investigation is possible whereby hydrogen can be compared to its antimatter counterpart. The next generation of precision hydrogen spectroscopy will likely require additional motional control of the atomic sample - similar to what is possible with heavier elements. Unfortunately, laser cooling - one of the cornerstones of modern precision atomic physics - is difficult in hydrogen due to the vacuum ultraviolet radiation required. Here, we sidestep the challenges inherent in laser cooling and demonstrate a technique whereby we load metastable atoms from a cryogenic beam into a moving optical lattice, decelerate the lattice, and observe a commensurate deceleration of the atoms. Since the optical lattice is governed by standard optoelectronics, this technique represents a robust platform for the motional control of hydrogen. Our technique could enable greater precision in hydrogen spectroscopy and be transferred to exotic simple atoms such as antihydrogen.
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Laser cooling to sub-Doppler temperatures by optical molasses is thought to be inhibited in atoms with unresolved, near-degenerate hyperfine structure in the excited state. We demonstrate that such cooling is possible in one to three dimensions, not only near the standard D2{D}_{2}D2​ line for laser cooling, but over a wide range extending to the D1{D}_{1}D1​ line. Via a combination of Sisyphus cooling followed by adiabatic expansion, we reach temperatures as low as 40 $\ensuremath{\mu}$K, which corresponds to atomic velocities a factor of 2.6 above the limit imposed by a single-photon recoil. Our method requires modest laser power at a frequency within reach of standard frequency-locking methods. It is largely insensitive to laser power, polarization and detuning, magnetic fields, and initial hyperfine populations. Our results suggest that optical molasses should be possible with all alkali-metal species.
We perform magnetically assisted Sisyphus laser cooling of the triatomic free radical strontium monohydroxide (SrOH). This is achieved with principal optical cycling in the rotationally closed P(N^{''}=1) branch of either the X[over ˜]^{2}Σ^{+}(000)↔A[over ˜]^{2}Π_{1/2}(000) or the X[over ˜]^{2}Σ^{+}(000)↔B[over ˜]^{2}Σ^{+}(000) vibronic transitions. Molecules lost into the excited vibrational states during the cooling process are repumped back through the B[over ˜](000) state for both the (100) level of the Sr-O stretching mode and the (02^{0}0) level of the bending mode. The transverse temperature of a SrOH molecular beam is reduced in one dimension by 2 orders of magnitude to ∼750 μK. This approach opens a path towards creating a variety of ultracold polyatomic molecules by means of direct laser cooling.
Laser cooling and trapping are central to modern atomic physics. It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields and a number of Nobel prizes. Prior to the work presented in this thesis, laser cooling had not yet been extended to molecules because of their complex internal structure. However, this complexity makes molecules potentially useful for a wide range of applications. The first direct laser cooling of a molecule and further results we present here provide a new route to ultracold temperatures for molecules. In particular, these methods bridge the gap between ultracold temperatures and the approximately 1 kelvin temperatures attainable with directly cooled molecules (e.g. with cryogenic buffer gas cooling or decelerated supersonic beams). Using the carefully chosen molecule strontium monofluoride (SrF), decays to unwanted vibrational states are suppressed. Driving a transition with rotational quantum number R=1 to an excited state with R'=0 eliminates decays to unwanted rotational states. The dark ground-state Zeeman sublevels present in this specific scheme are remixed via a static magnetic field. Using three lasers for this scheme, a given molecule should undergo an average of approximately 100,000 photon absorption/emission cycles before being lost via unwanted decays. This number of cycles should be sufficient to load a magneto-optical trap (MOT) of molecules. In this thesis, we demonstrate transverse cooling of an SrF beam, in both Doppler and a Sisyphus-type cooling regimes. We also realize longitudinal slowing of an SrF beam. Finally, we detail current progress towards trapping SrF in a MOT. Ultimately, this technique should enable the production of large samples of molecules at ultracold temperatures for molecules chemically distinct from competing methods.
Despite the prominent role of laser cooling in modern atomic physics, with applications ranging from quantum sensors to high-precision spectroscopy and ultracold chemistry, laser cooling techniques are still limited to atoms with simple energy level structure and closed transitions that are accessible by currently available continuous wave (cw) laser sources. Two main obstacles prevent the extension of laser cooling techniques to a variety of atomic species and molecules. The first is associated with technical difficulties in creating cw laser light in the vacuum ultraviolet (VUV) spectral range - the absence of those laser sources prevents laser cooling of simple atoms such as hydrogen, deuterium, and antihydrogen. The second obstacle is associated with complex energy level structure of many atoms and almost all molecules - it permits decay of an excited state into a number of lower-lying states that can be widely separated in energy, which makes laser cooling of such species inefficient and experimentally very challenging.