We develop a formalism for modelling exact time dynamics in waveguide quantum electrodynamics (QED) using the real-space approach. The formalism does not assume any specific configuration of emitters and allows the study of Markovian dynamics fully analytically and non-Markovian dynamics semi-analytically with a simple numerical integration step. We use the formalism to study subradiance, superradiance and bound states in continuum. We discuss new phenomena such as subdivision of collective decay rates into symmetric and anti-symmetric subsets and non-Markovian superradiance effects that can lead to collective decay stronger than Dicke superradiance. We also discuss possible applications such as pulse-shaping and coherent absorption. We thus broaden the range of applicability of real-space approaches beyond steady-state photon transport.
We develop a formalism for modelling exact time dynamics in waveguide quantum electrodynamics (QED) using the real-space approach. The formalism does not assume any specific configuration of emitters and allows the study of Markovian dynamics fully analytically and non-Markovian dynamics semi-analytically with a simple numerical integration step. We use the formalism to study subradiance, superradiance and bound states in continuum. We discuss new phenomena such as subdivision of collective decay rates into symmetric and anti-symmetric subsets and non-Markovian superradiance effects that can lead to collective decay stronger than Dicke superradiance. We also discuss possible applications such as pulse-shaping and coherent absorption. We thus broaden the range of applicability of real-space approaches beyond steady-state photon transport.
An array of initially excited emitters coupled to a one-dimensional waveguide exhibits superradiant decay under the Born-Markov approximation, manifested as a coherent burst of photons in the output field. In this work, we employ tensor-network methods to investigate its non-Markovian dynamics induced by finite time delays in photon exchange among the emitters. We find that the superradiant burst breaks into a structured train of correlated photons, each intensity peak corresponding to a specific photon number. We quantify the emitter-photon and emitter-emitter entanglement generated during this process and show that the latter emerges in the long-time limit, as part of the excitation becomes trapped within the emitters' singlet subspace. We finally consider the decay of the system's most radiant state, the symmetric Dicke state, and show that time delay can lead to decay rates exceeding those predicted by the Markovian approximation.
Spontaneous emission of a quantum emitter, such as an excited atom, is a fundamental process in quantum electrodynamics (QED), typically associated with exponential decay to the ground state accompanied by irreversible photon emission. This simple Markovian picture, however, is profoundly modified in the presence of time-delayed feedback, structured continua, or cooperative emission, as occurs when an emitter radiates in front of a mirror, when several emitters radiate collectively, or in the case of a giant atom. In such regimes, strong non-Markovian dynamics arise from photon reabsorption and interference effects, leading to pronounced deviations from exponential decay. Here we demonstrate the emergence of exceptional points (EPs) in these highly non-Markovian waveguide-QED environments, i.e., non-Markovian EPs. These EPs appear directly in the relaxation dynamics as sharp transitions to oscillatory behavior, manifested by the appearance of real zeros in the excited-state amplitude. We analyze in detail the spontaneous emission of giant atoms with two or more coupling points, highlighting the mechanisms leading to non-Markovian EPs, and show that similar phenomena arise in other waveguide-QED settings, such as the collective spontaneous emission of spatially separated point-like emitters. Our results reveal waveguide-QED systems as experimentally accessible platforms for realizing and exploring non-Markovian EP physics.
Non-Markovian time evolution of quantum systems is a challenging problem, often mitigated by employing numerical methods or making simplifying assumptions. In this work, we address this problem in waveguide quantum electrodynamics (QED) by developing a diagrammatic approach, which performs fully analytical non-Markovian time evolution of single-photon states. By revisiting Fermi's two-atom problem, we tackle the impeding question of whether the rotating-wave approximation violates causality in single-photon waveguide QED. Afterward, we introduce and prove the no upper half-plane poles (no-UHP) theorem, which connects the poles of scattering parameters to the causality principle. Finally, we visualize the time-delayed coherent quantum feedback mediated by the field and discuss the Markovian limit for microscopically separated qubits where short-distance causality violations occur and the emergence of collective decay rates in this limit. Our diagrammatic approach is a method to perform exact and analytical non-Markovian time evolution of multiemitter systems in waveguide QED.
Waveguide quantum electrodynamics constitutes a modern paradigm for the interaction of light and matter, in which strong coupling, bath structure, and propagation delays can break the radiative conditions that quantum emitters typically encounter in free space. These characteristics intertwine the excitations of quantum emitters and guided radiation modes to form complex multiphoton dynamics. So far, combining the collective decay of the emitters with the non-Markovian effects induced by the modes has escaped a full solution and the detailed physics behind these systems remains unknown. Here we analyze such a collective non-Markovian decay in a minimal system of two excited emitters coupled to a one-dimensional single-band waveguide. We develop an exact solution for this system in terms of elementary functions that unveils hidden symmetries and predicts new forms of spontaneous decay. The collective non-Markovian dynamics, which are strongly dependent on the vacuum coupling and the detuning from the center of the band, show exotic features that can be characterized with a simple and readily available criterion. Our analytic methods shed light on the complexity of collective light-matter interactions and open up a pathway for understanding multiparticle open quantum systems. Published by the American Physical Society 2024
We study the collective decay of two-level emitters coupled to a nonlinear waveguide, for example, a nanophotonic lattice or a superconducting resonator array with strong photon-photon interactions. Under these conditions, a new decay channel into bound photon pairs emerges, through which spatial correlations between emitters are established by regular interference as well as interactions between the photons. We derive an effective Markovian theory to model the resulting decay dynamics of an arbitrary distribution of emitters and identify collective effects beyond the usual phenomena of super- and subradiance. Specifically, in the limit of many close-by emitters, we find that the system undergoes a supercorrelated decay process where all the emitters are either in the excited state or in the ground state but not in any of the intermediate states. The predicted effects can be probed in state-of-the-art waveguide QED experiments and provide a striking example of how the dynamics of open quantum systems can be modified by many-body effects in a nonharmonic environment.
Abstract This work introduces a theoretical framework to model the collective dynamics of quantum emitters in highly non-Markovian environments, interacting through the exchange of photons with significant retardations. The formalism consists on a set of coupled delay differential equations for the emitter’s raising/lowering operators σ i ± , supplemented by input–output relations that describe the field mediating the interactions. These equations capture the dynamics of both linear (bosonic) and nonlinear (two-level) emitter arrays. It is exact in some limits—e.g. bosonic emitters or generic systems with up to one collective excitation—and can be integrated to provide accurate results for larger numbers of photons. These equations support a study of collective spontaneous emission of emitter arrays in open waveguide-QED environments. This study uncovers an effect we term cascaded super- and sub-radiance, characterized by light-cone-limited propagation and increasingly correlated photon emission across distant emitters. The collective nature of this dynamics for two-level systems is evident both in the enhancement of collective emission rates, as well as in a superradiant burst with a faster than linear growth. While these effects should be observable in existing circuit QED devices or slight generalizations thereof, the formalism put forward in this work can be extended to model other systems such as network of quantum emitters or the generation of correlated photon states.