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arXiv:1809.11097

Polarisation and Transparency of Relativistically Rotating Two-Level Atoms

Calum Maitland, Matteo Clerici, Fabio Biancalana

Published Sep 28, 2018• 0 citations
arXivHTMLPDF

Abstract

Electromagnetism and light-matter interaction in rotating systems is a rich area of ongoing research. We study the interaction of light with a gas of non-interacting two-level atoms confined to a rotating disk. We numerically solve the optical Bloch equations to investigate the how relativistic rotation affects the atoms' polarisation and inversion. The results are used to predict the steady-state stimulated emission seen by an observer at rest with the optical source in the laboratory frame. Competing physical effects due to time dilation and motion-induced detuning strongly modify solutions to the Bloch equations when the gas's velocity becomes relativistic. We account for the non-inertial motion by including acceleration-dependent excitation and emission rates, arising from a generalised Unruh effect. The effective thermal vacuum resulting from large accelerations de-polarises the gas while driving it towards population inversion, negating coherent driving due to the external light source. The results illustrate the intuitive, special-relativistic approach of assigning instantaneously comoving frames to understand non-inertial motion's influence when only local fields are physically significant.

DOI
10.48550/arxiv.1809.11097

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Electromagnetism and light-matter interaction in rotating systems is a rich area of ongoing research. We study the interaction of light with a gas of non-interacting two-level atoms confined to a rotating disk. We numerically solve the optical Bloch equations to investigate the how relativistic rotation affects the atoms' polarisation and inversion. The results are used to predict the steady-state stimulated emission seen by an observer at rest with the optical source in the laboratory frame. Competing physical effects due to time dilation and motion-induced detuning strongly modify solutions to the Bloch equations when the gas's velocity becomes relativistic. We account for the non-inertial motion by including acceleration-dependent excitation and emission rates, arising from a generalised Unruh effect. The effective thermal vacuum resulting from large accelerations de-polarises the gas while driving it towards population inversion, negating coherent driving due to the external light source. The results illustrate the intuitive, special-relativistic approach of assigning instantaneously comoving frames to understand non-inertial motion's influence when only local fields are physically significant.
We show that, in addition to the Unruh effect, there exist two new phenomena that are due to acceleration in the quantum theory of the light-matter interaction. The first is the phenomenon of acceleration-induced transparency which arises since acceleration impacts not only the counter-rotating terms in the light-matter interaction (the cause of the conventional Unruh effect) but also the rotating wave terms. The second new phenomenon is that the Unruh effect can be stimulated, a phenomenon that arises since not only rotating-wave terms can be stimulated (as in conventional stimulated emission) but also counter-rotating terms. The new phenomena are potentially strong enough to be experimentally observable.
When a gas of ultracold atoms is suddenly illuminated by light that is nearly resonant with an atomic transition, the atoms cannot respond instantaneously. This noninstantaneous response means the gas is initially more transparent to the applied light than in steady state. The timescale associated with the development of light absorption is set by the atomic excited-state lifetime. Similarly, the index of refraction in the gas also requires time to reach a steady-state value, but the development of the associated phase response is expected to be slower than absorption effects. Faraday rotation is one manifestation of differing indices of refraction for orthogonal circular light polarization components. We have performed experiments measuring the time-dependent development of polarization rotation in an ultracold gas subjected to a magnetic field. Our measurements match theoretical predictions based on solving optical Bloch equations. We are able to identify how parameters such as steady-state optical thickness and applied magnetic field strength influence the development of Faraday rotation.
Recently, a new physical picture for the spontaneous excitation of a uniformly accelerated two-level atom has been put forward [1]. Following a quantum optical approach it is based on the distinction of the two competing mechanisms which operate to excite an atom in the quantum vacuum: vacuum fluctuations and radiation reaction. Vacuum fluctuations tend to excite an atom in its ground state and de-excite it in an excited state. On the other hand, radiation reaction leads always to a loss of internal excitation energy. For an inertial atom in the ground state, the two contributions cancel exactly, so that a very sublime balance between vacuum fluctuations and radiation reaction prevents the spontaneous excitation of the atom [2]. If the atom is in the excited state, both contribution add up to the well-known spontaneous emission rate. It has been shown in [1] that uniform acceleration will disturb this balance. Spontaneous transitions from the ground state to the excited state become possible: the Unruh effect [3].
We study interactions of light with a sample of two-level atoms. Quantum statistical effects of degenerate boson and fermion gases are described by using the quantum field theory of atom-photon interactions, fully including the angular momentum degeneracies. Coupled propagation equations are given for light and matter fields, and plausible general simplifications are enumerated.^ In the limit of large atom-field detuning, multiple scattering of light and QED linewidths and line shifts may be ignored, and the propagation equations of light and matter fields may be decoupled. A general expression for the spectrum of the scattered light is derived, complete with the dependence on atomic level scheme, on various light polarizations, and on the geometry of the experiment. With these simplifications we are able to find distinct qualitative features in the spectrum of the scattered light in the case of both fermions and bosons that depend on the statistics of atoms. This is because for bosons (fermions), those scattering events in which an atom recoils to an already occupied state are enhanced (inhibited).^ As the driving light gets closer to the atomic resonance, multiple scattering and vacuum fluctuations of the electromagnetic fields should also be taken into account. We write the equations of motion for the excited state field operators by eliminating the vacuum electromagnetic field. It is always assumed that the driving external laser field is in the coherent state. We find in the limit of low light intensity, a hierarchy of equations of motion for correlation functions that contain one excited-atom field and one, two, three, etc., ground state atom fields. It is conjectured that the entire linear hierarchy may be solved by solving numerically the classical equations for the coupled system of electromagnetic fields and charged harmonic oscillators. We discuss the emergence of resonant dipole-dipole interactions and collective linewidths, and delineate the limits of validity of the column density approach in terms of non-cooperative atoms by presenting a mathematical example in which this approach is exact. ^
I study the coherent interaction of a three-level atom in the lambda configuration with pump, Stoke, and anti-Stokes laser fields. The pump laser field drives transitions from the two non-degenerate lower levels to the excited state which is highly detuned for either transition. This excited state is also coupled to each of the lower states by Stokes or anti-Stokes transitions so that this system may represent a model of four-wave mixing. Assuming large detunings, the excited state is adiabatically eliminated from obtaining an effective two-level system with Raman coupling between the levels. Optical Bloch equations are obtained for this effective two-level system, and phenomenological damping terms are added for collisional dephasing of the Raman transitions. The equations are solved for the steady-state as well as by the method of adiabatic following. From these solutions we obtain the polarization.
We propose and develop a method for theoretical description of circularly (elliptically) polarized optical pulse resonant coherent interactions with two-level atoms. The method is based on the time-evolution equations of a two-level quantum system in the presence of a time-dependent dipole perturbation for electric dipole transitions between states with total angular-momentum projection difference $(\ensuremath{\Delta}{J}_{z}=\ifmmode\pm\else\textpm\fi{}1)$ excited by a circularly polarized electromagnetic field [Feynman et al., J. Appl. Phys. 28, 49 (1957)]. The adopted real-vector representation approach allows for coupling with the vectorial Maxwell's equations for the optical wave propagation and thus the resulting Maxwell pseudospin equations can be numerically solved in the time domain without any approximations. The model permits a more exact study of the ultrafast coherent pulse propagation effects taking into account the vector nature of the electromagnetic field and hence the polarization state of the optical excitation. We demonstrate self-induced transparency effects and formation of polarized solitons. The model represents a qualitative extension of the well-known optical Maxwell-Bloch equations valid for linearly polarized light and a tool for studying coherent quantum control mechanisms.